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Title: Response to the comment “Uranyl-chloride speciation and uranium transport in hydrothermal brines: Comment on Migdisov et al. (2018)” by Dargent et al.

Abstract

We welcome the comments provided by Dargent et al. (2018) and appreciate the effort they have made to evaluate our recently reported data on the stability of uranyl(VI) chloride complexes as function of temperature (Migdisov et al., 2018). We also appreciate the opportunity provided by the editor to clarify issues in our paper that were not clearly articulated or in error.

Authors:
 [1];  [1];  [2];  [1];  [1];  [2]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. McGill Univ., Montreal, QC (Canada). Dept. of Earth and Planetary Sciences
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Laboratory Directed Research and Development (LDRD) Program
OSTI Identifier:
1457312
Report Number(s):
LA-UR-18-21513
Journal ID: ISSN 0016-7037; TRN: US1901352
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Geochimica et Cosmochimica Acta
Additional Journal Information:
Journal Volume: 235; Journal ID: ISSN 0016-7037
Publisher:
The Geochemical Society; The Meteoritical Society
Country of Publication:
United States
Language:
English
Subject:
38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY; response; spectroscopy; uranyl; chloride; hydrothermal

Citation Formats

Migdisov, A. A., Runde, W., Williams-Jones, A. E., Boukhalfa, H., Roback, R., and Timofeev, A. Response to the comment “Uranyl-chloride speciation and uranium transport in hydrothermal brines: Comment on Migdisov et al. (2018)” by Dargent et al.. United States: N. p., 2018. Web. doi:10.1016/j.gca.2018.06.015.
Migdisov, A. A., Runde, W., Williams-Jones, A. E., Boukhalfa, H., Roback, R., & Timofeev, A. Response to the comment “Uranyl-chloride speciation and uranium transport in hydrothermal brines: Comment on Migdisov et al. (2018)” by Dargent et al.. United States. doi:10.1016/j.gca.2018.06.015.
Migdisov, A. A., Runde, W., Williams-Jones, A. E., Boukhalfa, H., Roback, R., and Timofeev, A. Wed . "Response to the comment “Uranyl-chloride speciation and uranium transport in hydrothermal brines: Comment on Migdisov et al. (2018)” by Dargent et al.". United States. doi:10.1016/j.gca.2018.06.015. https://www.osti.gov/servlets/purl/1457312.
@article{osti_1457312,
title = {Response to the comment “Uranyl-chloride speciation and uranium transport in hydrothermal brines: Comment on Migdisov et al. (2018)” by Dargent et al.},
author = {Migdisov, A. A. and Runde, W. and Williams-Jones, A. E. and Boukhalfa, H. and Roback, R. and Timofeev, A.},
abstractNote = {We welcome the comments provided by Dargent et al. (2018) and appreciate the effort they have made to evaluate our recently reported data on the stability of uranyl(VI) chloride complexes as function of temperature (Migdisov et al., 2018). We also appreciate the opportunity provided by the editor to clarify issues in our paper that were not clearly articulated or in error.},
doi = {10.1016/j.gca.2018.06.015},
journal = {Geochimica et Cosmochimica Acta},
number = ,
volume = 235,
place = {United States},
year = {2018},
month = {6}
}

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Figures / Tables:

Figure 1 Figure 1: Erratum to Figure 11 from Migdisov et al. (2018): a-d) Distribution of uranyl-chloride species as a function of the logarithm of total molality of NaCl in aqueous solutions calculated for 25 to 300 °C based on the data obtained in this study. Shaded areas show the range ofmore » concentrations not covered in our study (contribution of other species is not excluded). e-h) Distribution of uranyl-chloride species at the same conditions calculated using the data reported by Dargent et al. (2013).« less

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