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Title: Remote Sensing of Droplet Number Concentration in Warm Clouds: A Review of the Current State of Knowledge and Perspectives

Journal Article · · Reviews of Geophysics (1985)
ORCiD logo [1];  [2]; ORCiD logo [3]; ORCiD logo [4];  [5];  [6]; ORCiD logo [7];  [4]; ORCiD logo [8];  [9];  [10]; ORCiD logo [11]; ORCiD logo [12]; ORCiD logo [4];  [10];  [13]; ORCiD logo [14]; ORCiD logo [15];  [1];  [10] more »; ORCiD logo [16];  [17]; ORCiD logo [18];  [19]; ORCiD logo [10];  [5]; ORCiD logo [20]; ORCiD logo [5]; ORCiD logo [2]; ORCiD logo [21]; ORCiD logo [11]; ORCiD logo [22]; ORCiD logo [2] « less
  1. Univ. of Leeds (United Kingdom)
  2. Universität Leipzig (Germany)
  3. Rosenstiel School of Marine and Atmospheric Science, Miami, FL (United States)
  4. NASA Goddard Inst. for Space Studies (GISS), New York, NY (United States)
  5. NASA Goddard Inst. for Space Studies (GISS), New York, NY (United States); Columbia Univ., New York, NY (United States)
  6. Vanderbilt Univ., Nashville, TN (United States); Univ. of Wisconsin-Madison, Madison, WI (United States)
  7. Royal Netherlands Meteorological Inst., De Bilt (Netherlands)
  8. Colorado State Univ., Fort Collins, CO (United States)
  9. Univ.of Oxford (United Kingdom)
  10. Leibniz Inst. for Tropospheric Research (Germany)
  11. Univ. of Washington, Seattle, WA (United States)
  12. National Center for Atmospheric Research, Boulder, CO (United States)
  13. Deutscher Wetterdienst, Lindenberg (Germany)
  14. Stony Brook Univ., NY (United States)
  15. NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States)
  16. NASA Langley Research Center, Hampton, VA (United States)
  17. Vanderbilt Univ., Nashville, TN (United States)
  18. Hebrew Univ. of Jerusalem (Israel)
  19. Delft Univ. of Technology (Netherlands)
  20. Univ. of Oxford (United Kingdom)
  21. Joint Center for Earth Systems Technology, Baltimore MD (United States)
  22. Univ. of Maryland Baltimore County (UMBC), Baltimore, MD (United States)

The cloud droplet number concentration (Nd) is of central interest to improve the understanding of cloud physics and for quantifying the effective radiative forcing by aerosol-cloud interactions. Current standard satellite retrievals do not operationally provide Nd, but it can be inferred from retrievals of cloud optical depth (τc) cloud droplet effective radius (re) and cloud top temperature. This review compiles issues with this approach and quantifies uncertainties. A total relative uncertainty of 78% is inferred for pixel-level retrievals for relatively homogeneous, optically thick and unobscured stratiform clouds with favorable viewing geometry. The uncertainty is even greater if these conditions are not met. For averages over 1° ×1° regions the uncertainty is reduced to 54% assuming random errors for instrument uncertainties. In contrast, the few evaluation studies against reference in situ observations suggest much better accuracy with little variability in the bias. More such studies are required for a better error characterization. Nd uncertainty is dominated by errors in re, and therefore, improvements in re retrievals would greatly improve the quality of the Nd retrievals. Recommendations are revealed for how this might be achieved. Some existing Nd data sets are compared and discussed, and best practices for the use of Nd data from current passive instruments (e.g., filtering criteria) are recommended. Emerging alternative Nd estimates are also considered. First, new ideas to use additional information from existing and upcoming spaceborne instruments are discussed, and second, approaches using high-quality ground-based observations are examined.

Research Organization:
NASA Goddard Space Flight Center (GSFC), Greenbelt, MD (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER); Federal Ministry for Education and Research in Germany (BMBF); European Research Council (ERC)
Grant/Contract Number:
SC0016237
OSTI ID:
1457505
Alternate ID(s):
OSTI ID: 1457507; OSTI ID: 1547362
Journal Information:
Reviews of Geophysics (1985), Vol. 56, Issue 2; ISSN 8755-1209
Publisher:
American Geophysical Union (AGU)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 143 works
Citation information provided by
Web of Science

