Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics

Li, Fei; Zhang, Shujun; Damjanovic, Dragan; Chen, Long‐Qing; Shrout, Thomas R.

doi:10.1002/adfm.201801504

Title: Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics

Authors:

^[1]; Zhang, Shujun ^[2]; Damjanovic, Dragan ^[3]; Chen, Long‐Qing ^[4]; Shrout, Thomas R. ^[4]

Electronic Materials Research Laboratory Key Laboratory of the Ministry of Education and International Center for Dielectric Research School of Electronic and Information Engineering State Key Laboratory for Mechanical Behaviour of Materials Xi'an Jiaotong University Xi'an 710049 China, Materials Research Institute Pennsylvania State University University Park PA 16802 USA
Materials Research Institute Pennsylvania State University University Park PA 16802 USA, Institute for Superconducting and Electronic Materials Australia Institute of Innovative Materials University of Wollongong NSW 2500 Australia
Group for Ferroelectrics and Functional Oxides Swiss Federal Institute of Technology in Lausanne‐EPFL 1015 Lausanne Switzerland
Materials Research Institute Pennsylvania State University University Park PA 16802 USA

Publication Date:: 2018-07-29

Sponsoring Org.:: USDOE

OSTI Identifier:: 1462121

Grant/Contract Number:: DE‐FG02‐07ER46417

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Advanced Functional Materials

Additional Journal Information:: Journal Name: Advanced Functional Materials Journal Volume: 28 Journal Issue: 37; Journal ID: ISSN 1616-301X

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: Germany

Language:: English

Citation Formats


                    Li, Fei, Zhang, Shujun, Damjanovic, Dragan, Chen, Long‐Qing, and Shrout, Thomas R. Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics.  Germany: N. p., 2018. 
Web.  doi:10.1002/adfm.201801504.

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                    Li, Fei, Zhang, Shujun, Damjanovic, Dragan, Chen, Long‐Qing, & Shrout, Thomas R. Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics.  Germany.  https://doi.org/10.1002/adfm.201801504

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                    Li, Fei, Zhang, Shujun, Damjanovic, Dragan, Chen, Long‐Qing, and Shrout, Thomas R. Sun .  
"Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics".  Germany.  https://doi.org/10.1002/adfm.201801504.

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@article{osti_1462121,

  title        = {Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics},

  author       = {Li, Fei and Zhang, Shujun and Damjanovic, Dragan and Chen, Long‐Qing and Shrout, Thomas R.},

  abstractNote = {},

  doi          = {10.1002/adfm.201801504},

  journal      = {Advanced Functional Materials},

  number       = 37,

  volume       = 28,

  place        = {Germany},

  year         = {2018},

  month        = {7}

}

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Title: Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics

Citation Formats

Investigation of piezoelectric property and nanodomain structures for PIN–PZ–PMN–PT single crystals as a function of crystallographic orientation and temperature journal, January 2017

Large electrostrictive effects in relaxor ferroelectrics journal, January 1980

Dielectric properties of tetragonal lanthanum modified lead zirconate titanate ceramics journal, September 1993

Relaxor Ferroelectric Complex Perovskites: Structure, Properties and Phase Transitions journal, February 1998

Importance of random fields on the properties and ferroelectric phase stability of 〈001〉 oriented 0.7 Pb(Mg1/3Nb2/3)O3–0.3 PbTiO3 crystals journal, May 2001

Symmetry of piezoelectric ( 1 − x )Pb(Mg 1 / 3 Nb 2 / 3 )O 3 - x PbTiO 3 ( x = 0.31 ) single crystal at different length scales in the morphotropic phase boundary region journal, November 2012

Domain glasses: Twin planes, Bloch lines, and Bloch points: Domain glasses - twin planes, Bloch lines, and Bloch points journal, August 2015

Electrostrictive effect in Pb(Mg 1/3 Nb 2/3 )O 3 -x PbTiO 3 crystals journal, April 2013

