Insights into the Na+ Storage Mechanism of Phosphorus-Functionalized Hard Carbon as Ultrahigh Capacity Anodes
Abstract
Abstract Hard carbon as a typical anode material for sodium ion batteries has received much attention in terms of its low cost and renewability. Herein, phosphorus‐functionalized hard carbon with a specific “honeycomb briquette” shaped morphology is synthesized via electrospinning technology. When applied as an anode material for Na + storage, it exhibits an impressively high reversible capacity of 393.4 mA h g −1 with the capacity retention up to 98.2% after 100 cycles. According to first‐principle calculation, the ultrahigh capacity of the as‐prepared anode is ascribed to the enhancement of Na‐absorption through formation of PO and PC bonds in graphitic layers when doped with phosphorus. Moreover, the increase of electron density around the Fermi level is found to be mainly caused by O atoms instead of P atoms.
- Authors:
-
[2]
- Beijing Institute of Technology, Beijing (People's Republic of China)
- Argonne National Lab. (ANL), Lemont, IL (United States)
- Beijing Institute of Technology, Beijing (People's Republic of China); Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing (People's Republic of China)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); National Basic Research Program of China; USDOE
- OSTI Identifier:
- 1466401
- Alternate Identifier(s):
- OSTI ID: 1423911
- Grant/Contract Number:
- AC02-06CH11357; DE‐AC02‐06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 18; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; first-principle calculations; hard carbon; phosphorous-functionalization; sodium ion batteries; ultrahigh capacity
Citation Formats
Li, Yu, Yuan, Yifei, Bai, Ying, Liu, Yuanchang, Wang, Zhaohua, Li, Limin, Wu, Feng, Amine, Khalil, Wu, Chuan, and Lu, Jun. Insights into the Na+ Storage Mechanism of Phosphorus-Functionalized Hard Carbon as Ultrahigh Capacity Anodes. United States: N. p., 2018.
Web. doi:10.1002/aenm.201702781.
Li, Yu, Yuan, Yifei, Bai, Ying, Liu, Yuanchang, Wang, Zhaohua, Li, Limin, Wu, Feng, Amine, Khalil, Wu, Chuan, & Lu, Jun. Insights into the Na+ Storage Mechanism of Phosphorus-Functionalized Hard Carbon as Ultrahigh Capacity Anodes. United States. https://doi.org/10.1002/aenm.201702781
Li, Yu, Yuan, Yifei, Bai, Ying, Liu, Yuanchang, Wang, Zhaohua, Li, Limin, Wu, Feng, Amine, Khalil, Wu, Chuan, and Lu, Jun. Tue .
"Insights into the Na+ Storage Mechanism of Phosphorus-Functionalized Hard Carbon as Ultrahigh Capacity Anodes". United States. https://doi.org/10.1002/aenm.201702781. https://www.osti.gov/servlets/purl/1466401.
@article{osti_1466401,
title = {Insights into the Na+ Storage Mechanism of Phosphorus-Functionalized Hard Carbon as Ultrahigh Capacity Anodes},
author = {Li, Yu and Yuan, Yifei and Bai, Ying and Liu, Yuanchang and Wang, Zhaohua and Li, Limin and Wu, Feng and Amine, Khalil and Wu, Chuan and Lu, Jun},
abstractNote = {Abstract Hard carbon as a typical anode material for sodium ion batteries has received much attention in terms of its low cost and renewability. Herein, phosphorus‐functionalized hard carbon with a specific “honeycomb briquette” shaped morphology is synthesized via electrospinning technology. When applied as an anode material for Na + storage, it exhibits an impressively high reversible capacity of 393.4 mA h g −1 with the capacity retention up to 98.2% after 100 cycles. According to first‐principle calculation, the ultrahigh capacity of the as‐prepared anode is ascribed to the enhancement of Na‐absorption through formation of PO and PC bonds in graphitic layers when doped with phosphorus. Moreover, the increase of electron density around the Fermi level is found to be mainly caused by O atoms instead of P atoms.},
doi = {10.1002/aenm.201702781},
journal = {Advanced Energy Materials},
number = 18,
volume = 8,
place = {United States},
year = {Tue Mar 06 00:00:00 EST 2018},
month = {Tue Mar 06 00:00:00 EST 2018}
}
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Figure 1: a) Schematic diagram of the synthesis of hard carbon anodes by electrospinning method, b) SEM images of HC-P15 precursor, c) magnified SEM image of sample HC-P15, d-e) EDX elemental distribution mapping of sample HC-P15 basde on c). HRTEM images of f) sample HC and g) sample HC-P15, themore »
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