DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Photoluminescence and gain/absorption spectra of a driven-dissipative electron-hole-photon condensate

Abstract

Here, we investigate theoretically nonequilibrium effects on photoluminescence and gain/absorption spectra of a driven-dissipative exciton-polariton condensate, by employing the combined Hartree-Fock-Bogoliubov theory with the generalized random phase approximation extended to the Keldysh formalism. Our calculated photoluminescence spectra is in semiquantitative agreement with experiments, where features such as a blue shift of the emission from the condensate, the appearance of the dispersionless feature of a diffusive Goldstone mode, and the suppression of the dispersive profile of the mode are obtained. We show that the nonequilibrium nature of the exciton-polariton condensate strongly suppresses the visibility of the Bogoliubov dispersion in the negative energy branch (ghost branch) in photoluminescence spectra. We also show that the trace of this branch can be captured as a hole burning effect in gain/absorption spectra. Our results indicate that the nonequilibrium nature of the exciton-polariton condensate strongly reduces quantum depletion, while a scattering channel to the ghost branch is still present.

Authors:
 [1];  [2];  [3]
  1. Osaka Univ., Toyonaka (Japan); Univ. of Chicago, Chicago, IL (United States)
  2. Univ. of Chicago, Chicago, IL (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
  3. Keio Univ., Yokohama (Japan)
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Japan Society for the Promotion of Science (JSPS)
OSTI Identifier:
1461540
Alternate Identifier(s):
OSTI ID: 1439916
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 97; Journal Issue: 24; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS

Citation Formats

Hanai, Ryo, Littlewood, Peter B., and Ohashi, Yoji. Photoluminescence and gain/absorption spectra of a driven-dissipative electron-hole-photon condensate. United States: N. p., 2018. Web. doi:10.1103/PhysRevB.97.245302.
Hanai, Ryo, Littlewood, Peter B., & Ohashi, Yoji. Photoluminescence and gain/absorption spectra of a driven-dissipative electron-hole-photon condensate. United States. https://doi.org/10.1103/PhysRevB.97.245302
Hanai, Ryo, Littlewood, Peter B., and Ohashi, Yoji. Fri . "Photoluminescence and gain/absorption spectra of a driven-dissipative electron-hole-photon condensate". United States. https://doi.org/10.1103/PhysRevB.97.245302. https://www.osti.gov/servlets/purl/1461540.
@article{osti_1461540,
title = {Photoluminescence and gain/absorption spectra of a driven-dissipative electron-hole-photon condensate},
author = {Hanai, Ryo and Littlewood, Peter B. and Ohashi, Yoji},
abstractNote = {Here, we investigate theoretically nonequilibrium effects on photoluminescence and gain/absorption spectra of a driven-dissipative exciton-polariton condensate, by employing the combined Hartree-Fock-Bogoliubov theory with the generalized random phase approximation extended to the Keldysh formalism. Our calculated photoluminescence spectra is in semiquantitative agreement with experiments, where features such as a blue shift of the emission from the condensate, the appearance of the dispersionless feature of a diffusive Goldstone mode, and the suppression of the dispersive profile of the mode are obtained. We show that the nonequilibrium nature of the exciton-polariton condensate strongly suppresses the visibility of the Bogoliubov dispersion in the negative energy branch (ghost branch) in photoluminescence spectra. We also show that the trace of this branch can be captured as a hole burning effect in gain/absorption spectra. Our results indicate that the nonequilibrium nature of the exciton-polariton condensate strongly reduces quantum depletion, while a scattering channel to the ghost branch is still present.},
doi = {10.1103/PhysRevB.97.245302},
journal = {Physical Review B},
number = 24,
volume = 97,
place = {United States},
year = {Fri Jun 01 00:00:00 EDT 2018},
month = {Fri Jun 01 00:00:00 EDT 2018}
}

Journal Article:

Citation Metrics:
Cited by: 17 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

From Single Particle to Superfluid Excitations in a Dissipative Polariton Gas
journal, June 2011


Temperature dependence of pulsed polariton lasing in a GaAs microcavity
journal, August 2012


Dynamical instability of a driven-dissipative electron-hole condensate in the BCS-BEC crossover region
journal, September 2017


Exciton-polariton Bose-Einstein condensation
journal, May 2010


Polariton lasing vs. photon lasing in a semiconductor microcavity
journal, December 2003

  • Deng, H.; Weihs, G.; Snoke, D.
  • Proceedings of the National Academy of Sciences, Vol. 100, Issue 26
  • DOI: 10.1073/pnas.2634328100