Thin-film ferroelectric materials and their applications journal, November 2016

Structural origin of room temperature poling enhanced piezoelectricity in modified Pb(Mg 1/3 Nb 2/3 )O 3 -30%PbTiO 3 crystals journal, June 2017

Ferroic glasses journal, October 2017

Phonon localization drives polar nanoregions in a relaxor ferroelectric journal, April 2014

Antiferroelectric phase transitions in single crystals PbZrO 3 :Sn revisited journal, January 2014

Dielectric relaxation in solids journal, January 1999

Enhanced energy storage properties of {Bi0.5[(Na0.8K0.2)1-Li ]0.5}0.96Sr0.04(Ti1--Ta Nb )O3 lead-free ceramics journal, November 2017

Static and dynamic polar nanoregions in relaxor ferroelectric Ba(Ti 1 − x Sn x )O 3 system at high temperature journal, January 2012

The Antiferroelectric ↔ Ferroelectric Phase Transition in Lead-Containing and Lead-Free Perovskite Ceramics journal, November 2011

Anisotropic Local Correlations and Dynamics in a Relaxor Ferroelectric journal, April 2013

High performance ferroelectric relaxor-PbTiO 3 single crystals: Status and perspective journal, February 2012

What is a ferroelectric–a materials designer perspective journal, August 2016

Compositional heterogeneity and the origins of the multicell cubic state in Sn‐doped lead zirconate titanate ceramics journal, April 1994

Glassy polarization behavior in ferroelectric compounds and journal, December 1983

Enhanced energy storage performance in (Pb0.858Ba0.1La0.02Y0.008)(Zr0.65Sn0.3Ti0.05)O3–(Pb0.97La0.02)(Zr0.9Sn0.05Ti0.05)O3 anti-ferroelectric composite ceramics by Spark Plasma Sintering journal, February 2015

Random Fields in Relaxor Ferroelectrics — a Jubilee Review journal, April 2012

Enhanced electromechanical response of ferroelectrics due to charged domain walls journal, January 2012

Nanodomain structure of Pb [ Zr 1 − x Ti x ] O 3 at its morphotropic phase boundary: Investigations from local to average structure journal, May 2007

Relationship between local structure and phase transitions of a disordered solid solution journal, October 2002

Dipolar-glass model for lead magnesium niobate journal, April 1991

NMR Evidence for the Coexistence of Order-Disorder and Displacive Components in Barium Titanate journal, January 2003

Doped Pb(Zr,Sn,Ti)O 3 Slim-Loop Ferroelectric Ceramics for High-Power Pulse Capacitors Application journal, May 2008

The role of B‐site cation disorder in diffuse phase transition behavior of perovskite ferroelectrics journal, August 1980

Dielectric and pyroelectric properties of the morphotropic phase boundary lead barium niobate (PBN) single crystals at low temperature (10–300 K) journal, May 1990

Contributions to the Piezoelectric Effect in Ferroelectric Single Crystals and Ceramics journal, October 2005

Phase coexistence and electric-field control of toroidal order in oxide superlattices journal, August 2017

A compositional fluctuation and properties of Pb(Zr, Ti)O3 journal, December 1977

Critical Property in Relaxor-PbTiO3 Single Crystals - Shear Piezoelectric Response journal, April 2011

The relaxational properties of compositionally disordered ABO 3 perovskites journal, February 2003

Tem observation of polar domains in relaxor ferroelectric Pb(Mg 1/3 Nb 2/3 )O 3 journal, September 1998

Direct Observation of the Formation of Polar Nanoregions in Pb ( Mg 1 / 3 Nb 2 / 3 ) O 3 Using Neutron Pair Distribution Function Analysis journal, April 2005

Finite-temperature properties of the relaxor PbMg 1 / 3 Nb 2 / 3 O 3 from atomistic simulations journal, June 2015

Relaxor Ferroelectric-Based Electrocaloric Polymer Nanocomposites with a Broad Operating Temperature Range and High Cooling Energy journal, February 2015

A structural evidence of polar clusters in PLZT relaxor ceramics journal, July 2016

Large strain response based on relaxor-antiferroelectric coherence in Bi 0.5 Na 0.5 TiO 3 –SrTiO 3 –(K 0.5 Na 0.5 )NbO 3 solid solutions journal, November 2014

Structural and dielectric relaxor properties of yttrium-doped Ba(Zr0.25Ti0.75)O3 ceramics journal, May 2010

Dielectric relaxor and ferroelectric relaxor: Bi-doped paraelectric SrTiO3 journal, February 2002

Lead-Free Relaxor Ferroelectrics journal, December 2011

Polarization and depolarization behavior of hot pressed lead lanthanum zirconate titanate ceramics journal, June 1983

Contribution of the irreversible displacement of domain walls to the piezoelectric effect in barium titanate and lead zirconate titanate ceramics journal, June 1997

Dielectric Relaxation in Relaxor Ferroelectrics journal, April 2012

Microscopic origins of the large piezoelectricity of leadfree (Ba,Ca)(Zr,Ti)O3 journal, June 2017

Response of polar nanoregions in 68%Pb(Mg1∕3Nb2∕3)O3-32%PbTiO3 to a [001] electric field journal, August 2008

Optical and dielectric relaxor behaviour of Ba(Zr 0.25 Ti 0.75 )O 3 ceramic explained by means of distorted clusters journal, August 2009

Improved Energy Storage Performance and Fatigue Endurance of Sr-Doped PbZrO 3 Antiferroelectric Thin Films journal, May 2009

Large Piezoelectric Effect in Pb-Free Ceramics journal, December 2009

Finite-Temperature Properties of Ba ( Zr , Ti ) O 3 Relaxors from First Principles journal, June 2012

Average and local structure of the Pb-free ferroelectric perovskites ( Sr , Sn ) TiO 3 and ( Ba , Ca , Sn ) TiO 3 journal, December 2015

Elastic softening and polarization memory in PZN-PT relaxor ferroelectrics journal, November 2011

Domain boundary-dominated systems: adaptive structures and functional twin boundaries journal, July 2014

Fluctuating defects in the incipient relaxor K 1 − x Li x TaO 3 ( x = 0.02 ) journal, December 2014

Relaxor ferroelectric devices journal, January 1994

Relaxorferroelectrics: An overview journal, January 1994

Twinning in ferroelectric and ferroelastic ceramics: stress relief journal, June 1990

Origin of polar nanoregions in relaxor ferroelectrics: Nonlinearity, discrete breather formation, and charge transfer journal, May 2011

A random field theory based model for ferroelectric relaxors journal, September 1996

Dielectric properties and field-induced phase switching of lead zirconate titanate stannate antiferroelectric thick films on silicon substrates journal, March 2000

Elastic excitations in BaTiO 3 single crystals and ceramics: Mobile domain boundaries and polar nanoregions observed by resonant ultrasonic spectroscopy journal, January 2013

State transition and electrocaloric effect of BaZr x Ti 1− x O 3 : Simulation and experiment journal, January 2017

Observation of polar vortices in oxide superlattices journal, January 2016

Diffuse phase transition and dielectric tunability of Ba(ZryTi1−y)O3 relaxor ferroelectric ceramics journal, October 2004

Interpretation of the diffuse scattering in Pb-based relaxor ferroelectrics in terms of three-dimensional nanodomains of the ⟨110⟩-directed relative interdomain atomic shifts journal, July 2007

Phase Transition in the Near-Surface Region of Ternary Pb ( In 1 / 2 Nb 1 / 2 ) O 3 − Pb ( Mg 1 / 3 Nb 2 / 3 ) O 3 − PbTiO 3 Relaxor Ferroelectric Crystals journal, September 2017