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journal April 2009
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Global indirect aerosol effects: a review journal January 2004
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A methodology for simultaneous retrieval of ice and liquid water cloud properties. Part I: Information content and case study: Multi-Layer Ice/Liquid Cloud Property Retrievals
  • Sourdeval, Odran; C. -Labonnote, Laurent; Baran, Anthony J.
  • Quarterly Journal of the Royal Meteorological Society, Vol. 141, Issue 688 https://doi.org/10.1002/qj.2405
journal August 2014
The role of the southern African easterly jet in modifying the southeast Atlantic aerosol and cloud environments: Role of the AEJ-S over Southeast Atlantic journal April 2016
Intercomparison of model simulations of mixed-phase clouds observed during the ARM Mixed-Phase Arctic Cloud Experiment. I: single-layer cloud
  • Klein, Stephen A.; McCoy, Renata B.; Morrison, Hugh
  • Quarterly Journal of the Royal Meteorological Society, Vol. 135, Issue 641 https://doi.org/10.1002/qj.416
journal April 2009
An observational study of the structure of stratiform cloud sheets: Part I. Structure journal April 1986
Metastable stratus tops journal April 1986
Pollution and the planetary albedo journal December 1974
New satellite project Aerosol-UA: Remote sensing of aerosols in the terrestrial atmosphere journal June 2016
Evaluation of ground-based remotely sensed liquid water cloud properties using shortwave radiation measurements journal May 2010
On the sensitivity of cloud effective radius retrieval based on spectral method to bi-modal droplet size distribution: A semi-analytical model journal November 2013
Accuracy assessments of cloud droplet size retrievals from polarized reflectance measurements by the research scanning polarimeter journal October 2012
Liquid water cloud properties during the Polarimeter Definition Experiment (PODEX) journal November 2015
Polarized view of supercooled liquid water clouds journal August 2016
Large contribution of natural aerosols to uncertainty in indirect forcing journal November 2013
Satellite-based estimate of global aerosol–cloud radiative forcing by marine warm clouds journal August 2014
Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability journal February 2016
Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers journal March 2016
Constraining the instantaneous aerosol influence on cloud albedo journal April 2017
Line Transfer in Two Dimensions journal July 1970
MODIS: advanced facility instrument for studies of the Earth as a system journal March 1989
The Influence of Cloud Nucleus Population on the Microstructure and Stability of Convective Clouds journal November 1959
The Multi-Viewing, -Channel, -Polarisation Imager (3MI) of the EUMETSAT Polar System - Second Generation (EPS-SG) dedicated to aerosol characterisation conference October 2013
Holographic measurements of inhomogeneous cloud mixing at the centimeter scale journal October 2015
The effect of overlying absorbing aerosol layers on remote sensing retrievals of cloud effective radius and cloud optical depth journal April 2004
Microphysical Properties of Winter Stratiform Clouds over the Southwest Islands Area in Japan [冬季南西諸島海域における層状雲の雲物理学的性質] journal January 1995
Long-term measurements of cloud droplet concentrations and aerosol–cloud interactions in continental boundary layer clouds journal September 2013
Subseasonal variability of low cloud radiative properties over the southeast Pacific Ocean journal January 2010
Microphysical variability in southeast Pacific Stratocumulus clouds: synoptic conditions and radiative response journal January 2010
Resolving both entrainment-mixing and number of activated CCN in deep convective clouds journal January 2011
Comparison of MODIS cloud microphysical properties with in-situ measurements over the Southeast Pacific journal January 2012
Composite study of aerosol export events from East Asia and North America journal January 2013
Development and impact of hooks of high droplet concentration on remote southeast Pacific stratocumulus journal January 2013
Study of global cloud droplet number concentration with A-Train satellites journal January 2014
The effect of solar zenith angle on MODIS cloud optical and microphysical retrievals within marine liquid water clouds journal January 2014
Global and regional modeling of clouds and aerosols in the marine boundary layer during VOCALS: the VOCA intercomparison journal January 2015
Unveiling aerosol–cloud interactions – Part 1: Cloud contamination in satellite products enhances the aerosol indirect forcing estimate journal January 2017
Sensitivity study of cloud parameterizations with relative dispersion in CAM5.1: impacts on aerosol indirect effects journal January 2017
Optimizing observations of drizzle onset with millimeter-wavelength radars journal January 2017
Differences in liquid cloud droplet effective radius and number concentration estimates between MODIS collections 5.1 and 6 over global oceans journal January 2017
Detection of multi-layer and vertically-extended clouds using A-train sensors journal January 2010
Cloud retrievals from satellite data using optimal estimation: evaluation and application to ATSR journal January 2012
Impact of cloud horizontal inhomogeneity and directional sampling on the retrieval of cloud droplet size by the POLDER instrument journal January 2015
Marine boundary layer cloud property retrievals from high-resolution ASTER observations: case studies and comparison with Terra MODIS journal January 2016

