Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering

Rajagopal, Adharsh; Yao, Kai; Jen, Alex K. ‐Y.

doi:10.1002/adma.201800455

Title: Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering

Journal Article · 08 June 2018 · Advanced Materials

DOI: https://doi.org/10.1002/adma.201800455 · OSTI ID:1463192

Rajagopal, Adharsh ^[1]; Yao, Kai ^[2];

^[3]

Department of Materials Science and Engineering University of Washington Seattle WA 98195 USA
Institute of Photovoltaics Nanchang University 999 Xuefu Avenue Nanchang 330031 China
Department of Materials Science and Engineering University of Washington Seattle WA 98195 USA, Department of Materials Science and Engineering City University of Hong Kong Kowloon 999077 Hong Kong

Abstract High‐efficiency and low‐cost perovskite solar cells (PVKSCs) are an ideal candidate for addressing the scalability challenge of solar‐based renewable energy. The dynamically evolving research field of PVKSCs has made immense progress in solving inherent challenges and capitalizing on their unique structure–property–processing–performance traits. This review offers a unique outlook on the paths toward commercialization of PVKSCs from the interfacial engineering perspective, relevant to both specialists and nonspecialists in the field through a brief introduction of the background of the field, current state‐of‐the‐art evolution, and future research prospects. The multifaceted role of interfaces in facilitating PVKSC development is explained. Beneficial impacts of diverse charge‐transporting materials and interfacial modifications are summarized. In addition, the role of interfaces in improving efficiency and stability for all emerging areas of PVKSC design are also evaluated. The authors' integral contributions in this area are highlighted on all fronts. Finally, future research opportunities for interfacial material development and applications along with scalability–durability–sustainability considerations pivotal for facilitating laboratory to industry translation are presented.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: DE‐EE 0006710

OSTI ID:: 1463192

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Vol. 30 Journal Issue: 32; ISSN 0935-9648

