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Title: Superconductivity in pressurized CeRhG e 3 and related noncentrosymmetric compounds

Abstract

Here, we report the discovery of superconductivity in pressurized CeRhGe3, a nonsuperconducting member of the isostructural family of noncentrosymmetric heavy-fermion compounds CeTX3(T = Co, Rh, Ir and X=Si, Ge). Superconductivity appears in CeRhGe3 at a pressure of 19.6 GPa and the transition temperature TC reaches a maximum value of 1.3 K at 21.5 GPa. This finding provides an opportunity to establish systematic correlations between superconductivity and material properties within this family. Though ambient-pressure unit-cell volumes and critical pressures for superconductivity vary substantially across the series, all family members reach a maximum TmaxC at a common (±1.7%) critical cell volume Vcrit, and TmaxC at Vcrit increases with increasing spin-orbit coupling strength of the d electrons. These correlations show that substantial Kondo and spin-orbit couplings favor superconductivity in this family, the latter reflecting the role of broken centrosymmetry.

Authors:
 [1];  [2]; ORCiD logo [3];  [4];  [1];  [1];  [2];  [1];  [1];  [5];  [5];  [2];  [2];  [2];  [1];  [2];  [1]; ORCiD logo [3];  [1]
  1. Chinese Academy of Sciences (CAS), Beijing (China); Univ. of Chinese Academy of Sciences, Beijing (China)
  2. Chinese Academy of Sciences (CAS), Beijing (China)
  3. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  4. Russian Academy of Sciences, Moscow (Russia)
  5. Chinese Academy of Sciences, Shanghai (China)
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1467208
Alternate Identifier(s):
OSTI ID: 1421885
Report Number(s):
LA-UR-17-27472
Journal ID: ISSN 2469-9950; PRBMDO
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 97; Journal Issue: 6; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; High Magnetic Field Science; Superconductivity; pressure; non-centrosymmetric

Citation Formats

Wang, Honghong, Guo, Jing, Bauer, Eric Dietzgen, Sidorov, Vladimir A., Zhao, Hengcan, Zhang, Jiahao, Zhou, Yazhou, Wang, Zhe, Cai, Shu, Yang, Ke, Li, Aiguo, Li, Xiaodong, Li, Yanchun, Sun, Peijie, Yang, Yi-feng, Wu, Qi, Xiang, Tao, Thompson, Joe David, and Sun, Liling. Superconductivity in pressurized CeRhGe3 and related noncentrosymmetric compounds. United States: N. p., 2018. Web. doi:10.1103/PhysRevB.97.064514.
Wang, Honghong, Guo, Jing, Bauer, Eric Dietzgen, Sidorov, Vladimir A., Zhao, Hengcan, Zhang, Jiahao, Zhou, Yazhou, Wang, Zhe, Cai, Shu, Yang, Ke, Li, Aiguo, Li, Xiaodong, Li, Yanchun, Sun, Peijie, Yang, Yi-feng, Wu, Qi, Xiang, Tao, Thompson, Joe David, & Sun, Liling. Superconductivity in pressurized CeRhGe3 and related noncentrosymmetric compounds. United States. https://doi.org/10.1103/PhysRevB.97.064514
Wang, Honghong, Guo, Jing, Bauer, Eric Dietzgen, Sidorov, Vladimir A., Zhao, Hengcan, Zhang, Jiahao, Zhou, Yazhou, Wang, Zhe, Cai, Shu, Yang, Ke, Li, Aiguo, Li, Xiaodong, Li, Yanchun, Sun, Peijie, Yang, Yi-feng, Wu, Qi, Xiang, Tao, Thompson, Joe David, and Sun, Liling. Tue . "Superconductivity in pressurized CeRhGe3 and related noncentrosymmetric compounds". United States. https://doi.org/10.1103/PhysRevB.97.064514. https://www.osti.gov/servlets/purl/1467208.
@article{osti_1467208,
title = {Superconductivity in pressurized CeRhGe3 and related noncentrosymmetric compounds},
author = {Wang, Honghong and Guo, Jing and Bauer, Eric Dietzgen and Sidorov, Vladimir A. and Zhao, Hengcan and Zhang, Jiahao and Zhou, Yazhou and Wang, Zhe and Cai, Shu and Yang, Ke and Li, Aiguo and Li, Xiaodong and Li, Yanchun and Sun, Peijie and Yang, Yi-feng and Wu, Qi and Xiang, Tao and Thompson, Joe David and Sun, Liling},
abstractNote = {Here, we report the discovery of superconductivity in pressurized CeRhGe3, a nonsuperconducting member of the isostructural family of noncentrosymmetric heavy-fermion compounds CeTX3(T = Co, Rh, Ir and X=Si, Ge). Superconductivity appears in CeRhGe3 at a pressure of 19.6 GPa and the transition temperature TC reaches a maximum value of 1.3 K at 21.5 GPa. This finding provides an opportunity to establish systematic correlations between superconductivity and material properties within this family. Though ambient-pressure unit-cell volumes and critical pressures for superconductivity vary substantially across the series, all family members reach a maximum TmaxC at a common (±1.7%) critical cell volume Vcrit, and TmaxC at Vcrit increases with increasing spin-orbit coupling strength of the d electrons. These correlations show that substantial Kondo and spin-orbit couplings favor superconductivity in this family, the latter reflecting the role of broken centrosymmetry.},
doi = {10.1103/PhysRevB.97.064514},
journal = {Physical Review B},
number = 6,
volume = 97,
place = {United States},
year = {Tue Feb 20 00:00:00 EST 2018},
month = {Tue Feb 20 00:00:00 EST 2018}
}

