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Title: An all-dielectric metasurface as a broadband optical frequency mixer

Abstract

A frequency mixer is a nonlinear device that combines electromagnetic waves to create waves at new frequencies. Mixers are ubiquitous components in modern radio-frequency technology and microwave signal processing. The development of versatile frequency mixers for optical frequencies remains challenging: such devices generally rely on weak nonlinear optical processes and, thus, must satisfy phase-matching conditions. Here we utilize a GaAs-based dielectric metasurface to demonstrate an optical frequency mixer that concurrently generates eleven new frequencies spanning the ultraviolet to near-infrared. The even and odd order nonlinearities of GaAs enable our observation of second-harmonic, third-harmonic, and fourth-harmonic generation, sum-frequency generation, two-photon absorption-induced photoluminescence, four-wave mixing and six-wave mixing. The simultaneous occurrence of these seven nonlinear processes is assisted by the combined effects of strong intrinsic material nonlinearities, enhanced electromagnetic fields, and relaxed phase-matching requirements. In conclusion, such ultracompact optical mixers may enable a plethora of applications in biology, chemistry, sensing, communications, and quantum optics.

Authors:
ORCiD logo [1]; ORCiD logo [1];  [2];  [3];  [1];  [1];  [2];  [3]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Friedrich Schiller Univ., Jena (Germany). Inst. of Applied Physics, Abbe Center of Photonics
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1464190
Report Number(s):
[SAND-2018-7466J]
[Journal ID: ISSN 2041-1723; 665684]
Grant/Contract Number:  
[AC04-94AL85000; NA0003525]
Resource Type:
Accepted Manuscript
Journal Name:
Nature Communications
Additional Journal Information:
[ Journal Volume: 9; Journal Issue: 1]; Journal ID: ISSN 2041-1723
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Liu, Sheng, Vabishchevich, Polina P., Vaskin, Aleksandr, Reno, John L., Keeler, Gordon A., Sinclair, Michael B., Staude, Isabelle, and Brener, Igal. An all-dielectric metasurface as a broadband optical frequency mixer. United States: N. p., 2018. Web. doi:10.1038/s41467-018-04944-9.
Liu, Sheng, Vabishchevich, Polina P., Vaskin, Aleksandr, Reno, John L., Keeler, Gordon A., Sinclair, Michael B., Staude, Isabelle, & Brener, Igal. An all-dielectric metasurface as a broadband optical frequency mixer. United States. doi:10.1038/s41467-018-04944-9.
Liu, Sheng, Vabishchevich, Polina P., Vaskin, Aleksandr, Reno, John L., Keeler, Gordon A., Sinclair, Michael B., Staude, Isabelle, and Brener, Igal. Thu . "An all-dielectric metasurface as a broadband optical frequency mixer". United States. doi:10.1038/s41467-018-04944-9. https://www.osti.gov/servlets/purl/1464190.
@article{osti_1464190,
title = {An all-dielectric metasurface as a broadband optical frequency mixer},
author = {Liu, Sheng and Vabishchevich, Polina P. and Vaskin, Aleksandr and Reno, John L. and Keeler, Gordon A. and Sinclair, Michael B. and Staude, Isabelle and Brener, Igal},
abstractNote = {A frequency mixer is a nonlinear device that combines electromagnetic waves to create waves at new frequencies. Mixers are ubiquitous components in modern radio-frequency technology and microwave signal processing. The development of versatile frequency mixers for optical frequencies remains challenging: such devices generally rely on weak nonlinear optical processes and, thus, must satisfy phase-matching conditions. Here we utilize a GaAs-based dielectric metasurface to demonstrate an optical frequency mixer that concurrently generates eleven new frequencies spanning the ultraviolet to near-infrared. The even and odd order nonlinearities of GaAs enable our observation of second-harmonic, third-harmonic, and fourth-harmonic generation, sum-frequency generation, two-photon absorption-induced photoluminescence, four-wave mixing and six-wave mixing. The simultaneous occurrence of these seven nonlinear processes is assisted by the combined effects of strong intrinsic material nonlinearities, enhanced electromagnetic fields, and relaxed phase-matching requirements. In conclusion, such ultracompact optical mixers may enable a plethora of applications in biology, chemistry, sensing, communications, and quantum optics.},
doi = {10.1038/s41467-018-04944-9},
journal = {Nature Communications},
number = [1],
volume = [9],
place = {United States},
year = {2018},
month = {6}
}

