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Title: Quantitative Mapping of Nanoscale Chemical Dynamics in Sub-Sampled Operando (S)TEM Images using Spatio-Temporal Analytics

Authors:
ORCiD logo [1]; ORCiD logo [1];  [2]; ORCiD logo [3]; ORCiD logo [3];  [2]; ORCiD logo [1]
  1. National Security Directorate, Pacific Northwest National Laboratory, Richland WA 99352 USA
  2. Department of Statistics, Iowa State University, Ames IA 50011 USA
  3. School of Engineering, University of Liverpool, Liverpool United Kingdom
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1460595
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
ChemCatChem
Additional Journal Information:
Journal Name: ChemCatChem Journal Volume: 10 Journal Issue: 14; Journal ID: ISSN 1867-3880
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English

Citation Formats

Stanfill, Bryan A., Reehl, Sarah M., Johnson, Margaret C., Browning, Nigel D., Mehdi, B. Layla, Caragea, Petruta C., and Bramer, Lisa M. Quantitative Mapping of Nanoscale Chemical Dynamics in Sub-Sampled Operando (S)TEM Images using Spatio-Temporal Analytics. Germany: N. p., 2018. Web. doi:10.1002/cctc.201800333.
Stanfill, Bryan A., Reehl, Sarah M., Johnson, Margaret C., Browning, Nigel D., Mehdi, B. Layla, Caragea, Petruta C., & Bramer, Lisa M. Quantitative Mapping of Nanoscale Chemical Dynamics in Sub-Sampled Operando (S)TEM Images using Spatio-Temporal Analytics. Germany. doi:10.1002/cctc.201800333.
Stanfill, Bryan A., Reehl, Sarah M., Johnson, Margaret C., Browning, Nigel D., Mehdi, B. Layla, Caragea, Petruta C., and Bramer, Lisa M. Tue . "Quantitative Mapping of Nanoscale Chemical Dynamics in Sub-Sampled Operando (S)TEM Images using Spatio-Temporal Analytics". Germany. doi:10.1002/cctc.201800333.
@article{osti_1460595,
title = {Quantitative Mapping of Nanoscale Chemical Dynamics in Sub-Sampled Operando (S)TEM Images using Spatio-Temporal Analytics},
author = {Stanfill, Bryan A. and Reehl, Sarah M. and Johnson, Margaret C. and Browning, Nigel D. and Mehdi, B. Layla and Caragea, Petruta C. and Bramer, Lisa M.},
abstractNote = {},
doi = {10.1002/cctc.201800333},
journal = {ChemCatChem},
number = 14,
volume = 10,
place = {Germany},
year = {2018},
month = {5}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1002/cctc.201800333

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Works referenced in this record:

Statistical Estimation of Atomic Positions from Exit Wave Reconstruction with a Precision in the Picometer Range
journal, March 2006


Probing the Degradation Mechanisms in Electrolyte Solutions for Li-Ion Batteries by in Situ Transmission Electron Microscopy
journal, February 2014

  • Abellan, Patricia; Mehdi, B. Layla; Parent, Lucas R.
  • Nano Letters, Vol. 14, Issue 3
  • DOI: 10.1021/nl404271k

A sub-sampled approach to extremely low-dose STEM
journal, January 2018

  • Stevens, A.; Luzi, L.; Yang, H.
  • Applied Physics Letters, Vol. 112, Issue 4
  • DOI: 10.1063/1.5016192

The potential for Bayesian compressive sensing to significantly reduce electron dose in high-resolution STEM images
journal, October 2013


Procedure to count atoms with trustworthy single-atom sensitivity
journal, February 2013


Robust uncertainty principles: exact signal reconstruction from highly incomplete frequency information
journal, February 2006

  • Candes, E.J.; Romberg, J.; Tao, T.
  • IEEE Transactions on Information Theory, Vol. 52, Issue 2, p. 489-509
  • DOI: 10.1109/TIT.2005.862083

In Situ Observation of Solid Electrolyte Interphase Formation in Ordered Mesoporous Hard Carbon by Small-Angle Neutron Scattering
journal, March 2012

  • Bridges, Craig A.; Sun, Xiao-Guang; Zhao, Jinkui
  • The Journal of Physical Chemistry C, Vol. 116, Issue 14
  • DOI: 10.1021/jp3012393

Direct Observation of Ferrielectricity at Ferroelastic Domain Boundaries in CaTiO 3 by Electron Microscopy
journal, December 2011

  • Van Aert, Sandra; Turner, Stuart; Delville, Rémi
  • Advanced Materials, Vol. 24, Issue 4
  • DOI: 10.1002/adma.201103717

Controlled Growth of Nanoparticles from Solution with In Situ Liquid Transmission Electron Microscopy
journal, July 2011

