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Title: Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2

Abstract

URu2Si2 exhibits an anomalous peak in the nonlinear magnetic susceptibility at the hidden order transition. In order to investigate this anomaly, we conducted direct magnetization measurements and investigated the detailed angular dependence of the 29Si nuclear magnetic resonance Knight shift tensor. We find that the nonlinear magnetization is smaller than previously reported, and the analogous nonlinear Knight shift tensor is below the detection limit. Our results suggest that the magnitude of the anomalous peak is sample dependent.

Authors:
 [1];  [1];  [1];  [1];  [2];  [3];  [4];  [4];  [4];  [5]
  1. Univ. of California, Davis, CA (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  2. Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
  3. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  4. Univ. of California, San Diego, CA (United States)
  5. Univ. of California, Davis, CA (United States)
Publication Date:
Research Org.:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Davis, CA (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1458656
Alternate Identifier(s):
OSTI ID: 1422251; OSTI ID: 1755369
Report Number(s):
LLNL-JRNL-738073
Journal ID: ISSN 2469-9950; 890970; TRN: US1901491
Grant/Contract Number:  
AC52-07NA27344; NA0002908; FG52-09NA29464; FG02-04ER46105
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 97; Journal Issue: 7-15; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Order parameters; Paramagnetism; Heavy-fermion systems; DC susceptibility measurements; Nuclear magnetic resonance

Citation Formats

Lawson, M., Bush, B. T., Kissikov, T., Brubaker, Z., Shirer, K. R., Jeffries, J. R., Ran, S., Jeon, I., Maple, M. B., and Curro, N. J.. Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2. United States: N. p., 2018. Web. https://doi.org/10.1103/PhysRevB.97.075138.
Lawson, M., Bush, B. T., Kissikov, T., Brubaker, Z., Shirer, K. R., Jeffries, J. R., Ran, S., Jeon, I., Maple, M. B., & Curro, N. J.. Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2. United States. https://doi.org/10.1103/PhysRevB.97.075138
Lawson, M., Bush, B. T., Kissikov, T., Brubaker, Z., Shirer, K. R., Jeffries, J. R., Ran, S., Jeon, I., Maple, M. B., and Curro, N. J.. Thu . "Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2". United States. https://doi.org/10.1103/PhysRevB.97.075138. https://www.osti.gov/servlets/purl/1458656.
@article{osti_1458656,
title = {Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2},
author = {Lawson, M. and Bush, B. T. and Kissikov, T. and Brubaker, Z. and Shirer, K. R. and Jeffries, J. R. and Ran, S. and Jeon, I. and Maple, M. B. and Curro, N. J.},
abstractNote = {URu2Si2 exhibits an anomalous peak in the nonlinear magnetic susceptibility at the hidden order transition. In order to investigate this anomaly, we conducted direct magnetization measurements and investigated the detailed angular dependence of the 29Si nuclear magnetic resonance Knight shift tensor. We find that the nonlinear magnetization is smaller than previously reported, and the analogous nonlinear Knight shift tensor is below the detection limit. Our results suggest that the magnitude of the anomalous peak is sample dependent.},
doi = {10.1103/PhysRevB.97.075138},
journal = {Physical Review B},
number = 7-15,
volume = 97,
place = {United States},
year = {2018},
month = {2}
}

Journal Article:

Citation Metrics:
Cited by: 1 work
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Figures / Tables:

FIG. 1 FIG. 1: 29Si NMR spectra of URu2Si2 as a function of angle at 16 K. Solid black lines are fits as described in the text. The inset shows the angular dependence of the mean frequency.

