DNA-Mediated Size-Selective Nanoparticle Assembly for Multiplexed Surface Encoding
Abstract
Multiplexed surface encoding is achieved by positioning two different sizes of gold nanocubes on gold surfaces with precisely defined locations for each particle via template-confined, DNA-mediated nanoparticle assembly. As a proof-of-concept demonstration, cubes with 86 and 63 nm edge lengths are assembled into arrangements that physically and spectrally encrypt two sets of patterns in the same location. These patterns can be decrypted by mapping the absorption intensity of the substrate at $$λ$$ = 773 and 687 nm, respectively. This multiplexed encoding platform dramatically increases the sophistication and density of codes that can be written using colloidal nanoparticles, which may enable high-security, high-resolution encoding applications.
- Authors:
-
[2];
[1];
[1];
[2];
[4]
- Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering, and International Inst. for Nanotechnology
- Northwestern Univ., Evanston, IL (United States). International Inst. for Nanotechnology, and Dept. of Electrical Engineering
- Northwestern Univ., Evanston, IL (United States). International Inst. for Nanotechnology, and Dept. of Chemistry
- Northwestern Univ., Evanston, IL (United States). International Inst. for Nanotechnology, Dept. of Chemistry, and Dept. of Materials Science and Engineering
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Bio-Inspired Energy Science (CBES)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1470552
- Grant/Contract Number:
- SC0000989
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 18; Journal Issue: 4; Related Information: CBES partners with Northwestern University (lead); Harvard University; New York University; Pennsylvania State University; University of Michigan; University of Pittsburgh; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 42 ENGINEERING; 77 NANOSCIENCE AND NANOTECHNOLOGY; catalysis (homogeneous); solar (photovoltaic); bio-inspired; charge transport; mesostructured materials; materials and chemistry by design; synthesis (novel materials); synthesis (self-assembly)
Citation Formats
Lin, Qing-Yuan, Palacios, Edgar, Zhou, Wenjie, Li, Zhongyang, Mason, Jarad A., Liu, Zizhuo, Lin, Haixin, Chen, Peng-Cheng, Dravid, Vinayak P., Aydin, Koray, and Mirkin, Chad A. DNA-Mediated Size-Selective Nanoparticle Assembly for Multiplexed Surface Encoding. United States: N. p., 2018.
Web. doi:10.1021/acs.nanolett.8b00509.
Lin, Qing-Yuan, Palacios, Edgar, Zhou, Wenjie, Li, Zhongyang, Mason, Jarad A., Liu, Zizhuo, Lin, Haixin, Chen, Peng-Cheng, Dravid, Vinayak P., Aydin, Koray, & Mirkin, Chad A. DNA-Mediated Size-Selective Nanoparticle Assembly for Multiplexed Surface Encoding. United States. https://doi.org/10.1021/acs.nanolett.8b00509
Lin, Qing-Yuan, Palacios, Edgar, Zhou, Wenjie, Li, Zhongyang, Mason, Jarad A., Liu, Zizhuo, Lin, Haixin, Chen, Peng-Cheng, Dravid, Vinayak P., Aydin, Koray, and Mirkin, Chad A. Fri .
"DNA-Mediated Size-Selective Nanoparticle Assembly for Multiplexed Surface Encoding". United States. https://doi.org/10.1021/acs.nanolett.8b00509. https://www.osti.gov/servlets/purl/1470552.
@article{osti_1470552,
title = {DNA-Mediated Size-Selective Nanoparticle Assembly for Multiplexed Surface Encoding},
author = {Lin, Qing-Yuan and Palacios, Edgar and Zhou, Wenjie and Li, Zhongyang and Mason, Jarad A. and Liu, Zizhuo and Lin, Haixin and Chen, Peng-Cheng and Dravid, Vinayak P. and Aydin, Koray and Mirkin, Chad A.},
abstractNote = {Multiplexed surface encoding is achieved by positioning two different sizes of gold nanocubes on gold surfaces with precisely defined locations for each particle via template-confined, DNA-mediated nanoparticle assembly. As a proof-of-concept demonstration, cubes with 86 and 63 nm edge lengths are assembled into arrangements that physically and spectrally encrypt two sets of patterns in the same location. These patterns can be decrypted by mapping the absorption intensity of the substrate at $λ$ = 773 and 687 nm, respectively. This multiplexed encoding platform dramatically increases the sophistication and density of codes that can be written using colloidal nanoparticles, which may enable high-security, high-resolution encoding applications.},
doi = {10.1021/acs.nanolett.8b00509},
journal = {Nano Letters},
number = 4,
volume = 18,
place = {United States},
year = {Fri Mar 23 00:00:00 EDT 2018},
month = {Fri Mar 23 00:00:00 EDT 2018}
}
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