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Title: Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids

We present an optical technique based on ultrafast photoacoustics to determine the local temperature distribution profile in liquid samples in contact with a laser heated optical transducer. This ultrafast pump-probe experiment uses time-domain Brillouin scattering (TDBS) to locally determine the light scattering frequency shift. As the temperature influences the Brillouin scattering frequency, the TDBS signal probes the local laser-induced temperature distribution in the liquid. Here, we demonstrate the relevance and the sensitivity of this technique for the measurement of the absolute laser-induced temperature gradient of a glass forming liquid prototype, glycerol, at different laser pump powers—i.e., different steady state background temperatures. Complementarily, our experiments illustrate how this TDBS technique can be applied to measure thermal diffusion in complex multilayer systems in contact with a surrounding liquid.
Authors:
 [1] ;  [2] ;  [2] ;  [1] ; ORCiD logo [3] ;  [2] ;  [1]
  1. Univ. du Maine, Le Mans (France). Inst. Molecules et Materiaux du Mans
  2. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Chemistry
  3. Univ. du Maine, Le Mans (France). Lab. d'Acoustique de l' Univ. du Maine
Publication Date:
Grant/Contract Number:
FG02-00ER15087
Type:
Accepted Manuscript
Journal Name:
Review of Scientific Instruments
Additional Journal Information:
Journal Volume: 88; Journal Issue: 7; Journal ID: ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)
Research Org:
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 47 OTHER INSTRUMENTATION
OSTI Identifier:
1474332
Alternate Identifier(s):
OSTI ID: 1371600

Chaban, Ievgeniia, Shin, Hyun D., Klieber, Christoph, Busselez, Rémi, Gusev, Vitalyi E., Nelson, Keith A., and Pezeril, Thomas. Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids. United States: N. p., Web. doi:10.1063/1.4993132.
Chaban, Ievgeniia, Shin, Hyun D., Klieber, Christoph, Busselez, Rémi, Gusev, Vitalyi E., Nelson, Keith A., & Pezeril, Thomas. Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids. United States. doi:10.1063/1.4993132.
Chaban, Ievgeniia, Shin, Hyun D., Klieber, Christoph, Busselez, Rémi, Gusev, Vitalyi E., Nelson, Keith A., and Pezeril, Thomas. 2017. "Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids". United States. doi:10.1063/1.4993132. https://www.osti.gov/servlets/purl/1474332.
@article{osti_1474332,
title = {Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids},
author = {Chaban, Ievgeniia and Shin, Hyun D. and Klieber, Christoph and Busselez, Rémi and Gusev, Vitalyi E. and Nelson, Keith A. and Pezeril, Thomas},
abstractNote = {We present an optical technique based on ultrafast photoacoustics to determine the local temperature distribution profile in liquid samples in contact with a laser heated optical transducer. This ultrafast pump-probe experiment uses time-domain Brillouin scattering (TDBS) to locally determine the light scattering frequency shift. As the temperature influences the Brillouin scattering frequency, the TDBS signal probes the local laser-induced temperature distribution in the liquid. Here, we demonstrate the relevance and the sensitivity of this technique for the measurement of the absolute laser-induced temperature gradient of a glass forming liquid prototype, glycerol, at different laser pump powers—i.e., different steady state background temperatures. Complementarily, our experiments illustrate how this TDBS technique can be applied to measure thermal diffusion in complex multilayer systems in contact with a surrounding liquid.},
doi = {10.1063/1.4993132},
journal = {Review of Scientific Instruments},
number = 7,
volume = 88,
place = {United States},
year = {2017},
month = {7}
}

Works referenced in this record:

Nanoscale thermal transport
journal, January 2003
  • Cahill, David G.; Ford, Wayne K.; Goodson, Kenneth E.
  • Journal of Applied Physics, Vol. 93, Issue 2, p. 793-818
  • DOI: 10.1063/1.1524305