Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices
Abstract
Perovskite nickelate heterostructures consisting of single unit cells of EuNiO3 and LaNiO3 have been grown on a set of single crystalline substrates by pulsed laser interval deposition to investigate the effect of epitaxial strain on electronic and magnetic properties at the extreme interface limit. Despite the variation of substrate in-plane lattice constants and lattice symmetry, the structural response to heterostructuring is primarily controlled by the presence of the EuNiO3 layer. In sharp contrast to bulk LaNiO3 or EuNiO3, the superlattices grown under tensile strains exhibit metal-to-insulator transitions (MIT) below room temperature. The onset of magnetic and electronic transitions associated with the MIT can be further separated by application of large tensile strain. Furthermore, these transitions can be entirely suppressed by very small compressive strain. X-ray resonant absorption spectroscopy measurements reveal that such strain-controlled MIT is directly linked to a strain-induced self-doping effect without any chemical doping.
- Authors:
-
- Indian Inst. of Science (IISc), Bangalore (India). Dept. of Physics
- Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
- Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics and Astronomy
- Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; Gordon and Betty Moore Foundation
- OSTI Identifier:
- 1466980
- Alternate Identifier(s):
- OSTI ID: 1459685; OSTI ID: 1481748
- Report Number(s):
- BNL-208013-2018-JAAM
Journal ID: ISSN 2469-9950; PRBMDO
- Grant/Contract Number:
- SC0012704; 1047478; GBMF4534; SC00012375; AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 98; Journal Issue: 4; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; antiferromagnetism; insulators; metals; surface and interfacial phenomena; charge-transfer insulators; ultrathin films; laser ablation; x-ray absorption spectroscopy
Citation Formats
Middey, S., Meyers, D., Ojha, Shashank Kumar, Kareev, M., Liu, X., Cao, Y., Freeland, J. W., and Chakhalian, J. Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices. United States: N. p., 2018.
Web. doi:10.1103/PhysRevB.98.045115.
Middey, S., Meyers, D., Ojha, Shashank Kumar, Kareev, M., Liu, X., Cao, Y., Freeland, J. W., & Chakhalian, J. Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices. United States. https://doi.org/10.1103/PhysRevB.98.045115
Middey, S., Meyers, D., Ojha, Shashank Kumar, Kareev, M., Liu, X., Cao, Y., Freeland, J. W., and Chakhalian, J. Tue .
"Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices". United States. https://doi.org/10.1103/PhysRevB.98.045115. https://www.osti.gov/servlets/purl/1466980.
@article{osti_1466980,
title = {Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices},
author = {Middey, S. and Meyers, D. and Ojha, Shashank Kumar and Kareev, M. and Liu, X. and Cao, Y. and Freeland, J. W. and Chakhalian, J.},
abstractNote = {Perovskite nickelate heterostructures consisting of single unit cells of EuNiO3 and LaNiO3 have been grown on a set of single crystalline substrates by pulsed laser interval deposition to investigate the effect of epitaxial strain on electronic and magnetic properties at the extreme interface limit. Despite the variation of substrate in-plane lattice constants and lattice symmetry, the structural response to heterostructuring is primarily controlled by the presence of the EuNiO3 layer. In sharp contrast to bulk LaNiO3 or EuNiO3, the superlattices grown under tensile strains exhibit metal-to-insulator transitions (MIT) below room temperature. The onset of magnetic and electronic transitions associated with the MIT can be further separated by application of large tensile strain. Furthermore, these transitions can be entirely suppressed by very small compressive strain. X-ray resonant absorption spectroscopy measurements reveal that such strain-controlled MIT is directly linked to a strain-induced self-doping effect without any chemical doping.},
doi = {10.1103/PhysRevB.98.045115},
journal = {Physical Review B},
number = 4,
volume = 98,
place = {United States},
year = {2018},
month = {7}
}
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Figure 1: (a) 1EuNiO3/1LaNiO3 superlattice along pseudocubic [0 0 1]. (b) Schematic of sequence for layer-by-layer deposition used for this study. (c) Intensity variation of RHEED specular spot during the deposition on NdGaO3 substrate. (d) Final RHEED pattern obtained along the [1 -1 0] direction of NGO after cooling themore »
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Works referencing / citing this record:
Tuning the Electronic Structure of LaNiO 3 through Alloying with Strontium to Enhance Oxygen Evolution Activity
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Conductivity noise across temperature driven transitions of rare-earth nickelate heterostructures
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