Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2

Lawson, M.; Bush, B. T.; Kissikov, T.; Brubaker, Z.; Shirer, K. R.; Jeffries, J. R.; Ran, S.; Jeon, I.; Maple, M. B.; Curro, N. J.

doi:10.1103/PhysRevB.97.075138

Title: Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu₂Si₂

Abstract

URu2Si2 exhibits an anomalous peak in the nonlinear magnetic susceptibility at the hidden order transition. In order to investigate this anomaly, we conducted direct magnetization measurements and investigated the detailed angular dependence of the 29Si nuclear magnetic resonance Knight shift tensor. We find that the nonlinear magnetization is smaller than previously reported, and the analogous nonlinear Knight shift tensor is below the detection limit. Our results suggest that the magnitude of the anomalous peak is sample dependent.

Authors:

Lawson, M. ^[1]; Bush, B. T. ^[1]; Kissikov, T. ^[1]; Brubaker, Z. ^[1]; Shirer, K. R. ^[2]; Jeffries, J. R. ^[3]; Ran, S. ^[4]; Jeon, I. ^[4]; Maple, M. B. ^[4]; Curro, N. J. ^[5]

Univ. of California, Davis, CA (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. of California, San Diego, CA (United States)
Univ. of California, Davis, CA (United States)

Publication Date:: 2018-02-22

Research Org.:: Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Davis, CA (United States)

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA)

OSTI Identifier:: 1458656

Alternate Identifier(s):: OSTI ID: 1422251; OSTI ID: 1755369

Report Number(s):: LLNL-JRNL-738073
Journal ID: ISSN 2469-9950; 890970; TRN: US1901491

Grant/Contract Number:: AC52-07NA27344; NA0002908; FG52-09NA29464; FG02-04ER46105

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 97; Journal Issue: 7-15; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Order parameters; Paramagnetism; Heavy-fermion systems; DC susceptibility measurements; Nuclear magnetic resonance

Citation Formats


                    Lawson, M., Bush, B. T., Kissikov, T., Brubaker, Z., Shirer, K. R., Jeffries, J. R., Ran, S., Jeon, I., Maple, M. B., and Curro, N. J.. Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2.  United States: N. p., 2018. 
Web.  https://doi.org/10.1103/PhysRevB.97.075138.

Copy to clipboard


                    Lawson, M., Bush, B. T., Kissikov, T., Brubaker, Z., Shirer, K. R., Jeffries, J. R., Ran, S., Jeon, I., Maple, M. B., & Curro, N. J.. Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2.  United States.  https://doi.org/10.1103/PhysRevB.97.075138

Copy to clipboard


                    Lawson, M., Bush, B. T., Kissikov, T., Brubaker, Z., Shirer, K. R., Jeffries, J. R., Ran, S., Jeon, I., Maple, M. B., and Curro, N. J.. Thu .  
"Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2".  United States.  https://doi.org/10.1103/PhysRevB.97.075138.  https://www.osti.gov/servlets/purl/1458656.

Copy to clipboard


                    
@article{osti_1458656,

  title        = {Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2},

  author       = {Lawson, M. and Bush, B. T. and Kissikov, T. and Brubaker, Z. and Shirer, K. R. and Jeffries, J. R. and Ran, S. and Jeon, I. and Maple, M. B. and Curro, N. J.},

  abstractNote = {URu2Si2 exhibits an anomalous peak in the nonlinear magnetic susceptibility at the hidden order transition. In order to investigate this anomaly, we conducted direct magnetization measurements and investigated the detailed angular dependence of the 29Si nuclear magnetic resonance Knight shift tensor. We find that the nonlinear magnetization is smaller than previously reported, and the analogous nonlinear Knight shift tensor is below the detection limit. Our results suggest that the magnitude of the anomalous peak is sample dependent.},

  doi          = {10.1103/PhysRevB.97.075138},

  journal      = {Physical Review B},

  number       = 7-15,

  volume       = 97,

  place        = {United States},

  year         = {2018},

  month        = {2}

}

Copy to clipboard

Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (Publisher)

Accepted Manuscript (DOE)

Publisher's Version of Record

https://doi.org/10.1103/PhysRevB.97.075138

Other availability

Search WorldCat to find libraries that may hold this journal

Citation Metrics:

Cited by: 1 work

Citation information provided by
Web of Science

Figures / Tables:

FIG. 1: ²⁹Si NMR spectra of URu₂Si₂ as a function of angle at 16 K. Solid black lines are fits as described in the text. The inset shows the angular dependence of the mean frequency.

All figures and tables (6 total)

Save / Share:

Export Metadata

Save to My Library

Works referenced in this record:

Long range order and two-fluid behavior in heavy electron materials
journal, September 2012

Shirer, K. R.; Shockley, A. C.; Dioguardi, A. P.
Proceedings of the National Academy of Sciences, Vol. 109, Issue 45
DOI: 10.1073/pnas.1209609109

Superconducting Pairs with Extreme Uniaxial Anisotropy in ${URu}_{2} {Si}_{2}$
journal, February 2012

Altarawneh, M. M.; Harrison, N.; Li, G.
Physical Review Letters, Vol. 108, Issue 6
DOI: 10.1103/PhysRevLett.108.066407

Sequential Spin Polarization of the Fermi Surface Pockets in ${URu}_{2} {Si}_{2}$ and Its Implications for the Hidden Order
journal, April 2011

Altarawneh, M. M.; Harrison, N.; Sebastian, S. E.
Physical Review Letters, Vol. 106, Issue 14
DOI: 10.1103/PhysRevLett.106.146403

NMR Study of In-Plane Twofold Ordering in ${URu}_{2} {Si}_{2}$
journal, June 2013

Kambe, S.; Tokunaga, Y.; Sakai, H.
Physical Review Letters, Vol. 110, Issue 24
DOI: 10.1103/PhysRevLett.110.246406

Magnetic properties of U(Ru _{1− x} Rh _x ) ₂ Si ₂ single crystals (0≤ x ≤1)
journal, November 1991

Miyako, Y.; Kawarazaki, S.; Amitsuka, H.
Journal of Applied Physics, Vol. 70, Issue 10
DOI: 10.1063/1.350162

A two-axis goniometer for low-temperature nuclear magnetic resonance measurements on single crystals
journal, September 2012

Shiroka, T.; Casola, F.; Mesot, J.
Review of Scientific Instruments, Vol. 83, Issue 9
DOI: 10.1063/1.4748861

Nuclear magnetic resonance in Kondo lattice systems
journal, May 2016

Curro, Nicholas J.
Reports on Progress in Physics, Vol. 79, Issue 6
DOI: 10.1088/0034-4885/79/6/064501

Momentum-Resolved Evolution of the Kondo Lattice into “Hidden Order” in ${URu}_{2} {Si}_{2}$
journal, April 2013

Boariu, F. L.; Bareille, C.; Schwab, H.
Physical Review Letters, Vol. 110, Issue 15
DOI: 10.1103/PhysRevLett.110.156404

Evidence of an odd-parity hidden order in a spin–orbit coupled correlated iridate
journal, October 2015

Zhao, L.; Torchinsky, D. H.; Chu, H.
Nature Physics, Vol. 12, Issue 1
DOI: 10.1038/nphys3517

Magnetic anisotropy in the paramagnetic phase of TbAl2
journal, January 1984

del Moral, A.; Arnaudas, J. I.; Cockaday, J. S.
Journal of Magnetism and Magnetic Materials, Vol. 40, Issue 3
DOI: 10.1016/0304-8853(84)90326-3

Disorder in quantum critical superconductors
journal, December 2013

Seo, S.; Lu, Xin; Zhu, J-X.
Nature Physics, Vol. 10, Issue 2
DOI: 10.1038/nphys2820

Distributed twofold ordering in ${URu}_{2} {Si}_{2}$
journal, January 2015

Kambe, S.; Tokunaga, Y.; Sakai, H.
Physical Review B, Vol. 91, Issue 3
DOI: 10.1103/PhysRevB.91.035111

Formation of the Coherent Heavy Fermion Liquid at the Hidden Order Transition in ${URu}_{2} {Si}_{2}$
journal, May 2013

Chatterjee, Shouvik; Trinckauf, Jan; Hänke, Torben
Physical Review Letters, Vol. 110, Issue 18
DOI: 10.1103/PhysRevLett.110.186401

Spatially Inhomogeneous Development of Antiferromagnetism in ${URu}_{2} {Si}_{2}$ : Evidence from ${}^{29}S i$ NMR under Pressure
journal, August 2001

Matsuda, K.; Kohori, Y.; Kohara, T.
Physical Review Letters, Vol. 87, Issue 8
DOI: 10.1103/PhysRevLett.87.087203

Nonlinear susceptibility measurements in heavy fermion systems
journal, April 1994

Chandra, P.; Ramirez, A. P.; Coleman, P.
Physica B: Condensed Matter, Vol. 199-200
DOI: 10.1016/0921-4526(94)91858-9

Nonlinear susceptibility as a probe of tensor spin order in ${URu}_{2}$ ${Si}_{2}$
journal, April 1992

Ramirez, A. P.; Coleman, P.; Chandra, P.
Physical Review Letters, Vol. 68, Issue 17
DOI: 10.1103/PhysRevLett.68.2680

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

Mydosh, J. A.; Oppeneer, P. M.
Reviews of Modern Physics, Vol. 83, Issue 4
DOI: 10.1103/RevModPhys.83.1301

²⁹ Si NMR Study of Antiferromagnetic Superconductor URu ₂ Si ₂
journal, April 1996

Kohori, Yoh; Matsuda, Kazuyuki; Kohara, Takao
Journal of the Physical Society of Japan, Vol. 65, Issue 4
DOI: 10.1143/JPSJ.65.1083

A global inversion-symmetry-broken phase inside the pseudogap region of YBa2Cu3Oy
journal, November 2016

Zhao, L.; Belvin, C. A.; Liang, R.
Nature Physics, Vol. 13, Issue 3
DOI: 10.1038/nphys3962

Thermodynamic Measurement of Angular Anisotropy at the Hidden Order Transition of ${URu}_{2} {Si}_{2}$
journal, October 2016

Trinh, Jennifer; Brück, Ekkes; Siegrist, Theo
Physical Review Letters, Vol. 117, Issue 15
DOI: 10.1103/PhysRevLett.117.157201

Chirality density wave of the "hidden order" phase in URu2Si2
journal, February 2015

Kung, H. - H.; Baumbach, R. E.; Bauer, E. D.
Science, Vol. 347, Issue 6228
DOI: 10.1126/science.1259729

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
journal, January 2011

Okazaki, R.; Shibauchi, T.; Shi, H. J.
Science, Vol. 331, Issue 6016
DOI: 10.1126/science.1197358

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2
journal, June 2014

Tonegawa, S.; Kasahara, S.; Fukuda, T.
Nature Communications, Vol. 5, Issue 1
DOI: 10.1038/ncomms5188

Hidden Order in ${URu}_{2} {Si}_{2}$ Unveiled
journal, August 2012

Ressouche, E.; Ballou, R.; Bourdarot, F.
Physical Review Letters, Vol. 109, Issue 6
DOI: 10.1103/PhysRevLett.109.067202

Works referencing / citing this record:

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
journal, January 2020

Mydosh, J. A.; Oppeneer, P. M.; Riseborough, P. S.
Journal of Physics: Condensed Matter, Vol. 32, Issue 14
DOI: 10.1088/1361-648x/ab5eba

Odd-parity electronic multipolar ordering in ${URu}_{2} {Si}_{2}$ : Conclusions from Si and Ru NMR measurements
journal, June 2018

Kambe, S.; Tokunaga, Y.; Sakai, H.
Physical Review B, Vol. 97, Issue 23
DOI: 10.1103/physrevb.97.235142

Figures / Tables found in this record:

Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.

Similar Records in DOE PAGES and OSTI.GOV collections:

²⁹Si nuclear magnetic resonance study of URu₂Si₂ under pressure

Journal Article Shirer, K. R. ; Dioguardi, A. P. ; Bush, B. T. ; ... - Physica. B, Condensed Matter

Here, we report ²⁹Si nuclear magnetic resonance measurements of single crystals and aligned powders of URu₂Si₂ under pressure in the hidden order and paramagnetic phases. We find evidence for a reduction of the Knight shift with applied pressure, consistent with previous measurements of the static magnetic susceptibility. Previous measurements of the spin lattice relaxation time revealed a partial suppression of the density of states below 30 K. Here, we find that the temperature at which this suppression occurs is enhanced with applied pressure.
Cited by 3
https://doi.org/10.1016/j.physb.2015.11.018

Full Text Available
Emergence of higher order rotational symmetry in the hidden order phase of URu₂Si₂

Journal Article Kanchanavatee, N. ; Janoschek, M. ; Huang, K. ; ... - Philosophical Magazine (2003, Print)

Electrical resistivity measurements were performed in this paper as functions of temperature, magnetic field, and angle θ between the magnetic field and the c-axis of a URu₂Si₂ single crystal. The resistivity exhibits a two-fold oscillation as a function of θ at high temperatures, which undergoes a 180°-phase shift (sign change) with decreasing temperature at around 35 K. The hidden order transition is manifested as a minimum in the magnetoresistance and amplitude of the two-fold oscillation. Interestingly, the resistivity also showed four-fold, six-fold, and eight-fold symmetries at the hidden order transition. These higher order symmetries were also detected at low temperatures,more »« less
https://doi.org/10.1080/14786435.2016.1235294

Full Text Available
sup 63 Cu Knight shifts in the superconducting state of YBa sub 2 Cu sub 3 O sub 7 minus. delta. ( T sub c =90 K)

Journal Article Barrett, S E ; Durand, D J ; Pennington, C H ; ... - Physical Review, B: Condensed Matter; (USA)

The authors have used {sup 89}Y NMR to measure the internal magnetic field of a sample of YBa{sub 2}Cu{sub 3}O{sub 7{minus}{delta}} ({ital T}{sub {ital c}}=90 K) in the superconducting state to correct for the effects of the Meissner shielding currents. They used this information to separate the magnetic-shift tensor into orbital (chemical-shift) and spin (Knight-shift) contributions. They find that the temperature dependence of the chain Cu Knight shift fits the classic Yosida function of weak-coupling, orbital-{ital s}-state, spin-singlet BCS theory. For the planes, the Knight shift also requires a spin singlet, but with a strong-coupling Yosida function. The best fitmore »« less
https://doi.org/10.1103/PhysRevB.41.6283
Inelastic x-ray scattering measurements of phonon dynamics in ${URu}_{2} {Si}_{2}$

Journal Article Gardner, D. R. ; Bonnoit, C. J. ; Chisnell, R. ; ... - Physical Review B

We report high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu2Si2. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. Our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the low temperature phase.
https://doi.org/10.1103/PhysRevB.93.075123
NMR Knight shifts and the electronic properties of Rb{sub 8}Na{sub 16}Si{sub 136} clathrate

Journal Article Latturner, Susan ; Iversen, Bo B ; Sepa, Jelena ; ... - Physical Review B

A silicon framework clathrate type-II compound was synthesized with rubidium and sodium atoms in cages. A single crystal of this material was characterized by both conventional and synchrotron x-ray diffraction; the structure belongs to the cubic space group Fd-3m, with a cell edge of 14.738(1) Aa. The alkali metals are ordered in the structure, with the small cages containing sodium, and the large cages containing rubidium. Variable temperature magic-angle-spinning NMR of all three nuclei show large Knight shifts with a strong temperature dependence, unlike conventional metals. The low conductivity (200 S/cm) and high paramagnetic susceptibility (5x10{sup -6}emu/g) indicate that asmore »« less
https://doi.org/10.1103/PhysRevB.63.125403

Similar Records

Title: Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu2Si2

Abstract

Citation Formats

Figures / Tables:

Long range order and two-fluid behavior in heavy electron materials journal, September 2012

Superconducting Pairs with Extreme Uniaxial Anisotropy in URu 2 Si 2 journal, February 2012

Sequential Spin Polarization of the Fermi Surface Pockets in URu 2 Si 2 and Its Implications for the Hidden Order journal, April 2011

NMR Study of In-Plane Twofold Ordering in URu 2 Si 2 journal, June 2013

Magnetic properties of U(Ru 1− x Rh x ) 2 Si 2 single crystals (0≤ x ≤1) journal, November 1991

A two-axis goniometer for low-temperature nuclear magnetic resonance measurements on single crystals journal, September 2012

Nuclear magnetic resonance in Kondo lattice systems journal, May 2016

Momentum-Resolved Evolution of the Kondo Lattice into “Hidden Order” in URu 2 Si 2 journal, April 2013

Evidence of an odd-parity hidden order in a spin–orbit coupled correlated iridate journal, October 2015