Nonequilibrium condensates and lasers without inversion: Exciton-polariton lasers
journal, June 1996


Characterization of two-threshold behavior of the emission from a GaAs microcavity
journal, February 2012


Field theories with « Superconductor » solutions
journal, January 1961


Temperature Dependence of Highly Excited Exciton Polaritons in Semiconductor Microcavities
journal, August 2013

  • Horikiri, Tomoyuki; Matsuo, Yasuhiro; Shikano, Yutaka
  • Journal of the Physical Society of Japan, Vol. 82, Issue 8
  • DOI: 10.7566/JPSJ.82.084709

Room-Temperature Polariton Lasing in All-Inorganic Perovskite Nanoplatelets
journal, May 2017


Lasing threshold doubling at the crossover from strong to weak coupling regime in GaAs microcavity
journal, February 2012


BCS Wave-Function Approach to the BEC-BCS Crossover of Exciton-Polariton Condensates
journal, October 2010


Nonequilibrium Quantum Condensation in an Incoherently Pumped Dissipative System
journal, June 2006


Excitations in a Nonequilibrium Bose-Einstein Condensate of Exciton Polaritons
journal, October 2007


Bose condensation in an attractive fermion gas: From weak to strong coupling superconductivity
journal, May 1985

  • Nozi�res, P.; Schmitt-Rink, S.
  • Journal of Low Temperature Physics, Vol. 59, Issue 3-4
  • DOI: 10.1007/BF00683774

Algebraic order and the Berezinskii-Kosterlitz-Thouless transition in an exciton-polariton gas
journal, November 2014


Quantized vortices in an exciton–polariton condensate
journal, August 2008

  • Lagoudakis, K. G.; Wouters, M.; Richard, M.
  • Nature Physics, Vol. 4, Issue 9
  • DOI: 10.1038/nphys1051

Observation of the Transition from Lasing Driven by a Bosonic to a Fermionic Reservoir in a GaAs Quantum Well Microcavity
journal, September 2016


Blueshifted Flat Dispersion Relation of Exciton–Polariton Condensates in a CuBr Microcavity
journal, May 2016

  • Nakayama, Masaaki; Murakami, Katsuya; Kim, DaeGwi
  • Journal of the Physical Society of Japan, Vol. 85, Issue 5
  • DOI: 10.7566/JPSJ.85.054702

Crossover from photon to exciton-polariton lasing
journal, October 2012


Microscopic theory of equilibrium polariton condensates
journal, December 2016


Higher order coherence of exciton-polariton condensates
journal, January 2010

  • Horikiri, Tomoyuki; Schwendimann, Paolo; Quattropani, Antonio
  • Physical Review B, Vol. 81, Issue 3
  • DOI: 10.1103/PhysRevB.81.033307

Resonance Superfluidity in a Quantum Degenerate Fermi Gas
journal, August 2001


Condensation of Pairs of Fermionic Atoms near a Feshbach Resonance
journal, March 2004


Highly excited exciton-polariton condensates
journal, June 2017


Exciton–polariton condensates
journal, October 2014

  • Byrnes, Tim; Kim, Na Young; Yamamoto, Yoshihisa
  • Nature Physics, Vol. 10, Issue 11
  • DOI: 10.1038/nphys3143

Superfluidity of polaritons in semiconductor microcavities
journal, September 2009

  • Amo, Alberto; Lefrère, Jérôme; Pigeon, Simon
  • Nature Physics, Vol. 5, Issue 11
  • DOI: 10.1038/nphys1364

Generating functional approach for spontaneous coherence in semiconductor electron-hole-photon systems
journal, March 2015


From polariton condensates to highly photonic quantum degenerate states of bosonic matter
journal, January 2011

  • Aßmann, Marc; Tempel, Jean-Sebastian; Veit, Franziska
  • Proceedings of the National Academy of Sciences, Vol. 108, Issue 5
  • DOI: 10.1073/pnas.1009847108

Two-Dimensional Superfluidity of Exciton Polaritons Requires Strong Anisotropy
journal, February 2015


Mean-field theory and fluctuation spectrum of a pumped decaying Bose-Fermi system across the quantum condensation transition
journal, May 2007


High-energy side-peak emission of exciton-polariton condensates in high density regime
journal, May 2016

  • Horikiri, Tomoyuki; Yamaguchi, Makoto; Kamide, Kenji
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep25655