  • Evans, James E.; Jungjohann, Katherine L.; Browning, Nigel D.
  • Nano Letters, Vol. 11, Issue 7
  • DOI: 10.1021/nl201166k

Atomic Structure of Quantum Gold Nanowires: Quantification of the Lattice Strain
journal, December 2013

  • Kundu, Paromita; Turner, Stuart; Van Aert, Sandra
  • ACS Nano, Vol. 8, Issue 1
  • DOI: 10.1021/nn4052315

Effective Gaussian mixture learning for video background subtraction
journal, May 2005

  • Dar-Shyang Lee,
  • IEEE Transactions on Pattern Analysis and Machine Intelligence, Vol. 27, Issue 5
  • DOI: 10.1109/TPAMI.2005.102

Visualization of oscillatory behaviour of Pt nanoparticles catalysing CO oxidation
journal, July 2014

  • Vendelbo, S. B.; Elkjær, C. F.; Falsig, H.
  • Nature Materials, Vol. 13, Issue 9
  • DOI: 10.1038/nmat4033

Implementing an accurate and rapid sparse sampling approach for low-dose atomic resolution STEM imaging
journal, October 2016

  • Kovarik, L.; Stevens, A.; Liyu, A.
  • Applied Physics Letters, Vol. 109, Issue 16
  • DOI: 10.1063/1.4965720

Maximum likelihood estimation of structure parameters from high resolution electron microscopy images. Part I: A theoretical framework
journal, September 2005


Direct Observation of Aggregative Nanoparticle Growth: Kinetic Modeling of the Size Distribution and Growth Rate
journal, December 2013

  • Woehl, Taylor J.; Park, Chiwoo; Evans, James E.
  • Nano Letters, Vol. 14, Issue 1
  • DOI: 10.1021/nl4043328

Compressed sensing
journal, April 2006


Maximum likelihood estimation of structure parameters from high resolution electron microscopy images. Part II: A practical example
journal, September 2005


A New Approach for Segmentation and Quantification of Cells or Nanoparticles
journal, June 2016


Direct in Situ Determination of the Mechanisms Controlling Nanoparticle Nucleation and Growth
journal, September 2012

  • Woehl, Taylor J.; Evans, James E.; Arslan, Ilke
  • ACS Nano, Vol. 6, Issue 10
  • DOI: 10.1021/nn303371y

ViBe: A Universal Background Subtraction Algorithm for Video Sequences
journal, June 2011

  • Barnich, O.; Van Droogenbroeck, M.
  • IEEE Transactions on Image Processing, Vol. 20, Issue 6
  • DOI: 10.1109/TIP.2010.2101613

Factors influencing quantitative liquid (scanning) transmission electron microscopy
journal, January 2014

  • Abellan, P.; Woehl, T. J.; Parent, L. R.
  • Chem. Commun., Vol. 50, Issue 38
  • DOI: 10.1039/C3CC48479C

Maximum likelihood estimation via the ECM algorithm: A general framework
journal, January 1993


StatSTEM: An efficient approach for accurate and precise model-based quantification of atomic resolution electron microscopy images
journal, December 2016


High-Resolution EM of Colloidal Nanocrystal Growth Using Graphene Liquid Cells
journal, April 2012


In situ liquid-cell electron microscopy of silver–palladium galvanic replacement reactions on silver nanoparticles
journal, September 2014

  • Sutter, E.; Jungjohann, K.; Bliznakov, S.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5946

Applying compressive sensing to TEM video: a substantial frame rate increase on any camera
journal, August 2015

  • Stevens, Andrew; Kovarik, Libor; Abellan, Patricia
  • Advanced Structural and Chemical Imaging, Vol. 1, Issue 10
  • DOI: 10.1186/s40679-015-0009-3

Atomic scale dynamics of ultrasmall germanium clusters
journal, January 2012

  • Bals, S.; Van Aert, S.; Romero, C. P.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms1887

Observation and Quantification of Nanoscale Processes in Lithium Batteries by Operando Electrochemical (S)TEM
journal, February 2015


Sub-ångstrom resolution using aberration corrected electron optics
journal, August 2002

  • Batson, P. E.; Dellby, N.; Krivanek, O. L.
  • Nature, Vol. 418, Issue 6898
  • DOI: 10.1038/nature00972

Visualization of Electrode–Electrolyte Interfaces in LiPF 6 /EC/DEC Electrolyte for Lithium Ion Batteries via in Situ TEM
journal, March 2014

  • Zeng, Zhiyuan; Liang, Wen-I; Liao, Hong-Gang
  • Nano Letters, Vol. 14, Issue 4
  • DOI: 10.1021/nl403922u

Understanding the Role of Solvation Forces on the Preferential Attachment of Nanoparticles in Liquid
journal, December 2015