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Title: Light-trapping design for thin-film silicon-perovskite tandem solar cells

Abstract

Using finite-difference time-domain simulations, we investigate the optical properties of tandem silicon/perovskite solar cells with a photonic crystal architecture, consisting of a square-lattice array of inverted pyramids with a center-to-center spacing of 2.5 μm. Here, we demonstrate that near-perfect light-trapping and absorption can be achieved over the 300–1100 nm wavelength range with this architecture, using less than 10 μm (equivalent bulk thickness) of crystalline silicon. Using a one-diode model, we obtain projected efficiencies of over 30% for the two-terminal tandem cell under a current-matching condition, well beyond the current record for single-junction silicon solar cells. Lastly, the architecture is amenable to mass fabrication through wet-etching and uses a fraction of the silicon of traditional designs, making it an attractive alternative to other silicon-perovskite tandem designs.

Authors:
 [1];  [1]
  1. Univ. of Toronto, ON (Canada). Dept. of Physics
Publication Date:
Research Org.:
Rensselaer Polytechnic Inst., Troy, NY (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1467885
Alternate Identifier(s):
OSTI ID: 1324362
Grant/Contract Number:  
FG02-06ER46347
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Applied Physics
Additional Journal Information:
Journal Volume: 120; Journal Issue: 10; Journal ID: ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE; 14 SOLAR ENERGY; 36 MATERIALS SCIENCE

Citation Formats

Foster, Stephen, and John, Sajeev. Light-trapping design for thin-film silicon-perovskite tandem solar cells. United States: N. p., 2016. Web. https://doi.org/10.1063/1.4962458.
Foster, Stephen, & John, Sajeev. Light-trapping design for thin-film silicon-perovskite tandem solar cells. United States. https://doi.org/10.1063/1.4962458
Foster, Stephen, and John, Sajeev. Tue . "Light-trapping design for thin-film silicon-perovskite tandem solar cells". United States. https://doi.org/10.1063/1.4962458. https://www.osti.gov/servlets/purl/1467885.
@article{osti_1467885,
title = {Light-trapping design for thin-film silicon-perovskite tandem solar cells},
author = {Foster, Stephen and John, Sajeev},
abstractNote = {Using finite-difference time-domain simulations, we investigate the optical properties of tandem silicon/perovskite solar cells with a photonic crystal architecture, consisting of a square-lattice array of inverted pyramids with a center-to-center spacing of 2.5 μm. Here, we demonstrate that near-perfect light-trapping and absorption can be achieved over the 300–1100 nm wavelength range with this architecture, using less than 10 μm (equivalent bulk thickness) of crystalline silicon. Using a one-diode model, we obtain projected efficiencies of over 30% for the two-terminal tandem cell under a current-matching condition, well beyond the current record for single-junction silicon solar cells. Lastly, the architecture is amenable to mass fabrication through wet-etching and uses a fraction of the silicon of traditional designs, making it an attractive alternative to other silicon-perovskite tandem designs.},
doi = {10.1063/1.4962458},
journal = {Journal of Applied Physics},
number = 10,
volume = 120,
place = {United States},
year = {2016},
month = {9}
}

Journal Article:
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Cited by: 4 works
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Works referenced in this record:

Achievement of More Than 25% Conversion Efficiency With Crystalline Silicon Heterojunction Solar Cell
journal, November 2014


Light-trapping optimization in wet-etched silicon photonic crystal solar cells
journal, July 2015

  • Eyderman, Sergey; John, Sajeev; Hafez, M.
  • Journal of Applied Physics, Vol. 118, Issue 2
  • DOI: 10.1063/1.4926548

Light trapping and absorption optimization in certain thin-film photonic crystal architectures
journal, August 2008


Efficient and Uniform Planar-Type Perovskite Solar Cells by Simple Sequential Vacuum Deposition
journal, September 2014

  • Chen, Chang-Wen; Kang, Hao-Wei; Hsiao, Sheng-Yi
  • Advanced Materials, Vol. 26, Issue 38
  • DOI: 10.1002/adma.201402461

Perovskite solar cells join the major league
journal, November 2015


Effective optical response of silicon to sunlight in the finite-difference time-domain method
journal, December 2011


Perovskite Solar Cells: Influence of Hole Transporting Materials on Power Conversion Efficiency
journal, December 2015


Hole-transport material-free perovskite-based solar cells
journal, August 2015


Microcrystalline silicon and micromorph tandem solar cells
journal, August 1999

  • Keppner, H.; Meier, J.; Torres, P.
  • Applied Physics A: Materials Science & Processing, Vol. 69, Issue 2
  • DOI: 10.1007/s003390050987