Electrodynamic duality and vortex unbinding in driven-dissipative condensates
journal, September 2016


Lattice duality for the compact Kardar-Parisi-Zhang equation
journal, September 2016


BEC–BCS-laser crossover in Coulomb-correlated electron–hole–photon systems
journal, June 2012


Second Thresholds in BEC-BCS-Laser Crossover of Exciton-Polariton Systems
journal, July 2013


Excitonic modes in a Bose-condensed electron-hole gas in the pairing approximation
journal, March 1988


BCS-BEC Crossover in a Gas of Fermi Atoms with a Feshbach Resonance
journal, September 2002


Perturbation theory in statistical mechanics and the theory of superconductivity
journal, August 1960


Negative Bogoliubov dispersion in exciton-polariton condensates
journal, February 2012


Ghost Branch Photoluminescence From a Polariton Fluid Under Nonresonant Excitation
journal, October 2015


Superfluidity and collective modes in a uniform gas of Fermi atoms with a Feshbach resonance
journal, June 2003


Quantum fluids of light
journal, February 2013


Probing the excitation spectrum of polariton condensates
journal, March 2009


Bose–Einstein condensation of exciton polaritons
journal, September 2006

  • Kasprzak, J.; Richard, M.; Kundermann, S.
  • Nature, Vol. 443, Issue 7110
  • DOI: 10.1038/nature05131

Observation of Bogoliubov excitations in exciton-polariton condensates
journal, August 2008

  • Utsunomiya, S.; Tian, L.; Roumpos, G.
  • Nature Physics, Vol. 4, Issue 9
  • DOI: 10.1038/nphys1034

Role of the stress trap in the polariton quasiequilibrium condensation in GaAs microcavities
journal, February 2009


Classical-quantum crossovers in quasi-one-dimensional electron-hole systems: Exciton-Mott physics and interband optical spectra
journal, September 2012


Lasing and polariton condensation: Two distinct transitions in GaAs microcavities with stress traps
journal, June 2009

  • Nelsen, B.; Balili, R.; Snoke, D. W.
  • Journal of Applied Physics, Vol. 105, Issue 12
  • DOI: 10.1063/1.3140822

Effects of Configuration Interaction on Intensities and Phase Shifts
journal, December 1961


Non-equilibrium Properties of a Pumped-Decaying Bose-Condensed Electron–Hole Gas in the BCS–BEC Crossover Region
journal, March 2016

  • Hanai, R.; Littlewood, P. B.; Ohashi, Y.
  • Journal of Low Temperature Physics, Vol. 183, Issue 3-4
  • DOI: 10.1007/s10909-016-1552-6

Power-law decay of the spatial correlation function in exciton-polariton condensates
journal, April 2012

  • Roumpos, G.; Lohse, M.; Nitsche, W. H.
  • Proceedings of the National Academy of Sciences, Vol. 109, Issue 17
  • DOI: 10.1073/pnas.1107970109

BCS-BEC crossover in a system of microcavity polaritons
journal, September 2005


Observation of Resonance Condensation of Fermionic Atom Pairs
journal, January 2004


Absorption, photoluminescence, and resonant Rayleigh scattering probes of condensed microcavity polaritons
journal, September 2007


Self-consistent T-matrix theory of semiconductor light-absorption and luminescence
journal, April 2009


Dynamic Scaling of Growing Interfaces
journal, March 1986


Dynamical screening and self-energy of excitons in the electron–hole plasma
journal, November 1978

  • Zimmermann, R.; Kilimann, K.; Kraeft, W. D.
  • Physica Status Solidi (b), Vol. 90, Issue 1
  • DOI: 10.1002/pssb.2220900119

Photon lasing in GaAs microcavity: Similarities with a polariton condensate
journal, November 2007


Works referencing / citing this record:

Dynamically Induced Excitonic Instability in Pumped Dirac Materials
journal, December 2019


Dispersion relation of the collective excitations in a resonantly driven polariton fluid
journal, August 2019


Observation of quantum depletion in a non-equilibrium exciton–polariton condensate
journal, January 2020

  • Pieczarka, Maciej; Estrecho, Eliezer; Boozarjmehr, Maryam
  • Nature Communications, Vol. 11, Issue 1
  • DOI: 10.1038/s41467-019-14243-6

Nonequilibrium strong-coupling theory for a driven-dissipative ultracold Fermi gas in the BCS-BEC crossover region
journal, January 2020


Non-Hermitian phase transition from a polariton Bose-Einstein condensate to a photon laser
text, January 2018