Theory and experimental evidence of phonon domains and their roles in pre-martensitic phenomena journal, December 2015

Effect of Ba Content on the Stress Sensitivity of the Antiferroelectric to Ferroelectric Phase Transition in (Pb,La,Ba,)(Zr,Sn,Ti)O 3 Ceramics journal, September 2013

Phase transitions in bismuth-modified silver niobate ceramics for high power energy storage journal, January 2017

Large strain and high energy storage density in orthorhombic perovskite (Pb0.97La0.02)(Zr1−x−ySnxTiy)O3 antiferroelectric thin films journal, October 2010

On short range ordering in the perovskite lead magnesium niobate journal, August 1990

Compressible spherical dipolar glass model of relaxor ferroelectrics journal, December 2012

Organic and inorganic relaxor ferroelectrics with giant electrocaloric effect journal, October 2010

Investigation of piezoelectric property and nanodomain structures for PIN–PZ–PMN–PT single crystals as a function of crystallographic orientation and temperature
journal, January 2017

Large electrostrictive effects in relaxor ferroelectrics
journal, January 1980

Dielectric properties of tetragonal lanthanum modified lead zirconate titanate ceramics
journal, September 1993

Relaxor Ferroelectric Complex Perovskites: Structure, Properties and Phase Transitions
journal, February 1998

Importance of random fields on the properties and ferroelectric phase stability of 〈001〉 oriented 0.7 Pb(Mg1/3Nb2/3)O3–0.3 PbTiO3 crystals
journal, May 2001

Symmetry of piezoelectric ( $1 - x$ )Pb(Mg $_{1 / 3}$ Nb $_{2 / 3}$ )O $_{3}$ - $x$ PbTiO $_{3}$ ( $x = 0.31$ ) single crystal at different length scales in the morphotropic phase boundary region
journal, November 2012

Domain glasses: Twin planes, Bloch lines, and Bloch points: Domain glasses - twin planes, Bloch lines, and Bloch points
journal, August 2015

Electrostrictive effect in Pb(Mg _1/3 Nb _2/3 )O ₃ -x PbTiO ₃ crystals
journal, April 2013

Thin-film ferroelectric materials and their applications
journal, November 2016

Structural origin of room temperature poling enhanced piezoelectricity in modified Pb(Mg _1/3 Nb _2/3 )O ₃ -30%PbTiO ₃ crystals
journal, June 2017

Ferroic glasses
journal, October 2017

Phonon localization drives polar nanoregions in a relaxor ferroelectric
journal, April 2014

Antiferroelectric phase transitions in single crystals PbZrO ₃ :Sn revisited
journal, January 2014

Dielectric relaxation in solids
journal, January 1999

Enhanced energy storage properties of {Bi0.5[(Na0.8K0.2)1-Li ]0.5}0.96Sr0.04(Ti1--Ta Nb )O3 lead-free ceramics
journal, November 2017

Static and dynamic polar nanoregions in relaxor ferroelectric Ba(Ti $_{1 - x}$ Sn $_{x}$ )O $_{3}$ system at high temperature
journal, January 2012

The Antiferroelectric ↔ Ferroelectric Phase Transition in Lead-Containing and Lead-Free Perovskite Ceramics
journal, November 2011

Anisotropic Local Correlations and Dynamics in a Relaxor Ferroelectric
journal, April 2013

High performance ferroelectric relaxor-PbTiO ₃ single crystals: Status and perspective
journal, February 2012

What is a ferroelectric–a materials designer perspective
journal, August 2016

Compositional heterogeneity and the origins of the multicell cubic state in Sn‐doped lead zirconate titanate ceramics
journal, April 1994

Glassy polarization behavior in ferroelectric compounds and
journal, December 1983