Nanopyramid Structure for Ultrathin c-Si Tandem Solar Cells
journal, April 2014

  • Li, Guijun; Li, He; Ho, Jacob Y. L.
  • Nano Letters, Vol. 14, Issue 5
  • DOI: 10.1021/nl500366c

Strong localization of photons in certain disordered dielectric superlattices
journal, June 1987


Wideband dye-sensitized solar cells employing a phosphine-coordinated ruthenium sensitizer
journal, June 2013


Near perfect solar absorption in ultra-thin-film GaAs photonic crystals
journal, January 2014

  • Eyderman, Sergey; Deinega, Alexei; John, Sajeev
  • J. Mater. Chem. A, Vol. 2, Issue 3
  • DOI: 10.1039/C3TA13655H

Hybrid tandem solar cells with depleted-heterojunction quantum dot and polymer bulk heterojunction subcells
journal, October 2015


Tandem colloidal quantum dot solar cells employing a graded recombination layer
journal, June 2011


The efficiency limit of CH 3 NH 3 PbI 3 perovskite solar cells
journal, June 2015

  • Sha, Wei E. I.; Ren, Xingang; Chen, Luzhou
  • Applied Physics Letters, Vol. 106, Issue 22
  • DOI: 10.1063/1.4922150

Epitaxial lift-off process for gallium arsenide substrate reuse and flexible electronics
journal, March 2013

  • Cheng, Cheng-Wei; Shiu, Kuen-Ting; Li, Ning
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms2583

Reassessment of the Limiting Efficiency for Crystalline Silicon Solar Cells
journal, October 2013


Highly Efficient Hybrid Polymer and Amorphous Silicon Multijunction Solar Cells with Effective Optical Management
journal, January 2016


Complex Refractive Index Spectra of CH 3 NH 3 PbI 3 Perovskite Thin Films Determined by Spectroscopic Ellipsometry and Spectrophotometry
journal, December 2014

  • Löper, Philipp; Stuckelberger, Michael; Niesen, Bjoern
  • The Journal of Physical Chemistry Letters, Vol. 6, Issue 1
  • DOI: 10.1021/jz502471h

Improvement of polycrystalline silicon wafer solar cell efficiency by forming nanoscale pyramids on wafer surface using a self-mask etching technique
journal, May 2013

  • Lin, Hsin-Han; Chen, Wen-Hwa; Hong, Franklin C. -N.
  • Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 31, Issue 3
  • DOI: 10.1116/1.4795862

Efficient planar heterojunction perovskite solar cells by vapour deposition
journal, September 2013

  • Liu, Mingzhen; Johnston, Michael B.; Snaith, Henry J.
  • Nature, Vol. 501, Issue 7467, p. 395-398
  • DOI: 10.1038/nature12509

High-Stable-Efficiency Tandem Thin-Film Silicon Solar Cell With Low-Refractive-Index Silicon-Oxide Interlayer
journal, November 2014


Lift-off of Free-standing Layers in the Kerfless Porous Silicon Process
journal, January 2013


An Efficient Triple-Junction Polymer Solar Cell Having a Power Conversion Efficiency Exceeding 11%
journal, July 2014

  • Chen, Chun-Chao; Chang, Wei-Hsuan; Yoshimura, Ken
  • Advanced Materials, Vol. 26, Issue 32
  • DOI: 10.1002/adma.201402072

Parasitic absorption in the rear reflector of a silicon solar cell: Simulation and measurement of the sub-bandgap reflectance for common dielectric/metal reflectors
journal, January 2014

  • Holman, Zachary C.; Filipič, Miha; Lipovšek, Benjamin
  • Solar Energy Materials and Solar Cells, Vol. 120
  • DOI: 10.1016/j.solmat.2013.06.024

High efficiency stable inverted perovskite solar cells without current hysteresis
journal, January 2015

  • Wu, Chun-Guey; Chiang, Chien-Hung; Tseng, Zong-Liang
  • Energy & Environmental Science, Vol. 8, Issue 9
  • DOI: 10.1039/C5EE00645G

A 2-terminal perovskite/silicon multijunction solar cell enabled by a silicon tunnel junction
journal, March 2015

  • Mailoa, Jonathan P.; Bailie, Colin D.; Johlin, Eric C.
  • Applied Physics Letters, Vol. 106, Issue 12
  • DOI: 10.1063/1.4914179