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Works referenced in this record:

Long range order and two-fluid behavior in heavy electron materials
journal, September 2012

  • Shirer, K. R.; Shockley, A. C.; Dioguardi, A. P.
  • Proceedings of the National Academy of Sciences, Vol. 109, Issue 45
  • DOI: 10.1073/pnas.1209609109

Superconducting Pairs with Extreme Uniaxial Anisotropy in URu 2 Si 2
journal, February 2012


Sequential Spin Polarization of the Fermi Surface Pockets in URu 2 Si 2 and Its Implications for the Hidden Order
journal, April 2011


NMR Study of In-Plane Twofold Ordering in URu 2 Si 2
journal, June 2013


Magnetic properties of U(Ru 1− x Rh x ) 2 Si 2 single crystals (0≤ x ≤1)
journal, November 1991

  • Miyako, Y.; Kawarazaki, S.; Amitsuka, H.
  • Journal of Applied Physics, Vol. 70, Issue 10
  • DOI: 10.1063/1.350162

A two-axis goniometer for low-temperature nuclear magnetic resonance measurements on single crystals
journal, September 2012

  • Shiroka, T.; Casola, F.; Mesot, J.
  • Review of Scientific Instruments, Vol. 83, Issue 9
  • DOI: 10.1063/1.4748861

Nuclear magnetic resonance in Kondo lattice systems
journal, May 2016


Momentum-Resolved Evolution of the Kondo Lattice into “Hidden Order” in URu 2 Si 2
journal, April 2013


Evidence of an odd-parity hidden order in a spin–orbit coupled correlated iridate
journal, October 2015

  • Zhao, L.; Torchinsky, D. H.; Chu, H.
  • Nature Physics, Vol. 12, Issue 1
  • DOI: 10.1038/nphys3517

Magnetic anisotropy in the paramagnetic phase of TbAl2
journal, January 1984

  • del Moral, A.; Arnaudas, J. I.; Cockaday, J. S.
  • Journal of Magnetism and Magnetic Materials, Vol. 40, Issue 3
  • DOI: 10.1016/0304-8853(84)90326-3

Disorder in quantum critical superconductors
journal, December 2013

  • Seo, S.; Lu, Xin; Zhu, J-X.
  • Nature Physics, Vol. 10, Issue 2
  • DOI: 10.1038/nphys2820

Distributed twofold ordering in URu 2 Si 2
journal, January 2015


Formation of the Coherent Heavy Fermion Liquid at the Hidden Order Transition in URu 2 Si 2
journal, May 2013


Spatially Inhomogeneous Development of Antiferromagnetism in URu 2 Si 2 : Evidence from S 29 i NMR under Pressure
journal, August 2001


Nonlinear susceptibility measurements in heavy fermion systems
journal, April 1994


Nonlinear susceptibility as a probe of tensor spin order in URu 2 Si 2
journal, April 1992


Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2
journal, November 2011


29 Si NMR Study of Antiferromagnetic Superconductor URu 2 Si 2
journal, April 1996

  • Kohori, Yoh; Matsuda, Kazuyuki; Kohara, Takao
  • Journal of the Physical Society of Japan, Vol. 65, Issue 4
  • DOI: 10.1143/JPSJ.65.1083

A global inversion-symmetry-broken phase inside the pseudogap region of YBa2Cu3Oy
journal, November 2016

  • Zhao, L.; Belvin, C. A.; Liang, R.
  • Nature Physics, Vol. 13, Issue 3
  • DOI: 10.1038/nphys3962

Thermodynamic Measurement of Angular Anisotropy at the Hidden Order Transition of URu 2 Si 2
journal, October 2016


Chirality density wave of the "hidden order" phase in URu2Si2
journal, February 2015


Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
journal, January 2011


Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2
journal, June 2014

  • Tonegawa, S.; Kasahara, S.; Fukuda, T.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5188

Hidden Order in URu 2 Si 2 Unveiled
journal, August 2012


    Works referencing / citing this record:

    Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu 2 Si 2
    journal, January 2020

    • Mydosh, J. A.; Oppeneer, P. M.; Riseborough, P. S.
    • Journal of Physics: Condensed Matter, Vol. 32, Issue 14
    • DOI: 10.1088/1361-648x/ab5eba

    Odd-parity electronic multipolar ordering in URu 2 Si 2 : Conclusions from Si and Ru NMR measurements
    journal, June 2018


      Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.