Evaluation of nitrous oxide as a substitute for sulfur hexafluoride to reduce global warming impacts of ANSI/HPS N13.1 gaseous uniformity testing
Abstract
The ANSI/HPS N13.1–2011 standard requires gaseous tracer uniformity testing for sampling associated with stacks used in radioactive air emissions. Sulfur hexafluoride (SF6), a greenhouse gas with a high global warming potential, has long been the gas tracer used in such testing. To reduce the impact of gas tracer tests on the environment, nitrous oxide (N2O) was evaluated as a potential replacement to SF6. The physical evaluation included the development of a test plan to record percent coefficient of variance and the percent maximum deviation between the two gases while considering variables such as fan configuration, injection position, and flow rate. Statistical power was calculated to determine how many sample sets were needed, and computational fluid dynamic modeling was utilized to estimate overall mixing in stacks. Results show there are no significant differences between the behaviors of the two gases, and SF6 modeling corroborated N2O test results. Although, in principle, all tracer gases should behave in an identical manner for measuring mixing within a stack, the series of physical tests guided by statistics was performed to demonstrate the equivalence of N2O testing to SF6 testing in the context of stack qualification tests. In conclusion, the results demonstrate that N2O is amore »
- Authors:
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1459450
- Alternate Identifier(s):
- OSTI ID: 1416970
- Report Number(s):
- PNNL-SA-128014
Journal ID: ISSN 1352-2310; S1352231017308567; PII: S1352231017308567
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Published Article
- Journal Name:
- Atmospheric Environment (1994)
- Additional Journal Information:
- Journal Name: Atmospheric Environment (1994) Journal Volume: 176 Journal Issue: C; Journal ID: ISSN 1352-2310
- Publisher:
- Elsevier
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; ANSI/HPS N13.1–2011; Gaseous tracer testing; Global warming potential; N2O; SF6; Standards
Citation Formats
Yu, Xiao-Ying, Barnett, J. Matthew, Amidan, Brett G., Recknagle, Kurtis P., Flaherty, Julia E., Antonio, Ernest J., and Glissmeyer, John A. Evaluation of nitrous oxide as a substitute for sulfur hexafluoride to reduce global warming impacts of ANSI/HPS N13.1 gaseous uniformity testing. United Kingdom: N. p., 2018.
Web. doi:10.1016/j.atmosenv.2017.12.015.
Yu, Xiao-Ying, Barnett, J. Matthew, Amidan, Brett G., Recknagle, Kurtis P., Flaherty, Julia E., Antonio, Ernest J., & Glissmeyer, John A. Evaluation of nitrous oxide as a substitute for sulfur hexafluoride to reduce global warming impacts of ANSI/HPS N13.1 gaseous uniformity testing. United Kingdom. https://doi.org/10.1016/j.atmosenv.2017.12.015
Yu, Xiao-Ying, Barnett, J. Matthew, Amidan, Brett G., Recknagle, Kurtis P., Flaherty, Julia E., Antonio, Ernest J., and Glissmeyer, John A. Thu .
"Evaluation of nitrous oxide as a substitute for sulfur hexafluoride to reduce global warming impacts of ANSI/HPS N13.1 gaseous uniformity testing". United Kingdom. https://doi.org/10.1016/j.atmosenv.2017.12.015.
@article{osti_1459450,
title = {Evaluation of nitrous oxide as a substitute for sulfur hexafluoride to reduce global warming impacts of ANSI/HPS N13.1 gaseous uniformity testing},
author = {Yu, Xiao-Ying and Barnett, J. Matthew and Amidan, Brett G. and Recknagle, Kurtis P. and Flaherty, Julia E. and Antonio, Ernest J. and Glissmeyer, John A.},
abstractNote = {The ANSI/HPS N13.1–2011 standard requires gaseous tracer uniformity testing for sampling associated with stacks used in radioactive air emissions. Sulfur hexafluoride (SF6), a greenhouse gas with a high global warming potential, has long been the gas tracer used in such testing. To reduce the impact of gas tracer tests on the environment, nitrous oxide (N2O) was evaluated as a potential replacement to SF6. The physical evaluation included the development of a test plan to record percent coefficient of variance and the percent maximum deviation between the two gases while considering variables such as fan configuration, injection position, and flow rate. Statistical power was calculated to determine how many sample sets were needed, and computational fluid dynamic modeling was utilized to estimate overall mixing in stacks. Results show there are no significant differences between the behaviors of the two gases, and SF6 modeling corroborated N2O test results. Although, in principle, all tracer gases should behave in an identical manner for measuring mixing within a stack, the series of physical tests guided by statistics was performed to demonstrate the equivalence of N2O testing to SF6 testing in the context of stack qualification tests. In conclusion, the results demonstrate that N2O is a viable choice leading to a four times reduction in global warming impacts for future similar compliance driven testing.},
doi = {10.1016/j.atmosenv.2017.12.015},
journal = {Atmospheric Environment (1994)},
number = C,
volume = 176,
place = {United Kingdom},
year = {Thu Mar 01 00:00:00 EST 2018},
month = {Thu Mar 01 00:00:00 EST 2018}
}
https://doi.org/10.1016/j.atmosenv.2017.12.015
Figures / Tables:
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Figures / Tables found in this record: