Atomically Thin Mesoporous Co3O4 Layers Strongly Coupled with N-rGO Nanosheets as High-Performance Bifunctional Catalysts for 1D Knittable Zinc-Air Batteries [Atomically Thin Mesoporous Co3O4/N-rGO Nanosheets as the Bifunctional Catalysts for One-Dimensional Knittable Zinc-Air Batteries]
Abstract
Here, under development for next–generation wearable electronics are flexible, knittable, and wearable energy–storage devices with high energy density that can be integrated into textiles. Herein, knittable fiber–shaped zinc–air batteries with high volumetric energy density (36.1 mWh cm–3) are fabricated via a facile and continuous method with low–cost materials. Furthermore, a high–yield method is developed to prepare the key component of the fiber–shaped zinc–air battery, i.e., a bifunctional catalyst composed of atomically thin layer–by–layer mesoporous Co3O4/nitrogen–doped reduced graphene oxide (N–rGO) nanosheets. Benefiting from the high surface area, mesoporous structure, and strong synergetic effect between the Co3O4 and N–rGO nanosheets, the bifunctional catalyst exhibits high activity and superior durability for oxygen reduction and evolution reactions. Compared to a fiber–shaped zinc–air battery using state–of–the–art Pt/C + RuO2 catalysts, the battery based on these Co3O4/N–rGO nanosheets demonstrates enhanced and stable electrochemical performance, even under severe deformation. Such batteries, for the first time, can be successfully knitted into clothes without short circuits under external forces and can power various electronic devices and even charge a cellphone.
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- National Key Research and Development Program of China; National Natural Science Foundation of China (NNSFC); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); USDOE
- OSTI Identifier:
- 1466320
- Alternate Identifier(s):
- OSTI ID: 1412569
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 30; Journal Issue: 4; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; atomically thin hybrid nanosheets; cobalt oxides; knittable; wearable electronics; zinc-air batteries
Citation Formats
Li, Yingbo, Zhong, Cheng, Liu, Jie, Zeng, Xiaoqiao, Qu, Shengxiang, Han, Xiaopeng, Deng, Yida, Hu, Wenbin, and Lu, Jun. Atomically Thin Mesoporous Co3O4 Layers Strongly Coupled with N-rGO Nanosheets as High-Performance Bifunctional Catalysts for 1D Knittable Zinc-Air Batteries [Atomically Thin Mesoporous Co3O4/N-rGO Nanosheets as the Bifunctional Catalysts for One-Dimensional Knittable Zinc-Air Batteries]. United States: N. p., 2017.
Web. doi:10.1002/adma.201703657.
Li, Yingbo, Zhong, Cheng, Liu, Jie, Zeng, Xiaoqiao, Qu, Shengxiang, Han, Xiaopeng, Deng, Yida, Hu, Wenbin, & Lu, Jun. Atomically Thin Mesoporous Co3O4 Layers Strongly Coupled with N-rGO Nanosheets as High-Performance Bifunctional Catalysts for 1D Knittable Zinc-Air Batteries [Atomically Thin Mesoporous Co3O4/N-rGO Nanosheets as the Bifunctional Catalysts for One-Dimensional Knittable Zinc-Air Batteries]. United States. doi:10.1002/adma.201703657.
Li, Yingbo, Zhong, Cheng, Liu, Jie, Zeng, Xiaoqiao, Qu, Shengxiang, Han, Xiaopeng, Deng, Yida, Hu, Wenbin, and Lu, Jun. Wed .
"Atomically Thin Mesoporous Co3O4 Layers Strongly Coupled with N-rGO Nanosheets as High-Performance Bifunctional Catalysts for 1D Knittable Zinc-Air Batteries [Atomically Thin Mesoporous Co3O4/N-rGO Nanosheets as the Bifunctional Catalysts for One-Dimensional Knittable Zinc-Air Batteries]". United States. doi:10.1002/adma.201703657. https://www.osti.gov/servlets/purl/1466320.