Meep: A flexible free-software package for electromagnetic simulations by the FDTD method
journal, March 2010

  • Oskooi, Ardavan F.; Roundy, David; Ibanescu, Mihai
  • Computer Physics Communications, Vol. 181, Issue 3, p. 687-702
  • DOI: 10.1016/j.cpc.2009.11.008

A mixed-cation lead mixed-halide perovskite absorber for tandem solar cells
journal, January 2016


Monolithic perovskite/silicon-heterojunction tandem solar cells processed at low temperature
journal, January 2016

  • Albrecht, Steve; Saliba, Michael; Correa Baena, Juan Pablo
  • Energy & Environmental Science, Vol. 9, Issue 1
  • DOI: 10.1039/C5EE02965A

Solar light trapping in slanted conical-pore photonic crystals: Beyond statistical ray trapping
journal, April 2013

  • Eyderman, Sergey; John, Sajeev; Deinega, Alexei
  • Journal of Applied Physics, Vol. 113, Issue 15
  • DOI: 10.1063/1.4802442

Inhibited Spontaneous Emission in Solid-State Physics and Electronics
journal, May 1987


CH_3NH_3PbI_3 perovskite / silicon tandem solar cells: characterization based optical simulations
journal, January 2015

  • Filipič, Miha; Löper, Philipp; Niesen, Bjoern
  • Optics Express, Vol. 23, Issue 7
  • DOI: 10.1364/OE.23.00A263

Perovskite/c-Si tandem solar cell with inverted nanopyramids: realizing high efficiency by controllable light trapping
journal, November 2015

  • Shi, Dai; Zeng, Yang; Shen, Wenzhong
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep16504

A polymer tandem solar cell with 10.6% power conversion efficiency
journal, February 2013

  • You, Jingbi; Dou, Letian; Yoshimura, Ken
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms2411

Pyramidal surface textures for light trapping and antireflection in perovskite-on-silicon tandem solar cells
journal, January 2014

  • Schneider, Bennett W.; Lal, Niraj N.; Baker-Finch, Simeon
  • Optics Express, Vol. 22, Issue S6
  • DOI: 10.1364/OE.22.0A1422

Photovoltaic Technology: The Case for Thin-Film Solar Cells
journal, July 1999


Electrically Tunable Plasmonic Behavior of Nanocube–Polymer Nanomaterials Induced by a Redox-Active Electrochromic Polymer
journal, May 2014

  • König, Tobias A. F.; Ledin, Petr A.; Kerszulis, Justin
  • ACS Nano, Vol. 8, Issue 6
  • DOI: 10.1021/nn501601e

    Works referencing / citing this record:

    Photonic crystal light trapping: Beyond 30% conversion efficiency for silicon photovoltaics
    journal, February 2020

    • Bhattacharya, Sayak; John, Sajeev
    • APL Photonics, Vol. 5, Issue 2
    • DOI: 10.1063/1.5128664

    Computational screening of methylammonium based halide perovskites with bandgaps suitable for perovskite-perovskite tandem solar cells
    journal, December 2018

    • Kar, M.; Körzdörfer, T.
    • The Journal of Chemical Physics, Vol. 149, Issue 21
    • DOI: 10.1063/1.5037535

    Simulation of perovskite solar cells by using CuSCN as an inorganic hole-transport material
    journal, July 2019

    • Hazeghi, Farzaneh; Ghorashi, Seyed Mohamad Bagher
    • Materials Research Express, Vol. 6, Issue 9
    • DOI: 10.1088/2053-1591/ab2f1b

    A review of recent progress in heterogeneous silicon tandem solar cells
    journal, March 2018

    • Yamaguchi, Masafumi; Lee, Kan-Hua; Araki, Kenji
    • Journal of Physics D: Applied Physics, Vol. 51, Issue 13
    • DOI: 10.1088/1361-6463/aaaf08

    New-generation integrated devices based on dye-sensitized and perovskite solar cells
    journal, January 2018

    • Yun, Sining; Qin, Yong; Uhl, Alexander R.
    • Energy & Environmental Science, Vol. 11, Issue 3
    • DOI: 10.1039/c7ee03165c

    Metal halide perovskite tandem and multiple-junction photovoltaics
    journal, November 2017

    • Eperon, Giles E.; Hörantner, Maximilian T.; Snaith, Henry J.
    • Nature Reviews Chemistry, Vol. 1, Issue 12
    • DOI: 10.1038/s41570-017-0095