Magnetic anisotropy in the paramagnetic phase of TbAl2 journal, January 1984

Disorder in quantum critical superconductors journal, December 2013

Distributed twofold ordering in URu 2 Si 2 journal, January 2015

Formation of the Coherent Heavy Fermion Liquid at the Hidden Order Transition in URu 2 Si 2 journal, May 2013

Spatially Inhomogeneous Development of Antiferromagnetism in URu 2 Si 2 : Evidence from S 29 i NMR under Pressure journal, August 2001

Nonlinear susceptibility measurements in heavy fermion systems journal, April 1994

Nonlinear susceptibility as a probe of tensor spin order in URu 2 Si 2 journal, April 1992

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

29 Si NMR Study of Antiferromagnetic Superconductor URu 2 Si 2 journal, April 1996

A global inversion-symmetry-broken phase inside the pseudogap region of YBa2Cu3Oy journal, November 2016

Thermodynamic Measurement of Angular Anisotropy at the Hidden Order Transition of URu 2 Si 2 journal, October 2016

Chirality density wave of the "hidden order" phase in URu2Si2 journal, February 2015

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 journal, January 2011

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 journal, June 2014

Hidden Order in URu 2 Si 2 Unveiled journal, August 2012

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu 2 Si 2 journal, January 2020

Odd-parity electronic multipolar ordering in URu 2 Si 2 : Conclusions from Si and Ru NMR measurements journal, June 2018

Title: Measurements of the NMR Knight shift tensor and nonlinear magnetization in URu₂Si₂

Long range order and two-fluid behavior in heavy electron materials
journal, September 2012

Superconducting Pairs with Extreme Uniaxial Anisotropy in ${URu}_{2} {Si}_{2}$
journal, February 2012

Sequential Spin Polarization of the Fermi Surface Pockets in ${URu}_{2} {Si}_{2}$ and Its Implications for the Hidden Order
journal, April 2011

NMR Study of In-Plane Twofold Ordering in ${URu}_{2} {Si}_{2}$
journal, June 2013

Magnetic properties of U(Ru _{1− x} Rh _x ) ₂ Si ₂ single crystals (0≤ x ≤1)
journal, November 1991

A two-axis goniometer for low-temperature nuclear magnetic resonance measurements on single crystals
journal, September 2012

Nuclear magnetic resonance in Kondo lattice systems
journal, May 2016

Momentum-Resolved Evolution of the Kondo Lattice into “Hidden Order” in ${URu}_{2} {Si}_{2}$
journal, April 2013

Evidence of an odd-parity hidden order in a spin–orbit coupled correlated iridate
journal, October 2015

Magnetic anisotropy in the paramagnetic phase of TbAl2
journal, January 1984

Disorder in quantum critical superconductors
journal, December 2013

Distributed twofold ordering in ${URu}_{2} {Si}_{2}$
journal, January 2015

Formation of the Coherent Heavy Fermion Liquid at the Hidden Order Transition in ${URu}_{2} {Si}_{2}$
journal, May 2013

Spatially Inhomogeneous Development of Antiferromagnetism in ${URu}_{2} {Si}_{2}$ : Evidence from ${}^{29}S i$ NMR under Pressure
journal, August 2001

Nonlinear susceptibility measurements in heavy fermion systems
journal, April 1994

Nonlinear susceptibility as a probe of tensor spin order in ${URu}_{2}$ ${Si}_{2}$
journal, April 1992

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

²⁹ Si NMR Study of Antiferromagnetic Superconductor URu ₂ Si ₂
journal, April 1996

A global inversion-symmetry-broken phase inside the pseudogap region of YBa2Cu3Oy
journal, November 2016

Thermodynamic Measurement of Angular Anisotropy at the Hidden Order Transition of ${URu}_{2} {Si}_{2}$
journal, October 2016

Chirality density wave of the "hidden order" phase in URu2Si2
journal, February 2015

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
journal, January 2011

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2
journal, June 2014

Hidden Order in ${URu}_{2} {Si}_{2}$ Unveiled
journal, August 2012

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
journal, January 2020

Odd-parity electronic multipolar ordering in ${URu}_{2} {Si}_{2}$ : Conclusions from Si and Ru NMR measurements
journal, June 2018