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Cited by: 295 works

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High-Performance Flexible Perovskite Solar Cells on Ultrathin Glass: Implications of the TCO Dou, Benjia; Miller, Elisa M.; Christians, Jeffrey A. The Journal of Physical Chemistry Letters, Vol. 8, Issue 19 https://doi.org/10.1021/acs.jpclett.7b02128	journal	September 2017
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Reducing Hysteresis and Enhancing Performance of Perovskite Solar Cells Using Low-Temperature Processed Y-Doped SnO ₂ Nanosheets as Electron Selective Layers Yang, Guang; Lei, Hongwei; Tao, Hong Small, Vol. 13, Issue 2 https://doi.org/10.1002/smll.201601769	journal	November 2016
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Superflexible, high-efficiency perovskite solar cells utilizing graphene electrodes: towards future foldable power sources Yoon, Jungjin; Sung, Hyangki; Lee, Gunhee Energy & Environmental Science, Vol. 10, Issue 1 https://doi.org/10.1039/C6EE02650H	journal	January 2017
Low-Temperature Processed Electron Collection Layers of Graphene/TiO₂ Nanocomposites in Thin Film Perovskite Solar Cells Wang, Jacob Tse-Wei; Ball, James M.; Barea, Eva M. Nano Letters, Vol. 14, Issue 2, p. 724-730 https://doi.org/10.1021/nl403997a	journal	December 2013
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The Significance of Ion Conduction in a Hybrid Organic-Inorganic Lead-Iodide-Based Perovskite Photosensitizer Yang, Tae-Youl; Gregori, Giuliano; Pellet, Norman Angewandte Chemie International Edition, Vol. 54, Issue 27 https://doi.org/10.1002/anie.201500014	journal	May 2015
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Cooperative Effect of GO and Glucose on PEDOT:PSS for High V _OC and Hysteresis-Free Solution-Processed Perovskite Solar Cells Giuri, Antonella; Masi, Sofia; Colella, Silvia Advanced Functional Materials, Vol. 26, Issue 38 https://doi.org/10.1002/adfm.201603023	journal	August 2016
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Nanocrystalline Rutile Electron Extraction Layer Enables Low-Temperature Solution Processed Perovskite Photovoltaics with 13.7% Efficiency Yella, Aswani; Heiniger, Leo-Philipp; Gao, Peng Nano Letters, Vol. 14, Issue 5, p. 2591-2596 https://doi.org/10.1021/nl500399m	journal	April 2014
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Crosslinked Remote-Doped Hole-Extracting Contacts Enhance Stability under Accelerated Lifetime Testing in Perovskite Solar Cells Xu, Jixian; Voznyy, Oleksandr; Comin, Riccardo Advanced Materials, Vol. 28, Issue 14 https://doi.org/10.1002/adma.201505630	journal	January 2016
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Highly Efficient Electron Transport Obtained by Doping PCBM with Graphdiyne in Planar-Heterojunction Perovskite Solar Cells Kuang, Chaoyang; Tang, Gang; Jiu, Tonggang Nano Letters, Vol. 15, Issue 4 https://doi.org/10.1021/acs.nanolett.5b00787	journal	March 2015
Highly Efficient Integrated Perovskite Solar Cells Containing a Small Molecule-PC ₇₀ BM Bulk Heterojunction Layer with an Extended Photovoltaic Response Up to 900 nm Cheng, Ming; Chen, Cheng; Aitola, Kerttu Chemistry of Materials, Vol. 28, Issue 23 https://doi.org/10.1021/acs.chemmater.6b03564	journal	November 2016
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The Progress of Interface Design in Perovskite-Based Solar Cells Fan, Rundong; Huang, Yuan; Wang, Ligang Advanced Energy Materials, Vol. 6, Issue 17 https://doi.org/10.1002/aenm.201600460	journal	June 2016
Surface optimization to eliminate hysteresis for record efficiency planar perovskite solar cells Yang, Dong; Zhou, Xin; Yang, Ruixia Energy & Environmental Science, Vol. 9, Issue 10 https://doi.org/10.1039/C6EE02139E	journal	January 2016
Iodide-reduced graphene oxide with dopant-free spiro-OMeTAD for ambient stable and high-efficiency perovskite solar cells Luo, Qiang; Zhang, Ye; Liu, Chengyang Journal of Materials Chemistry A, Vol. 3, Issue 31 https://doi.org/10.1039/C5TA02710A	journal	January 2015
Dopant-free polymeric hole transport materials for highly efficient and stable perovskite solar cells Kim, Guan-Woo; Kang, Gyeongho; Kim, Jinseck Energy & Environmental Science, Vol. 9, Issue 7 https://doi.org/10.1039/C6EE00709K	journal	January 2016