Journal Article:

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Cited by: 19 works
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Figures / Tables:

Figure 1 Figure 1: Temperature dependences of heat capacity divided by temperature (C/T) at different pressures. TN1 and TN2 correspond to the higher and lower AFM transition temperatures, respectively.

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Works referenced in this record:

Pressure-Induced Heavy-Fermion Superconductivity in Antiferromagnet CeIrSi 3 without Inversion Symmetry
journal, April 2006

  • Sugitani, Ichiro; Okuda, Yusuke; Shishido, Hiroaki
  • Journal of the Physical Society of Japan, Vol. 75, Issue 4
  • DOI: 10.1143/JPSJ.75.043703

Evaluations of pressure-transmitting media for cryogenic experiments with diamond anvil cell
journal, December 2009

  • Tateiwa, Naoyuki; Haga, Yoshinori
  • Review of Scientific Instruments, Vol. 80, Issue 12
  • DOI: 10.1063/1.3265992

Effect of pressure on the superconducting T c of lanthanum
journal, April 1996

  • Tissen, V. G.; Ponyatovskii, E. G.; Nefedova, M. V.
  • Physical Review B, Vol. 53, Issue 13
  • DOI: 10.1103/PhysRevB.53.8238

Re-emerging superconductivity at 48 kelvin in iron chalcogenides
journal, February 2012


Pressure Effect of Electronic States in Antiferromagnets CeTX 3 (T: Transition Metal, X: Si and Ge)
journal, January 2007

  • Kawai, Tomoya; Nakashima, Miho; Okuda, Yusuke
  • Journal of the Physical Society of Japan, Vol. 76, Issue Suppl.A
  • DOI: 10.1143/JPSJS.76SA.166

Pressure-Induced Superconductivity in Noncentrosymmetric Heavy-Fermion CeRhSi 3
journal, December 2005


Absence of Quantum Criticality and Presence of Superconducting Fluctuation in Pressure-Induced Heavy-Fermion Superconductor CeRhSi 3
journal, May 2012

  • Sugawara, Tetsuya; Iida, Hiroki; Aoki, Haruyoshi
  • Journal of the Physical Society of Japan, Vol. 81, Issue 5
  • DOI: 10.1143/JPSJ.81.054711