@article{osti_1466320,
title = {Atomically Thin Mesoporous Co3O4 Layers Strongly Coupled with N-rGO Nanosheets as High-Performance Bifunctional Catalysts for 1D Knittable Zinc-Air Batteries [Atomically Thin Mesoporous Co3O4/N-rGO Nanosheets as the Bifunctional Catalysts for One-Dimensional Knittable Zinc-Air Batteries]},
author = {Li, Yingbo and Zhong, Cheng and Liu, Jie and Zeng, Xiaoqiao and Qu, Shengxiang and Han, Xiaopeng and Deng, Yida and Hu, Wenbin and Lu, Jun},
abstractNote = {Here, under development for next–generation wearable electronics are flexible, knittable, and wearable energy–storage devices with high energy density that can be integrated into textiles. Herein, knittable fiber–shaped zinc–air batteries with high volumetric energy density (36.1 mWh cm–3) are fabricated via a facile and continuous method with low–cost materials. Furthermore, a high–yield method is developed to prepare the key component of the fiber–shaped zinc–air battery, i.e., a bifunctional catalyst composed of atomically thin layer–by–layer mesoporous Co3O4/nitrogen–doped reduced graphene oxide (N–rGO) nanosheets. Benefiting from the high surface area, mesoporous structure, and strong synergetic effect between the Co3O4 and N–rGO nanosheets, the bifunctional catalyst exhibits high activity and superior durability for oxygen reduction and evolution reactions. Compared to a fiber–shaped zinc–air battery using state–of–the–art Pt/C + RuO2 catalysts, the battery based on these Co3O4/N–rGO nanosheets demonstrates enhanced and stable electrochemical performance, even under severe deformation. Such batteries, for the first time, can be successfully knitted into clothes without short circuits under external forces and can power various electronic devices and even charge a cellphone.},
doi = {10.1002/adma.201703657},
journal = {Advanced Materials},
number = 4,
volume = 30,
place = {United States},
year = {2017},
month = {12}
}
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Nonsiliceous Mesoporous Materials: Design and Applications in Energy Conversion and Storage
journal, March 2019
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General and Scalable Fabrication of Core–Shell Metal Sulfides@C Anchored on 3D N‐Doped Foam toward Flexible Sodium Ion Batteries
journal, September 2019
- Ma, Xiangdong; Xiong, Xunhui; Zou, Pinjuan
- Small, Vol. 15, Issue 45
Surface and Interface Engineering: Molybdenum Carbide–Based Nanomaterials for Electrochemical Energy Conversion
journal, September 2019
- Ge, Riyue; Huo, Juanjuan; Sun, Mingjie
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Oxygen Vacancy–Rich In‐Doped CoO/CoP Heterostructure as an Effective Air Cathode for Rechargeable Zn–Air Batteries
journal, September 2019
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- Small, Vol. 15, Issue 46
Designing Advanced Catalysts for Energy Conversion Based on Urea Oxidation Reaction
journal, January 2020
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Self-templated nitrogen-doped mesoporous carbon decorated with double transition-metal active sites for enhanced oxygen electrode catalysis
journal, December 2019
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Energy autonomous electronic skin
journal, January 2019
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Electrochemical energy storage devices for wearable technology: a rationale for materials selection and cell design
journal, January 2018
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N,S-Atom-coordinated Co 9 S 8 trinary dopants within a porous graphene framework as efficient catalysts for oxygen reduction/evolution reactions
journal, January 2018
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Highly active bifunctional oxygen electrocatalysts derived from nickel– or cobalt–phytic acid xerogel for zinc–air batteries
journal, January 2018
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- Nanoscale, Vol. 10, Issue 33
Robust N-doped carbon aerogels strongly coupled with iron–cobalt particles as efficient bifunctional catalysts for rechargeable Zn–air batteries
journal, January 2018
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- Nanoscale, Vol. 10, Issue 42
Controllable synthesis of nickel sulfide nanocatalysts and their phase-dependent performance for overall water splitting
journal, January 2019
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- Nanoscale, Vol. 11, Issue 12
Methacrylated gelatin-embedded fabrication of 3D graphene-supported Co 3 O 4 nanoparticles for water splitting
journal, January 2019
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- Nanoscale, Vol. 11, Issue 14
Bifunctional electrocatalysts of MOF-derived Co–N/C on bamboo-like MnO nanowires for high-performance liquid- and solid-state Zn–air batteries
journal, January 2018
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Palladium single atoms supported by interwoven carbon nanotube and manganese oxide nanowire networks for enhanced electrocatalysis
journal, January 2018
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- Journal of Materials Chemistry A, Vol. 6, Issue 46
Subnanometer iron clusters confined in a porous carbon matrix for highly efficient zinc–air batteries
journal, January 2020
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Co 3 O 4 nanosheets on zeolite-templated carbon as an efficient oxygen electrocatalyst for a zinc–air battery
journal, January 2019
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Nanostructured Co-based bifunctional electrocatalysts for energy conversion and storage: current status and perspectives
journal, January 2019
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- Journal of Materials Chemistry A, Vol. 7, Issue 32
Long-battery-life flexible zinc–air battery with near-neutral polymer electrolyte and nanoporous integrated air electrode
journal, January 2019
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Enhanced performance of multi-dimensional CoS nanoflake/NiO nanosheet architecture with synergetic effect for asymmetric supercapacitor
journal, September 2018
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Review—Energy Autonomous Wearable Sensors for Smart Healthcare: A Review
journal, January 2020
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BCNO Nanosheet Supported Co 3 O 4 Nanoparticles as an Enhanced Electrocatalyst for Oxygen Evolution Reaction
journal, January 2019
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- Journal of The Electrochemical Society, Vol. 166, Issue 6
Controlled Synthesis of Porous Co 3 O 4 Nanostructures for Efficient Electrochemical Sensing of Glucose
journal, September 2019
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- Journal of Nanomaterials, Vol. 2019
Effective Oxygen Reduction Reaction Performance of FeCo Alloys In Situ Anchored on Nitrogen-Doped Carbon by the Microwave-Assistant Carbon Bath Method and Subsequent Plasma Etching
journal, September 2019
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