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Overcoming ultraviolet light instability of sensitized TiO2 with meso-superstructured organometal tri-halide perovskite solar cells Leijtens, Tomas; Eperon, Giles E.; Pathak, Sandeep Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms3885	journal	December 2013
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Universal energy level tailoring of self-organized hole extraction layers in organic solar cells and organic–inorganic hybrid perovskite solar cells Lim, Kyung-Geun; Ahn, Soyeong; Kim, Young-Hoon Energy & Environmental Science, Vol. 9, Issue 3 https://doi.org/10.1039/C5EE03560K	journal	January 2016
CH3NH3PbI3 Perovskite Sensitized Solar Cells Using a D-A Copolymer as Hole Transport Material Nagarjuna, P.; Narayanaswamy, K.; Swetha, T. Electrochimica Acta, Vol. 151 https://doi.org/10.1016/j.electacta.2014.11.003	journal	January 2015
Induced Crystallization of Perovskites by a Perylene Underlayer for High-Performance Solar Cells Wang, Zhao-Kui; Gong, Xiu; Li, Meng ACS Nano, Vol. 10, Issue 5 https://doi.org/10.1021/acsnano.6b01904	journal	May 2016
Origin of the Thermal Instability in CH ₃ NH ₃ PbI ₃ Thin Films Deposited on ZnO Yang, Jinli; Siempelkamp, Braden D.; Mosconi, Edoardo Chemistry of Materials, Vol. 27, Issue 12 https://doi.org/10.1021/acs.chemmater.5b01598	journal	June 2015
Enhancement of the Performance of Perovskite Solar Cells, LEDs, and Optical Amplifiers by Anti-Solvent Additive Deposition Ngo, Thi Tuyen; Suarez, Isaac; Antonicelli, Gabriella Advanced Materials, Vol. 29, Issue 7 https://doi.org/10.1002/adma.201604056	journal	December 2016
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Oxygen Degradation in Mesoporous Al ₂ O ₃ /CH ₃ NH ₃ PbI _3- _x Cl _x Perovskite Solar Cells: Kinetics and Mechanisms Pearson, Andrew J.; Eperon, Giles E.; Hopkinson, Paul E. Advanced Energy Materials, Vol. 6, Issue 13 https://doi.org/10.1002/aenm.201600014	journal	April 2016
Improving Perovskite Solar Cells: Insights From a Validated Device Model Sherkar, Tejas S.; Momblona, Cristina; Gil-Escrig, Lidón Advanced Energy Materials, Vol. 7, Issue 13 https://doi.org/10.1002/aenm.201602432	journal	February 2017
Metal halide perovskites for energy applications Zhang, Wei; Eperon, Giles E.; Snaith, Henry J. Nature Energy, Vol. 1, Issue 6 https://doi.org/10.1038/nenergy.2016.48	journal	May 2016
Gas-Induced Formation/Transformation of Organic–Inorganic Halide Perovskites Zhou, Yuanyuan; Padture, Nitin P. ACS Energy Letters, Vol. 2, Issue 9 https://doi.org/10.1021/acsenergylett.7b00667	journal	August 2017
Low-cost solution-processed copper iodide as an alternative to PEDOT:PSS hole transport layer for efficient and stable inverted planar heterojunction perovskite solar cells Chen, Wei-Yi; Deng, Lin-Long; Dai, Si-Min Journal of Materials Chemistry A, Vol. 3, Issue 38 https://doi.org/10.1039/C5TA05286F	journal	January 2015
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Spiro-Phenylpyrazole-9,9′-Thioxanthene Analogues as Hole-Transporting Materials for Efficient Planar Perovskite Solar Cells Wang, Yang; Zhu, Zonglong; Chueh, Chu-Chen Advanced Energy Materials, Vol. 7, Issue 19 https://doi.org/10.1002/aenm.201700823	journal	June 2017
Nonstoichiometric Adduct Approach for High-Efficiency Perovskite Solar Cells Park, Nam-Gyu Inorganic Chemistry, Vol. 56, Issue 1 https://doi.org/10.1021/acs.inorgchem.6b01294	journal	October 2016
Interface engineering of highly efficient perovskite solar cells Zhou, H.; Chen, Q.; Li, G. Science, Vol. 345, Issue 6196 https://doi.org/10.1126/science.1254050	journal	July 2014
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Unraveling the High Open Circuit Voltage and High Performance of Integrated Perovskite/Organic Bulk-Heterojunction Solar Cells Dong, Shiqi; Liu, Yongsheng; Hong, Ziruo Nano Letters, Vol. 17, Issue 8 https://doi.org/10.1021/acs.nanolett.7b02532	journal	July 2017
Defect Passivation of Organic–Inorganic Hybrid Perovskites by Diammonium Iodide toward High-Performance Photovoltaic Devices Zhao, Ting; Chueh, Chu-Chen; Chen, Qi ACS Energy Letters, Vol. 1, Issue 4 https://doi.org/10.1021/acsenergylett.6b00327	journal	September 2016