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Cited by: 16 works
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Works referenced in this record:

Monolithic AlGaAs second-harmonic nanoantennas
journal, January 2016

  • Gili, V. F.; Carletti, L.; Locatelli, A.
  • Optics Express, Vol. 24, Issue 14, p. 15965-15971
  • DOI: 10.1364/OE.24.015965

Edge Nonlinear Optics on a MoS2 Atomic Monolayer
journal, May 2014


Quantum optics: Science and technology in a new light
journal, April 2015


Degenerate Four-Wave Mixing in a Multiresonant Germanium Nanodisk
journal, August 2017


Resonantly Enhanced Second-Harmonic Generation Using III–V Semiconductor All-Dielectric Metasurfaces
journal, August 2016


Observation of high-order harmonic generation in a bulk crystal
journal, December 2010

  • Ghimire, Shambhu; DiChiara, Anthony D.; Sistrunk, Emily
  • Nature Physics, Vol. 7, Issue 2
  • DOI: 10.1038/nphys1847

Phase matching using an isotropic nonlinear optical material
journal, January 1998

  • Fiore, A.; Berger, V.; Rosencher, E.
  • Nature, Vol. 391, Issue 6666
  • DOI: 10.1038/35091

Two-photon absorption and emission dynamics of bulk GaAs
journal, July 1989

  • Penzkofer, A.; Bugayev, A. A.
  • Optical and Quantum Electronics, Vol. 21, Issue 4
  • DOI: 10.1007/BF02027300

Attosecond science
journal, June 2007

  • Corkum, P. B.; Krausz, Ferenc
  • Nature Physics, Vol. 3, Issue 6
  • DOI: 10.1038/nphys620

Nonlinear metasurfaces: a paradigm shift in nonlinear optics
journal, January 2018


Ultrafast all-optical tuning of direct-gap semiconductor metasurfaces
journal, May 2017


Wavelength conversion by difference frequency generation in AlGaAs waveguides with periodic domain inversion achieved by wafer bonding
journal, May 1996

  • Yoo, S. J. B.; Caneau, C.; Bhat, R.
  • Applied Physics Letters, Vol. 68, Issue 19
  • DOI: 10.1063/1.116197

Nonlinear Generation of Vector Beams From AlGaAs Nanoantennas
journal, October 2016


Ultrafast nonlinear response of AlGaAs two-dimensional photonic crystal waveguides
journal, August 2003

  • Bristow, A. D.; Wells, J. -P. R.; Fan, W. H.
  • Applied Physics Letters, Vol. 83, Issue 5
  • DOI: 10.1063/1.1598647

Auger recombination in intrinsic GaAs
journal, January 1993

  • Strauss, U.; Rühle, W. W.; Köhler, K.
  • Applied Physics Letters, Vol. 62, Issue 1
  • DOI: 10.1063/1.108817

III–V Semiconductor Nanoresonators—A New Strategy for Passive, Active, and Nonlinear All‐Dielectric Metamaterials
journal, June 2016

  • Liu, Sheng; Keeler, Gordon A.; Reno, John L.
  • Advanced Optical Materials, Vol. 4, Issue 10
  • DOI: 10.1002/adom.201600240

Ultrafast All-Optical Switching with Magnetic Resonances in Nonlinear Dielectric Nanostructures
journal, September 2015

  • Shcherbakov, Maxim R.; Vabishchevich, Polina P.; Shorokhov, Alexander S.
  • Nano Letters, Vol. 15, Issue 10
  • DOI: 10.1021/acs.nanolett.5b02989

