Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering
Abstract
Abstract High‐efficiency and low‐cost perovskite solar cells (PVKSCs) are an ideal candidate for addressing the scalability challenge of solar‐based renewable energy. The dynamically evolving research field of PVKSCs has made immense progress in solving inherent challenges and capitalizing on their unique structure–property–processing–performance traits. This review offers a unique outlook on the paths toward commercialization of PVKSCs from the interfacial engineering perspective, relevant to both specialists and nonspecialists in the field through a brief introduction of the background of the field, current state‐of‐the‐art evolution, and future research prospects. The multifaceted role of interfaces in facilitating PVKSC development is explained. Beneficial impacts of diverse charge‐transporting materials and interfacial modifications are summarized. In addition, the role of interfaces in improving efficiency and stability for all emerging areas of PVKSC design are also evaluated. The authors' integral contributions in this area are highlighted on all fronts. Finally, future research opportunities for interfacial material development and applications along with scalability–durability–sustainability considerations pivotal for facilitating laboratory to industry translation are presented.
- Authors:
-
- Department of Materials Science and Engineering University of Washington Seattle WA 98195 USA
- Institute of Photovoltaics Nanchang University 999 Xuefu Avenue Nanchang 330031 China
- Department of Materials Science and Engineering University of Washington Seattle WA 98195 USA, Department of Materials Science and Engineering City University of Hong Kong Kowloon 999077 Hong Kong
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1463192
- Grant/Contract Number:
- DE‐EE 0006710
- Resource Type:
- Publisher's Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Name: Advanced Materials Journal Volume: 30 Journal Issue: 32; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley Blackwell (John Wiley & Sons)
- Country of Publication:
- Germany
- Language:
- English
Citation Formats
Rajagopal, Adharsh, Yao, Kai, and Jen, Alex K. ‐Y. Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering. Germany: N. p., 2018.
Web. doi:10.1002/adma.201800455.
Rajagopal, Adharsh, Yao, Kai, & Jen, Alex K. ‐Y. Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering. Germany. https://doi.org/10.1002/adma.201800455
Rajagopal, Adharsh, Yao, Kai, and Jen, Alex K. ‐Y. Fri .
"Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering". Germany. https://doi.org/10.1002/adma.201800455.
@article{osti_1463192,
title = {Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering},
author = {Rajagopal, Adharsh and Yao, Kai and Jen, Alex K. ‐Y.},
abstractNote = {Abstract High‐efficiency and low‐cost perovskite solar cells (PVKSCs) are an ideal candidate for addressing the scalability challenge of solar‐based renewable energy. The dynamically evolving research field of PVKSCs has made immense progress in solving inherent challenges and capitalizing on their unique structure–property–processing–performance traits. This review offers a unique outlook on the paths toward commercialization of PVKSCs from the interfacial engineering perspective, relevant to both specialists and nonspecialists in the field through a brief introduction of the background of the field, current state‐of‐the‐art evolution, and future research prospects. The multifaceted role of interfaces in facilitating PVKSC development is explained. Beneficial impacts of diverse charge‐transporting materials and interfacial modifications are summarized. In addition, the role of interfaces in improving efficiency and stability for all emerging areas of PVKSC design are also evaluated. The authors' integral contributions in this area are highlighted on all fronts. Finally, future research opportunities for interfacial material development and applications along with scalability–durability–sustainability considerations pivotal for facilitating laboratory to industry translation are presented.},
doi = {10.1002/adma.201800455},
journal = {Advanced Materials},
number = 32,
volume = 30,
place = {Germany},
year = {Fri Jun 08 00:00:00 EDT 2018},
month = {Fri Jun 08 00:00:00 EDT 2018}
}
https://doi.org/10.1002/adma.201800455
Web of Science
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Unraveling the High Open Circuit Voltage and High Performance of Integrated Perovskite/Organic Bulk-Heterojunction Solar Cells
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Defect Passivation of Organic–Inorganic Hybrid Perovskites by Diammonium Iodide toward High-Performance Photovoltaic Devices
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Effect of Photogenerated Dipoles in the Hole Transport Layer on Photovoltaic Performance of Organic-Inorganic Perovskite Solar Cells
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Efficient and Air-Stable Mixed-Cation Lead Mixed-Halide Perovskite Solar Cells with n-Doped Organic Electron Extraction Layers
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Achieving Large-Area Planar Perovskite Solar Cells by Introducing an Interfacial Compatibilizer