Effect of Photogenerated Dipoles in the Hole Transport Layer on Photovoltaic Performance of Organic-Inorganic Perovskite Solar Cells Ahmadi, Mahshid; Hsiao, Yu-Che; Wu, Ting Advanced Energy Materials, Vol. 7, Issue 4 https://doi.org/10.1002/aenm.201601575	journal	October 2016
Efficient and Air-Stable Mixed-Cation Lead Mixed-Halide Perovskite Solar Cells with n-Doped Organic Electron Extraction Layers Wang, Zhiping; McMeekin, David P.; Sakai, Nobuya Advanced Materials, Vol. 29, Issue 5 https://doi.org/10.1002/adma.201604186	journal	December 2016
Achieving Large-Area Planar Perovskite Solar Cells by Introducing an Interfacial Compatibilizer Lee, Jinho; Kang, Hongkyu; Kim, Geunjin Advanced Materials, Vol. 29, Issue 22 https://doi.org/10.1002/adma.201606363	journal	April 2017
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Air-stable, hole-conductor-free high photocurrent perovskite solar cells with CH3NH3PbI3–NiO nanoparticles composite Wang, Yousheng; Rho, Won-Yeop; Yang, Hwa-Young Nano Energy, Vol. 27 https://doi.org/10.1016/j.nanoen.2016.08.006	journal	September 2016
Efficient Semitransparent Perovskite Solar Cells for 23.0%-Efficiency Perovskite/Silicon Four-Terminal Tandem Cells Chen, Bo; Bai, Yang; Yu, Zhengshan Advanced Energy Materials, Vol. 6, Issue 19 https://doi.org/10.1002/aenm.201601128	journal	July 2016
Perovskite and Organic Solar Cells Fabricated by Inkjet Printing: Progress and Prospects Peng, Xiaojin; Yuan, Jian; Shen, Shirley Advanced Functional Materials, Vol. 27, Issue 41 https://doi.org/10.1002/adfm.201703704	journal	September 2017
Lead-Free Organic-Inorganic Hybrid Perovskites for Photovoltaic Applications: Recent Advances and Perspectives Shi, Zejiao; Guo, Jia; Chen, Yonghua Advanced Materials, Vol. 29, Issue 16 https://doi.org/10.1002/adma.201605005	journal	February 2017
Perovskite ink with wide processing window for scalable high-efficiency solar cells Yang, Mengjin; Li, Zhen; Reese, Matthew O. Nature Energy, Vol. 2, Issue 5 https://doi.org/10.1038/nenergy.2017.38	journal	March 2017
Inverted Current-Voltage Hysteresis in Mixed Perovskite Solar Cells: Polarization, Energy Barriers, and Defect Recombination Tress, Wolfgang; Correa Baena, Juan Pablo; Saliba, Michael Advanced Energy Materials, Vol. 6, Issue 19 https://doi.org/10.1002/aenm.201600396	journal	July 2016
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Phenylalkylamine Passivation of Organolead Halide Perovskites Enabling High-Efficiency and Air-Stable Photovoltaic Cells Wang, Feng; Geng, Wei; Zhou, Yang Advanced Materials, Vol. 28, Issue 45 https://doi.org/10.1002/adma.201603062	journal	September 2016
Non-Conjugated Polymer as an Efficient Dopant-Free Hole-Transporting Material for Perovskite Solar Cells Xu, Yachao; Bu, Tongle; Li, Meijin ChemSusChem, Vol. 10, Issue 12 https://doi.org/10.1002/cssc.201700584	journal	May 2017
Liquid Water- and Heat-Resistant Hybrid Perovskite Photovoltaics via an Inverted ALD Oxide Electron Extraction Layer Design Kim, In Soo; Cao, Duyen H.; Buchholz, D. Bruce Nano Letters, Vol. 16, Issue 12 https://doi.org/10.1021/acs.nanolett.6b03989	journal	November 2016
Low Temperature Solution-Processed Sb:SnO ₂ Nanocrystals for Efficient Planar Perovskite Solar Cells Bai, Yang; Fang, Yanjun; Deng, Yehao ChemSusChem, Vol. 9, Issue 18 https://doi.org/10.1002/cssc.201600944	journal	August 2016
Emergence of highly transparent photovoltaics for distributed applications Traverse, Christopher J.; Pandey, Richa; Barr, Miles C. Nature Energy, Vol. 2, Issue 11 https://doi.org/10.1038/s41560-017-0016-9	journal	October 2017
Perovskite/Silicon Tandem Solar Cells: Marriage of Convenience or True Love Story? - An Overview Werner, Jérémie; Niesen, Bjoern; Ballif, Christophe Advanced Materials Interfaces, Vol. 5, Issue 1 https://doi.org/10.1002/admi.201700731	journal	September 2017
Contact Engineering: Electrode Materials for Highly Efficient and Stable Perovskite Solar Cells Xiao, Jia-Wen; Shi, Congbo; Zhou, Chenxiao Solar RRL, Vol. 1, Issue 9 https://doi.org/10.1002/solr.201700082	journal	August 2017
Identifying and suppressing interfacial recombination to achieve high open-circuit voltage in perovskite solar cells Correa-Baena, Juan-Pablo; Tress, Wolfgang; Domanski, Konrad Energy & Environmental Science, Vol. 10, Issue 5 https://doi.org/10.1039/C7EE00421D	journal	January 2017