Experiments on second- and third-harmonic generation from magnetic metamaterials
journal, January 2007

  • Klein, Matthias W.; Wegener, Martin; Feth, Nils
  • Optics Express, Vol. 15, Issue 8
  • DOI: 10.1364/OE.15.005238

Optically resonant dielectric nanostructures
journal, November 2016

  • Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Brongersma, Mark L.
  • Science, Vol. 354, Issue 6314
  • DOI: 10.1126/science.aag2472

Microresonator-Based Optical Frequency Combs
journal, April 2011


Enhanced Third-Harmonic Generation in Silicon Nanoparticles Driven by Magnetic Response
journal, October 2014

  • Shcherbakov, Maxim R.; Neshev, Dragomir N.; Hopkins, Ben
  • Nano Letters, Vol. 14, Issue 11, p. 6488-6492
  • DOI: 10.1021/nl503029j

Plasmonics for extreme light concentration and manipulation
journal, February 2010

  • Schuller, Jon A.; Barnard, Edward S.; Cai, Wenshan
  • Nature Materials, Vol. 9, Issue 3
  • DOI: 10.1038/nmat2630

Phased-array sources based on nonlinear metamaterial nanocavities
journal, July 2015

  • Wolf, Omri; Campione, Salvatore; Benz, Alexander
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms8667

Nonlinear photonic metasurfaces
journal, March 2017


All-dielectric metamaterials
journal, January 2016


On the origin of third harmonic light from hybrid metal-dielectric nanoantennas
journal, September 2016


Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions
journal, July 2014

  • Lee, Jongwon; Tymchenko, Mykhailo; Argyropoulos, Christos
  • Nature, Vol. 511, Issue 7507
  • DOI: 10.1038/nature13455

Optical Frequency Mixing at Coupled Gold Nanoparticles
journal, January 2007


Ultrafast Optical Modulation of Second- and Third-Harmonic Generation from Cut-Disk-Based Metasurfaces
journal, June 2016


Broken Symmetry Dielectric Resonators for High Quality Factor Fano Metasurfaces
journal, November 2016


Ultrafast all-optical modulation in GaAs photonic crystal cavities
journal, January 2009

  • Husko, Chad; De Rossi, Alfredo; Combrié, Sylvain
  • Applied Physics Letters, Vol. 94, Issue 2
  • DOI: 10.1063/1.3068755

Mode matching in multiresonant plasmonic nanoantennas for enhanced second harmonic generation
journal, April 2015

  • Celebrano, Michele; Wu, Xiaofei; Baselli, Milena
  • Nature Nanotechnology, Vol. 10, Issue 5, p. 412-417
  • DOI: 10.1038/nnano.2015.69

Measurement of the nonlinear coefficient of orientation-patterned GaAs and demonstration of highly efficient second-harmonic generation
journal, January 2002

  • Skauli, T.; Vodopyanov, K. L.; Pinguet, T. J.
  • Optics Letters, Vol. 27, Issue 8
  • DOI: 10.1364/OL.27.000628

Quasi-phase-matched optical parametric oscillators in bulk periodically poled LiNbO_3
journal, January 1995

  • Myers, L. E.; Eckardt, R. C.; Fejer, M. M.
  • Journal of the Optical Society of America B, Vol. 12, Issue 11
  • DOI: 10.1364/JOSAB.12.002102

Magnetic light
journal, July 2012

  • Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Fu, Yuan Hsing
  • Scientific Reports, Vol. 2, Issue 1
  • DOI: 10.1038/srep00492

Colloquium : Nonlinear metamaterials
journal, September 2014

  • Lapine, Mikhail; Shadrivov, Ilya V.; Kivshar, Yuri S.
  • Reviews of Modern Physics, Vol. 86, Issue 3
  • DOI: 10.1103/RevModPhys.86.1093

Electromagnetic multipole theory for optical nanomaterials
journal, September 2012