Observations of non-linear plasmon damping in dense plasmas

Witte, B. B. L.; Sperling, P.; French, M.; Recoules, V.; Glenzer, S. H.; Redmer, R.

doi:10.1063/1.5017889

Title: Observations of non-linear plasmon damping in dense plasmas

Journal Article · 16 March 2018 · Physics of Plasmas

DOI: https://doi.org/10.1063/1.5017889 · OSTI ID:1458535

Witte, B. B. L. ^[1]; Sperling, P. ^[2]; French, M. ^[3]; Recoules, V. ^[4]; Glenzer, S. H. ^[5];

^[3]

SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. Rostock, Rostock (Germany)
SLAC National Accelerator Lab., Menlo Park, CA (United States); European XFEL, Schenefeld (Germany); Aible GmbH, Rostock (Germany)
Univ. Rostock, Rostock (Germany)
CEA, DAM, DIF, Arpajon Cedex (France)
SLAC National Accelerator Lab., Menlo Park, CA (United States)

Here, we present simulations using finite-temperature density-functional-theory molecular-dynamics to calculate dynamic dielectric properties in warm dense aluminum. The comparison between exchange-correlation functionals in the Perdew, Burke, Ernzerhof approximation, Strongly Constrained and Appropriately Normed Semilocal Density Functional, and Heyd, Scuseria, Ernzerhof (HSE) approximation indicates evident differences in the electron transition energies, dc conductivity, and Lorenz number. The HSE calculations show excellent agreement with x-ray scattering data as well as dc conductivity and absorption measurements. These findings demonstrate non-Drude behavior of the dynamic conductivity above the Cooper minimum that needs to be taken into account to determine optical properties in the warm dense matter regime.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-76SF00515; FOR 2440; SFB 652; FWP 100182

OSTI ID:: 1458535

Alternate ID(s):: OSTI ID: 1426526

Journal Information:: Physics of Plasmas, Vol. 25, Issue 5; ISSN 1070-664X

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 28 works

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