Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material

Christensen, Thomas; Yan, Wei; Jauho, Antti-Pekka; Soljačić, Marin; Mortensen, N. Asger

doi:10.1103/PhysRevLett.118.157402

Title: Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material

Journal Article · 11 April 2017 · Physical Review Letters

DOI: https://doi.org/10.1103/PhysRevLett.118.157402 · OSTI ID:1470504

Christensen, Thomas ^[1]; Yan, Wei ^[2]; Jauho, Antti-Pekka ^[3]; Soljačić, Marin ^[1]; Mortensen, N. Asger ^[3]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Physics
Univ. Bordeaux, Talence (France); Centre National de la Recherche Scientifique (CNRS), Talence (France)
Technical Univ. of Denmark, Lyngby (Denmark). Center for Nanostructured Graphene, and Dept. of Micro- and Nanotechnology

The classical treatment of plasmonics is insufficient at the nanometer-scale due to quantum mechanical surface phenomena. Here, an extension of the classical paradigm is reported which rigorously remedies this deficiency through the incorporation of first-principles surface response functions—the Feibelman d parameters—in general geometries. Several analytical results for the leading-order plasmonic quantum corrections are obtained in a first-principles setting; particularly, a clear separation of the roles of shape, scale, and material is established. The utility of the formalism is illustrated by the derivation of a modified sum rule for complementary structures, a rigorous reformulation of Kreibig’s phenomenological damping prescription, and an account of the small-scale resonance shifting of simple and noble metal nanostructures.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Solid-State Solar-Thermal Energy Conversion Center (S3TEC); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0001299; FG02-09ER46577

OSTI ID:: 1470504

Alternate ID(s):: OSTI ID: 1351126

Journal Information:: Physical Review Letters, Vol. 118, Issue 15; Related Information: S3TEC partners with Massachusetts Institute of Technology (lead); Boston College; Oak Ridge National Laboratory; Rensselaer Polytechnic Institute; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 99 works

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