Observations of non-linear plasmon damping in dense plasmas
Abstract
Here, we present simulations using finite-temperature density-functional-theory molecular-dynamics to calculate dynamic dielectric properties in warm dense aluminum. The comparison between exchange-correlation functionals in the Perdew, Burke, Ernzerhof approximation, Strongly Constrained and Appropriately Normed Semilocal Density Functional, and Heyd, Scuseria, Ernzerhof (HSE) approximation indicates evident differences in the electron transition energies, dc conductivity, and Lorenz number. The HSE calculations show excellent agreement with x-ray scattering data as well as dc conductivity and absorption measurements. These findings demonstrate non-Drude behavior of the dynamic conductivity above the Cooper minimum that needs to be taken into account to determine optical properties in the warm dense matter regime.
- Authors:
-
[3]
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. Rostock, Rostock (Germany)
- SLAC National Accelerator Lab., Menlo Park, CA (United States); European XFEL, Schenefeld (Germany); Aible GmbH, Rostock (Germany)
- Univ. Rostock, Rostock (Germany)
- CEA, DAM, DIF, Arpajon Cedex (France)
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1458535
- Alternate Identifier(s):
- OSTI ID: 1426526
- Grant/Contract Number:
- AC02-76SF00515; FOR 2440; SFB 652; FWP 100182
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physics of Plasmas
- Additional Journal Information:
- Journal Volume: 25; Journal Issue: 5; Journal ID: ISSN 1070-664X
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY
Citation Formats
Witte, B. B. L., Sperling, P., French, M., Recoules, V., Glenzer, S. H., and Redmer, R. Observations of non-linear plasmon damping in dense plasmas. United States: N. p., 2018.
Web. doi:10.1063/1.5017889.
Witte, B. B. L., Sperling, P., French, M., Recoules, V., Glenzer, S. H., & Redmer, R. Observations of non-linear plasmon damping in dense plasmas. United States. https://doi.org/10.1063/1.5017889
Witte, B. B. L., Sperling, P., French, M., Recoules, V., Glenzer, S. H., and Redmer, R. Fri .
"Observations of non-linear plasmon damping in dense plasmas". United States. https://doi.org/10.1063/1.5017889. https://www.osti.gov/servlets/purl/1458535.
@article{osti_1458535,
title = {Observations of non-linear plasmon damping in dense plasmas},
author = {Witte, B. B. L. and Sperling, P. and French, M. and Recoules, V. and Glenzer, S. H. and Redmer, R.},
abstractNote = {Here, we present simulations using finite-temperature density-functional-theory molecular-dynamics to calculate dynamic dielectric properties in warm dense aluminum. The comparison between exchange-correlation functionals in the Perdew, Burke, Ernzerhof approximation, Strongly Constrained and Appropriately Normed Semilocal Density Functional, and Heyd, Scuseria, Ernzerhof (HSE) approximation indicates evident differences in the electron transition energies, dc conductivity, and Lorenz number. The HSE calculations show excellent agreement with x-ray scattering data as well as dc conductivity and absorption measurements. These findings demonstrate non-Drude behavior of the dynamic conductivity above the Cooper minimum that needs to be taken into account to determine optical properties in the warm dense matter regime.},
doi = {10.1063/1.5017889},
journal = {Physics of Plasmas},
number = 5,
volume = 25,
place = {United States},
year = {Fri Mar 16 00:00:00 EDT 2018},
month = {Fri Mar 16 00:00:00 EDT 2018}
}
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Figures / Tables:
FIG. 1. : Calculated dynamic electrical conductivity showing the influence of the XC functional in DFT-MD simulations. Calculations are performed for solid density aluminum at a temperature of $T$ = 0.5 eV. For small energies, the conductivity agrees with the Drude model62 (dotted lines). For hω > 21 eV, themore »
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Works referencing / citing this record:
Ionization dynamics of dense matter generated by intense ultrashort X-ray pulses
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- Shihab, Mohammed; Bornath, Thomas; Redmer, Ronald
- Contributions to Plasma Physics, Vol. 59, Issue 4-5
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