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Cloud Adiabaticity and Its Relationship to Marine Stratocumulus Characteristics Over the Northeast Pacific Ocean journal December 2018
The Impact of Ship Emission Controls Recorded by Cloud Properties journal November 2019
Observations of Aerosol‐Cloud Interactions During the North Atlantic Aerosol and Marine Ecosystem Study journal February 2020
Regional Biases in MODIS Marine Liquid Water Cloud Drop Effective Radius Deduced Through Fusion With MISR journal December 2019
Competing Effects of Droplet Sedimentation and Wind Shear on Entrainment in Stratocumulus journal June 2019
Analysis of polarimetric satellite measurements suggests stronger cooling due to aerosol-cloud interactions journal November 2019
Evaluating the diurnal cycle of South Atlantic stratocumulus clouds as observed by MSG SEVIRI journal January 2018
Subgrid variations of the cloud water and droplet number concentration over the tropical ocean: satellite observations and implications for warm rain simulations in climate models journal January 2019
The diurnal cycle of the smoky marine boundary layer observed during August in the remote southeast Atlantic journal January 2019
Is positive correlation between cloud droplet effective radius and aerosol optical depth over land due to retrieval artifacts or real physical processes? journal January 2019
The global aerosol–climate model ECHAM6.3–HAM2.3 – Part 2: Cloud evaluation, aerosol radiative forcing, and climate sensitivity journal January 2019
Cloud physics from space
  • Stephens, Graeme L.; Christensen, Matthew; Andrews, Timothy
  • Quarterly Journal of the Royal Meteorological Society, Vol. 145, Issue 724 https://doi.org/10.1002/qj.3589
journal August 2019
Reconstruction of Cloud Vertical Structure With a Generative Adversarial Network journal June 2019
Weak average liquid-cloud-water response to anthropogenic aerosols journal July 2019
The challenge of simulating the sensitivity of the Amazonian cloud microstructure to cloud condensation nuclei number concentrations journal January 2020
Ultra-clean and smoky marine boundary layers frequently occur in the same season over the southeast Atlantic journal January 2020
Parameterizing cloud top effective radii from satellite retrieved values, accounting for vertical photon transport: quantification and correction of the resulting bias in droplet concentration and liquid water path retrievals journal January 2018
Improvement of airborne retrievals of cloud droplet number concentration of trade wind cumulus using a synergetic approach journal January 2019
The global aerosol-climate model ECHAM6.3-HAM2.3-Part 2: Cloud evaluation, aerosol radiative forcing, and climate sensitivity text January 2019
Constraining the aerosol influence on cloud liquid water path journal January 2019
Anthropogenic Air Pollution Delays Marine Stratocumulus Breakup to Open Cells journal December 2019
The sub-adiabatic model as a concept for evaluating the representation and radiative effects of low-level clouds in a high-resolution atmospheric model journal January 2020
Sensitivity of liquid cloud optical thickness and effective radius retrievals to cloud bow and glory conditions using two SEVIRI imagers journal January 2019
A new approach to estimate supersaturation fluctuations in stratocumulus cloud using ground-based remote-sensing measurements journal January 2019
Anthropogenic aerosol forcing – insights from multiple estimates from aerosol-climate models with reduced complexity journal January 2019
Ultra-clean and smoky marine boundary layers frequently occur in the same season over the southeast Atlantic journal July 2019
Competing Effects of Droplet Sedimentation and Wind Shear on Entrainment in Stratocumulus text January 2019
Marine liquid cloud geometric thickness retrieved from OCO-2's oxygen A-band spectrometer journal January 2019
Observations of Aerosol‐Cloud Interactions During the North Atlantic Aerosol and Marine Ecosystem Study text January 2020
Regional Biases in MODIS Marine Liquid Water Cloud Drop Effective Radius Deduced Through Fusion With MISR journal December 2019
Analysis of polarimetric satellite measurements suggests stronger cooling due to aerosol-cloud interactions journal November 2019
Evaluating the diurnal cycle of South Atlantic stratocumulus clouds as observed by MSG SEVIRI journal January 2018
Ice crystal number concentration estimates from lidar–radar satellite remote sensing – Part 1: Method and evaluation journal January 2018
The diurnal cycle of the smoky marine boundary layer observed during August in the remote southeast Atlantic journal January 2019
The value of remote marine aerosol measurements for constraining radiative forcing uncertainty journal January 2020
The decomposition of cloud–aerosol forcing in the UK Earth System Model (UKESM1) journal January 2020
Evaluation of aerosol and cloud properties in three climate models using MODIS observations and its corresponding COSP simulator, as well as their application in aerosol–cloud interactions journal February 2020
Untangling causality in midlatitude aerosol–cloud adjustments journal April 2020
An observational study of the effects of aerosols on diurnal variation of heavy rainfall and associated clouds over Beijing–Tianjin–Hebei journal January 2020
Ultra-clean and smoky marine boundary layers frequently occur in the same season over the southeast Atlantic journal July 2019
Vertical dependence of horizontal variation of cloud microphysics: observations from the ACE-ENA field campaign and implications for warm-rain simulation in climate models journal January 2021
A new approach to estimate supersaturation fluctuations in stratocumulus cloud using ground-based remote-sensing measurements journal January 2019
Detection and attribution of aerosol-cloud interactions in large-domain large-eddy simulations with the ICOsahedral Non-hydrostatic model text January 2020