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Title: Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode

Here, we report the development, testing, and demonstration of a setup for modulation excitation spectroscopy experiments at the Inner Shell Spectroscopy beamline of National Synchrotron Light Source - II. A computer algorithm and dedicated software were developed for asynchronous data processing and analysis. We demonstrate the reconstruction of X-ray absorption spectra for different time points within the modulation pulse using a model system. This setup and the software are intended for a broad range of functional materials which exhibit structural and/or electronic responses to the external stimulation, such as catalysts, energy and battery materials, and electromechanical devices.
Authors:
ORCiD logo [1] ;  [1] ; ORCiD logo [1] ; ORCiD logo [2] ;  [1] ; ORCiD logo [1] ;  [3] ;  [2] ; ORCiD logo [1]
  1. Stony Brook Univ., Stony Brook, NY (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Weizmann Institute of Science, Rehovot (Israel)
Publication Date:
Report Number(s):
BNL-207845-2018-JAAM
Journal ID: ISSN 0034-6748
Grant/Contract Number:
SC0012704; AC02-98CH10886
Type:
Accepted Manuscript
Journal Name:
Review of Scientific Instruments
Additional Journal Information:
Journal Volume: 89; Journal Issue: 4; Journal ID: ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)
Research Org:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE
OSTI Identifier:
1460821
Alternate Identifier(s):
OSTI ID: 1433575

Singh, H., Donetsky, D., Liu, J., Attenkofer, K., Cheng, B., Trelewicz, J. R., Lubomirsky, Igor, Stavitski, E., and Frenkel, A. I.. Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode. United States: N. p., Web. doi:10.1063/1.5000679.
Singh, H., Donetsky, D., Liu, J., Attenkofer, K., Cheng, B., Trelewicz, J. R., Lubomirsky, Igor, Stavitski, E., & Frenkel, A. I.. Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode. United States. doi:10.1063/1.5000679.
Singh, H., Donetsky, D., Liu, J., Attenkofer, K., Cheng, B., Trelewicz, J. R., Lubomirsky, Igor, Stavitski, E., and Frenkel, A. I.. 2018. "Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode". United States. doi:10.1063/1.5000679.
@article{osti_1460821,
title = {Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode},
author = {Singh, H. and Donetsky, D. and Liu, J. and Attenkofer, K. and Cheng, B. and Trelewicz, J. R. and Lubomirsky, Igor and Stavitski, E. and Frenkel, A. I.},
abstractNote = {Here, we report the development, testing, and demonstration of a setup for modulation excitation spectroscopy experiments at the Inner Shell Spectroscopy beamline of National Synchrotron Light Source - II. A computer algorithm and dedicated software were developed for asynchronous data processing and analysis. We demonstrate the reconstruction of X-ray absorption spectra for different time points within the modulation pulse using a model system. This setup and the software are intended for a broad range of functional materials which exhibit structural and/or electronic responses to the external stimulation, such as catalysts, energy and battery materials, and electromechanical devices.},
doi = {10.1063/1.5000679},
journal = {Review of Scientific Instruments},
number = 4,
volume = 89,
place = {United States},
year = {2018},
month = {4}
}