Silicone fluid as a high‐pressure medium in diamond anvil cells
journal, February 1996

  • Ragan, Deirdre D.; Clarke, David R.; Schiferl, David
  • Review of Scientific Instruments, Vol. 67, Issue 2
  • DOI: 10.1063/1.1146627

Textured Superconducting Phase in the Heavy Fermion CeRhIn 5
journal, February 2012


High Pressure Phase Diagram of the Non-centrosymmetric Antiferromagnet CeCoGe 3
journal, July 2009

  • Knebel, Georg; Aoki, Dai; Lapertot, Gerard
  • Journal of the Physical Society of Japan, Vol. 78, Issue 7
  • DOI: 10.1143/JPSJ.78.074714

Superconducting phases of f -electron compounds
journal, November 2009


Textured superconductivity in the presence of a coexisting order: Ce115s and other heavy-fermion compounds
journal, November 2012


Normal and Superconducting Properties of Noncentrosymmetric Heavy Fermion CeRhSi 3
journal, May 2007

  • Kimura, Noriaki; Muro, Yuji; Aoki, Haruyoshi
  • Journal of the Physical Society of Japan, Vol. 76, Issue 5
  • DOI: 10.1143/JPSJ.76.051010

Characteristics of silicone fluid as a pressure transmitting medium in diamond anvil cells
journal, November 2004

  • Shen, Yongrong; Kumar, Ravhi S.; Pravica, Michael
  • Review of Scientific Instruments, Vol. 75, Issue 11
  • DOI: 10.1063/1.1786355

Hydrostatic limits in liquids and solids to 100 kbar
journal, December 1973

  • Piermarini, G. J.; Block, S.; Barnett, J. D.
  • Journal of Applied Physics, Vol. 44, Issue 12
  • DOI: 10.1063/1.1662159

Magnetic and Superconducting Properties of CeTX 3 (T: Transition Metal and X: Si and Ge) with Non-centrosymmetric Crystal Structure
journal, June 2008

  • Kawai, Tomoya; Muranaka, Hiroshi; Measson, Marie-Aude
  • Journal of the Physical Society of Japan, Vol. 77, Issue 6
  • DOI: 10.1143/JPSJ.77.064716

Superconductivity at 17 K in yttrium metal under nearly hydrostatic pressures up to 89 GPa
journal, March 2006


Comparison of the pressure dependences of T c in the trivalent d -electron superconductors Sc, Y, La, and Lu up to megabar pressures
journal, August 2008


The Kondo lattice and weak antiferromagnetism
journal, July 1977


Huge Upper Critical Field and Electronic Instability in Pressure-induced Superconductor CeIrSi 3 without Inversion Symmetry in the Crystal Structure
journal, July 2008

  • Settai, Rikio; Miyauchi, Yuichiro; Takeuchi, Tetsuya
  • Journal of the Physical Society of Japan, Vol. 77, Issue 7
  • DOI: 10.1143/JPSJ.77.073705

Superconductivity and spin–orbit coupling in non-centrosymmetric materials: a review
journal, January 2017


Magnetic and electronic properties in and (T: transition metal)
journal, March 2007

  • Shimoda, T.; Okuda, Y.; Takeda, Y.
  • Journal of Magnetism and Magnetic Materials, Vol. 310, Issue 2
  • DOI: 10.1016/j.jmmm.2006.10.055

NON-CENTROSYMMETRIC HEAVY FERMION SUPERCONDUCTIVITY IN CeCoGe 3
journal, July 2007

  • Settai, R.; Okuda, Y.; Sugitani, I.
  • International Journal of Modern Physics B, Vol. 21, Issue 18n19
  • DOI: 10.1142/S0217979207044287

Works referencing / citing this record:

Evidence of a Nodal Line in the Superconducting Gap Symmetry of Noncentrosymmetric ThCoC 2
journal, April 2019


Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.