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Effects of interfacial characteristics on photovoltaic performance in CH 3 NH 3 PbBr 3 -based bulk perovskite solar cells with core/shell nanoarray as electron transporter
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Air-stable, hole-conductor-free high photocurrent perovskite solar cells with CH3NH3PbI3–NiO nanoparticles composite
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Efficient Semitransparent Perovskite Solar Cells for 23.0%-Efficiency Perovskite/Silicon Four-Terminal Tandem Cells
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Perovskite and Organic Solar Cells Fabricated by Inkjet Printing: Progress and Prospects
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Lead-Free Organic-Inorganic Hybrid Perovskites for Photovoltaic Applications: Recent Advances and Perspectives
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Perovskite ink with wide processing window for scalable high-efficiency solar cells
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Inverted Current-Voltage Hysteresis in Mixed Perovskite Solar Cells: Polarization, Energy Barriers, and Defect Recombination
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Dual Interfacial Modifications Enable High Performance Semitransparent Perovskite Solar Cells with Large Open Circuit Voltage and Fill Factor
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Phenylalkylamine Passivation of Organolead Halide Perovskites Enabling High-Efficiency and Air-Stable Photovoltaic Cells
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Non-Conjugated Polymer as an Efficient Dopant-Free Hole-Transporting Material for Perovskite Solar Cells
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Liquid Water- and Heat-Resistant Hybrid Perovskite Photovoltaics via an Inverted ALD Oxide Electron Extraction Layer Design
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Low Temperature Solution-Processed Sb:SnO 2 Nanocrystals for Efficient Planar Perovskite Solar Cells
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Emergence of highly transparent photovoltaics for distributed applications
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Perovskite/Silicon Tandem Solar Cells: Marriage of Convenience or True Love Story? - An Overview
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Contact Engineering: Electrode Materials for Highly Efficient and Stable Perovskite Solar Cells
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Identifying and suppressing interfacial recombination to achieve high open-circuit voltage in perovskite solar cells
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Making and Breaking of Lead Halide Perovskites
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A–D–A-type S,N-heteropentacene-based hole transport materials for dopant-free perovskite solar cells
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Hexagonal β-NaYF 4 :Yb 3+ , Er 3+ Nanoprism-Incorporated Upconverting Layer in Perovskite Solar Cells for Near-Infrared Sunlight Harvesting
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Synthesis and use of a hyper-connecting cross-linking agent in the hole-transporting layer of perovskite solar cells
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Cross-Linkable Fullerene Derivatives for Solution-Processed n–i–p Perovskite Solar Cells
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Light and Electrically Induced Phase Segregation and Its Impact on the Stability of Quadruple Cation High Bandgap Perovskite Solar Cells
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An Hydrophilic Anode Interlayer for Solution Processed Organohalide Perovskite Solar Cells
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Nonhazardous Solvent Systems for Processing Perovskite Photovoltaics
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Stabilized Wide Bandgap Perovskite Solar Cells by Tin Substitution
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Optoelectronic Quality and Stability of Hybrid Perovskites from MAPbI 3 to MAPbI 2 Br Using Composition Spread Libraries
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Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer
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Photoluminescence Lifetimes Exceeding 8 μs and Quantum Yields Exceeding 30% in Hybrid Perovskite Thin Films by Ligand Passivation
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Noncapacitive Hysteresis in Perovskite Solar Cells at Room Temperature
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Semi-transparent Perovskite Solar Cells Developed by Considering Human Luminosity Function
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Templated microstructural growth of perovskite thin films via colloidal monolayer lithography
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CuSCN-Based Inverted Planar Perovskite Solar Cell with an Average PCE of 15.6%
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Conjugated Small Molecule for Efficient Hole Transport in High-Performance p-i-n Type Perovskite Solar Cells
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