Enhanced energy storage performance in (Pb0.858Ba0.1La0.02Y0.008)(Zr0.65Sn0.3Ti0.05)O3–(Pb0.97La0.02)(Zr0.9Sn0.05Ti0.05)O3 anti-ferroelectric composite ceramics by Spark Plasma Sintering
journal, February 2015

Random Fields in Relaxor Ferroelectrics — a Jubilee Review
journal, April 2012

Enhanced electromechanical response of ferroelectrics due to charged domain walls
journal, January 2012

Nanodomain structure of $Pb [{Zr}_{1 - x} {Ti}_{x}] O_{3}$ at its morphotropic phase boundary: Investigations from local to average structure
journal, May 2007

Relationship between local structure and phase transitions of a disordered solid solution
journal, October 2002

Dipolar-glass model for lead magnesium niobate
journal, April 1991

NMR Evidence for the Coexistence of Order-Disorder and Displacive Components in Barium Titanate
journal, January 2003

Doped Pb(Zr,Sn,Ti)O ₃ Slim-Loop Ferroelectric Ceramics for High-Power Pulse Capacitors Application
journal, May 2008

The role of B‐site cation disorder in diffuse phase transition behavior of perovskite ferroelectrics
journal, August 1980

Dielectric and pyroelectric properties of the morphotropic phase boundary lead barium niobate (PBN) single crystals at low temperature (10–300 K)
journal, May 1990

Contributions to the Piezoelectric Effect in Ferroelectric Single Crystals and Ceramics
journal, October 2005

Phase coexistence and electric-field control of toroidal order in oxide superlattices
journal, August 2017

A compositional fluctuation and properties of Pb(Zr, Ti)O3
journal, December 1977

Critical Property in Relaxor-PbTiO3 Single Crystals - Shear Piezoelectric Response
journal, April 2011

The relaxational properties of compositionally disordered ABO ₃ perovskites
journal, February 2003

Tem observation of polar domains in relaxor ferroelectric Pb(Mg _1/3 Nb _2/3 )O ₃
journal, September 1998

Direct Observation of the Formation of Polar Nanoregions in $Pb ({Mg}_{1 / 3} {Nb}_{2 / 3}) O_{3}$ Using Neutron Pair Distribution Function Analysis
journal, April 2005

Finite-temperature properties of the relaxor ${PbMg}_{1 / 3} {Nb}_{2 / 3} O_{3}$ from atomistic simulations
journal, June 2015

Relaxor Ferroelectric-Based Electrocaloric Polymer Nanocomposites with a Broad Operating Temperature Range and High Cooling Energy
journal, February 2015

A structural evidence of polar clusters in PLZT relaxor ceramics
journal, July 2016

Large strain response based on relaxor-antiferroelectric coherence in Bi _0.5 Na _0.5 TiO ₃ –SrTiO ₃ –(K _0.5 Na _0.5 )NbO ₃ solid solutions
journal, November 2014

Structural and dielectric relaxor properties of yttrium-doped Ba(Zr0.25Ti0.75)O3 ceramics
journal, May 2010

Dielectric relaxor and ferroelectric relaxor: Bi-doped paraelectric SrTiO3
journal, February 2002

Lead-Free Relaxor Ferroelectrics
journal, December 2011

Polarization and depolarization behavior of hot pressed lead lanthanum zirconate titanate ceramics
journal, June 1983

Contribution of the irreversible displacement of domain walls to the piezoelectric effect in barium titanate and lead zirconate titanate ceramics
journal, June 1997

Dielectric Relaxation in Relaxor Ferroelectrics
journal, April 2012

Microscopic origins of the large piezoelectricity of leadfree (Ba,Ca)(Zr,Ti)O3
journal, June 2017

Response of polar nanoregions in 68%Pb(Mg1∕3Nb2∕3)O3-32%PbTiO3 to a [001] electric field
journal, August 2008