Making and Breaking of Lead Halide Perovskites Manser, Joseph S.; Saidaminov, Makhsud I.; Christians, Jeffrey A. Accounts of Chemical Research, Vol. 49, Issue 2 https://doi.org/10.1021/acs.accounts.5b00455	journal	January 2016
A–D–A-type S,N-heteropentacene-based hole transport materials for dopant-free perovskite solar cells Steck, Christopher; Franckevičius, Marius; Zakeeruddin, Shaik Mohammed Journal of Materials Chemistry A, Vol. 3, Issue 34 https://doi.org/10.1039/C5TA03865K	journal	January 2015
Hexagonal β-NaYF ₄ :Yb ³⁺ , Er ³⁺ Nanoprism-Incorporated Upconverting Layer in Perovskite Solar Cells for Near-Infrared Sunlight Harvesting Roh, Jongmin; Yu, Haejun; Jang, Jyongsik ACS Applied Materials & Interfaces, Vol. 8, Issue 31 https://doi.org/10.1021/acsami.6b04760	journal	July 2016
Synthesis and use of a hyper-connecting cross-linking agent in the hole-transporting layer of perovskite solar cells Watson, Brian L.; Rolston, Nicholas; Bush, Kevin A. Journal of Materials Chemistry A, Vol. 5, Issue 36 https://doi.org/10.1039/C7TA05004F	journal	January 2017
Cross-Linkable Fullerene Derivatives for Solution-Processed n–i–p Perovskite Solar Cells Wojciechowski, Konrad; Ramirez, Ivan; Gorisse, Therese ACS Energy Letters, Vol. 1, Issue 4 https://doi.org/10.1021/acsenergylett.6b00229	journal	August 2016
Light and Electrically Induced Phase Segregation and Its Impact on the Stability of Quadruple Cation High Bandgap Perovskite Solar Cells Duong, The; Mulmudi, Hemant Kumar; Wu, YiLiang ACS Applied Materials & Interfaces, Vol. 9, Issue 32 https://doi.org/10.1021/acsami.7b06816	journal	August 2017
An Hydrophilic Anode Interlayer for Solution Processed Organohalide Perovskite Solar Cells Lin, Qianqian; Stoltzfus, Dani M.; Armin, Ardalan Advanced Materials Interfaces, Vol. 3, Issue 2 https://doi.org/10.1002/admi.201500420	journal	October 2015
Nonhazardous Solvent Systems for Processing Perovskite Photovoltaics Gardner, Kira L.; Tait, Jeffrey G.; Merckx, Tamara Advanced Energy Materials, Vol. 6, Issue 14 https://doi.org/10.1002/aenm.201600386	journal	May 2016
Stabilized Wide Bandgap Perovskite Solar Cells by Tin Substitution Yang, Zhibin; Rajagopal, Adharsh; Jo, Sae Byeok Nano Letters, Vol. 16, Issue 12 https://doi.org/10.1021/acs.nanolett.6b03857	journal	November 2016
Optoelectronic Quality and Stability of Hybrid Perovskites from MAPbI ₃ to MAPbI ₂ Br Using Composition Spread Libraries Braly, Ian L.; Hillhouse, Hugh W. The Journal of Physical Chemistry C, Vol. 120, Issue 2 https://doi.org/10.1021/acs.jpcc.5b10728	journal	January 2016
Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer Yeo, Jun-Seok; Kang, Rira; Lee, Sehyun Nano Energy, Vol. 12 https://doi.org/10.1016/j.nanoen.2014.12.022	journal	March 2015
Photoluminescence Lifetimes Exceeding 8 μs and Quantum Yields Exceeding 30% in Hybrid Perovskite Thin Films by Ligand Passivation deQuilettes, Dane W.; Koch, Susanne; Burke, Sven ACS Energy Letters, Vol. 1, Issue 2 https://doi.org/10.1021/acsenergylett.6b00236	journal	July 2016
Noncapacitive Hysteresis in Perovskite Solar Cells at Room Temperature Almora, Osbel; Aranda, Clara; Zarazua, Isaac ACS Energy Letters, Vol. 1, Issue 1 https://doi.org/10.1021/acsenergylett.6b00116	journal	June 2016
Semi-transparent Perovskite Solar Cells Developed by Considering Human Luminosity Function Kim, Gyu Min; Tatsuma, Tetsu Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-11193-1	journal	September 2017
Templated microstructural growth of perovskite thin films via colloidal monolayer lithography Hörantner, M. T.; Zhang, W.; Saliba, M. Energy & Environmental Science, Vol. 8, Issue 7 https://doi.org/10.1039/C5EE01169H	journal	January 2015
CuSCN-Based Inverted Planar Perovskite Solar Cell with an Average PCE of 15.6% Ye, Senyun; Sun, Weihai; Li, Yunlong Nano Letters, Vol. 15, Issue 6 https://doi.org/10.1021/acs.nanolett.5b00116	journal	May 2015
Conjugated Small Molecule for Efficient Hole Transport in High-Performance p-i-n Type Perovskite Solar Cells Yang, Liyan; Cai, Feilong; Yan, Yu Advanced Functional Materials, Vol. 27, Issue 31 https://doi.org/10.1002/adfm.201702613	journal	July 2017

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Journal Article · 2023 · Chemical Reviews · OSTI ID:1975377

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