Title: A terahertz pump mega-electron-volt ultrafast electron diffraction probe apparatus at the SLAC Accelerator Structure Test Area facility

Journal Article · · Journal of Instrumentation
 [1];  [2];  [2];  [2];  [2];  [2];  [3];  [4];  [2];  [2];  [2];  [2];  [2];  [4];  [5];  [2];  [2]
  1. SLAC National Accelerator Lab., Menlo Park, CA (United States); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Chemistry
  2. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Stanford Univ., CA (United States). Dept. of Materials Science and Engineering
  4. SLAC National Accelerator Lab., Menlo Park, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
  5. SLAC National Accelerator Lab., Menlo Park, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); SLAC National Accelerator Lab., Menlo Park, CA (United States). Photon Ultrafast Laser Science and Engineering Inst. (PULSE)

Here, we describe a new experimental setup capable of measuring structural dynamics following intense terahertz excitation. This system, developed at the SLAC Accelerator Structure Test Area facility, uses a high-energy ultrafast laser to produce intense terahertz pulses and femtosecond electron bunches that are accelerated to mega-electron-volt kinetic energies. The focused terahertz pulses have electric fields in excess of 600 kV/cm, and the resulting structural dynamics can be followed by electron diffraction. We also present some examples demonstrating its implementation where interactions between the THz pulses and the electron bunch are used to characterize the spatial and temporal characteristics of the THz field.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); USDOE Office of Science (SC), Fusion Energy Sciences (FES) (SC-24)
Grant/Contract Number:
AC02-76SF00515
OSTI ID:
1461477
Journal Information:
Journal of Instrumentation, Journal Name: Journal of Instrumentation Journal Issue: 06 Vol. 13; ISSN 1748-0221
Publisher:
Institute of Physics (IOP)Copyright Statement
Country of Publication:
United States
Language:
English

References (37)

Derivation of the pulse front tilt caused by angular dispersion journal December 1996
THz generation via optical rectification with ultrashort laser pulse focused to a line journal May 2005
Group velocity dispersion in prisms and its application to pulse compression and travelling-wave excitation journal June 1985
Femtosecond mega-electron-volt electron microdiffraction journal January 2018
The potential and limitations of neutrons, electrons and X-rays for atomic resolution microscopy of unstained biological molecules journal May 1995
Dynamic Structural Response and Deformations of Monolayer MoS 2 Visualized by Femtosecond Electron Diffraction journal September 2015
Terahertz-driven linear electron acceleration journal October 2015
Single-shot terahertz-field-driven X-ray streak camera journal August 2009
First lasing and operation of an ångstrom-wavelength free-electron laser journal August 2010
A compact X-ray free-electron laser emitting in the sub-ångström region journal June 2012
Resonant and nonresonant control over matter and light by intense terahertz transients journal August 2013
Ultrabright X-ray laser scattering for dynamic warm dense matter physics journal March 2015
Efficient generation of subpicosecond terahertz radiation by phase-matched optical rectification using ultrashort laser pulses with tilted pulse fronts journal October 2003
Ultrafast time-resolved electron diffraction with megavolt electron beams journal October 2006
Generation of 10μJ ultrashort terahertz pulses by optical rectification journal April 2007
Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3 journal February 2011
Mega-electron-volt ultrafast electron diffraction at SLAC National Accelerator Laboratory journal July 2015
Single-shot mega-electronvolt ultrafast electron diffraction for structure dynamic studies of warm dense matter journal August 2016
Optical antennas and plasmonics journal March 2009
A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses journal June 2014
Nonlinear high-temperature superconducting terahertz metamaterials journal October 2013
Femtosecond profiling of shaped x-ray pulses journal March 2018
Numerical simulation of THz-wave-assisted electron diffraction for ultrafast molecular imaging journal March 2017
Nonlinear Terahertz Metamaterials via Field-Enhanced Carrier Dynamics in GaAs journal May 2013
GV / m Single-Cycle Terahertz Fields from a Laser-Driven Large-Size Partitioned Organic Crystal journal May 2014
FLASH free-electron laser single-shot temporal diagnostic: terahertz-field-driven streaking journal January 2018
THz Nonlinear Spectroscopy of Solids journal September 2011
Local Enhancement of Terahertz Waves in Structured Metals journal May 2016
Femtosecond Crystallography with Ultrabright Electrons and X-rays: Capturing Chemistry in Action journal March 2014
All-optical control and metrology of electron pulses journal April 2016
Mapping Atomic Motions with Ultrabright Electrons: The Chemists' Gedanken Experiment Enters the Lab Frame journal April 2014
4d Ultrafast Electron Diffraction, Crystallography, and Microscopy journal May 2006
Velocity matching by pulse front tilting for large area THz-pulse generation journal January 2002
THz streak camera method for synchronous arrival time measurement of two-color hard X-ray FEL pulses journal January 2017
Generation of 30 μJ single-cycle terahertz pulses at 100 Hz repetition rate by optical rectification journal January 2008
Generation of 09-mJ THz pulses in DSTMS pumped by a Cr:Mg_2SiO_4 laser journal January 2014
Terahertz-driven, all-optical electron gun journal January 2016

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