Optical and dielectric relaxor behaviour of Ba(Zr _0.25 Ti _0.75 )O ₃ ceramic explained by means of distorted clusters
journal, August 2009

Improved Energy Storage Performance and Fatigue Endurance of Sr-Doped PbZrO ₃ Antiferroelectric Thin Films
journal, May 2009

Large Piezoelectric Effect in Pb-Free Ceramics
journal, December 2009

Finite-Temperature Properties of $Ba (Zr, Ti) O_{3}$ Relaxors from First Principles
journal, June 2012

Average and local structure of the Pb-free ferroelectric perovskites ${(Sr, Sn) TiO}_{3}$ and $(Ba, Ca, Sn) {TiO}_{3}$
journal, December 2015

Elastic softening and polarization memory in PZN-PT relaxor ferroelectrics
journal, November 2011

Domain boundary-dominated systems: adaptive structures and functional twin boundaries
journal, July 2014

Fluctuating defects in the incipient relaxor $K_{1 - x} {Li}_{x} {TaO}_{3}$ $(x = 0.02)$
journal, December 2014

Relaxor ferroelectric devices
journal, January 1994

Relaxorferroelectrics: An overview
journal, January 1994

Twinning in ferroelectric and ferroelastic ceramics: stress relief
journal, June 1990

Origin of polar nanoregions in relaxor ferroelectrics: Nonlinearity, discrete breather formation, and charge transfer
journal, May 2011

A random field theory based model for ferroelectric relaxors
journal, September 1996

Dielectric properties and field-induced phase switching of lead zirconate titanate stannate antiferroelectric thick films on silicon substrates
journal, March 2000

Elastic excitations in BaTiO $_{3}$ single crystals and ceramics: Mobile domain boundaries and polar nanoregions observed by resonant ultrasonic spectroscopy
journal, January 2013

State transition and electrocaloric effect of BaZr _x Ti _{1− x} O ₃ : Simulation and experiment
journal, January 2017

Observation of polar vortices in oxide superlattices
journal, January 2016

Diffuse phase transition and dielectric tunability of Ba(ZryTi1−y)O3 relaxor ferroelectric ceramics
journal, October 2004

Interpretation of the diffuse scattering in Pb-based relaxor ferroelectrics in terms of three-dimensional nanodomains of the ⟨110⟩-directed relative interdomain atomic shifts
journal, July 2007

Phase Transition in the Near-Surface Region of Ternary $Pb ({In}_{1 / 2} {Nb}_{1 / 2}) O_{3} − Pb ({Mg}_{1 / 3} {Nb}_{2 / 3}) O_{3} − {PbTiO}_{3}$ Relaxor Ferroelectric Crystals
journal, September 2017

Theory and experimental evidence of phonon domains and their roles in pre-martensitic phenomena
journal, December 2015

Effect of Ba Content on the Stress Sensitivity of the Antiferroelectric to Ferroelectric Phase Transition in (Pb,La,Ba,)(Zr,Sn,Ti)O ₃ Ceramics
journal, September 2013

Phase transitions in bismuth-modified silver niobate ceramics for high power energy storage
journal, January 2017

Large strain and high energy storage density in orthorhombic perovskite (Pb0.97La0.02)(Zr1−x−ySnxTiy)O3 antiferroelectric thin films
journal, October 2010

On short range ordering in the perovskite lead magnesium niobate
journal, August 1990

Compressible spherical dipolar glass model of relaxor ferroelectrics
journal, December 2012

Organic and inorganic relaxor ferroelectrics with giant electrocaloric effect
journal, October 2010

Cryogenic dielectric and piezoelectric activities in rhombohedral (1 − x )Pb(Mg _1/3 Nb _2/3 )O ₃ – x PbTiO ₃ single crystals with different crystallographic orientations
journal, August 2009

Nonlinear dynamics of polar regions in paraelectric phase of (Ba _1-x ,Sr _x )TiO ₃ ceramics
journal, May 2017