Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond
Abstract
Quantum emitters are an integral component for a broad range of quantum technologies, including quantum communication, quantum repeaters, and linear optical quantum computation. Solid-state color centers are promising candidates for scalable quantum optics due to their long coherence time and small inhomogeneous broadening. However, once excited, color centers often decay through phonon-assisted processes, limiting the efficiency of single-photon generation and photon-mediated entanglement generation. Herein, we demonstrate strong enhancement of spontaneous emission rate of a single silicon-vacancy center in diamond embedded within a monolithic optical cavity, reaching a regime in which the excited-state lifetime is dominated by spontaneous emission into the cavity mode. We observe 10-fold lifetime reduction and 42-fold enhancement in emission intensity when the cavity is tuned into resonance with the optical transition of a single silicon-vacancy center, corresponding to 90% of the excited-state energy decay occurring through spontaneous emission into the cavity mode. Here, we also demonstrate the largest coupling strength (g/2π = 4.9 ± 0.3 GHz) and cooperativity (C = 1.4) to date for color-center-based cavity quantum electrodynamics systems, bringing the system closer to the strong coupling regime.
- Authors:
-
[1];
[1];
[1];
- Stanford Univ., Stanford, CA (United States)
- Harvard Univ., Cambridge, MA (United States)
- Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1457052
- Grant/Contract Number:
- EFRI-5710004174; W911NF1310309; N00014-15-1-2761; AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 18; Journal Issue: 2; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; color center; defect-center materials; diamond; nanophotonics; Purcell enhancement; silicon-vacancy center; single-photon generation
Citation Formats
Zhang, Jingyuan Linda, Sun, Shuo, Burek, Michael J., Dory, Constantin, Tzeng, Yan -Kai, Fischer, Kevin A., Kelaita, Yousif, Lagoudakis, Konstantinos G., Radulaski, Marina, Shen, Zhi -Xun, Melosh, Nicholas A., Chu, Steven, Loncar, Marko, and Vuckovic, Jelena. Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond. United States: N. p., 2018.
Web. doi:10.1021/acs.nanolett.7b05075.
Zhang, Jingyuan Linda, Sun, Shuo, Burek, Michael J., Dory, Constantin, Tzeng, Yan -Kai, Fischer, Kevin A., Kelaita, Yousif, Lagoudakis, Konstantinos G., Radulaski, Marina, Shen, Zhi -Xun, Melosh, Nicholas A., Chu, Steven, Loncar, Marko, & Vuckovic, Jelena. Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond. United States. https://doi.org/10.1021/acs.nanolett.7b05075
Zhang, Jingyuan Linda, Sun, Shuo, Burek, Michael J., Dory, Constantin, Tzeng, Yan -Kai, Fischer, Kevin A., Kelaita, Yousif, Lagoudakis, Konstantinos G., Radulaski, Marina, Shen, Zhi -Xun, Melosh, Nicholas A., Chu, Steven, Loncar, Marko, and Vuckovic, Jelena. Mon .
"Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond". United States. https://doi.org/10.1021/acs.nanolett.7b05075. https://www.osti.gov/servlets/purl/1457052.
@article{osti_1457052,
title = {Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond},
author = {Zhang, Jingyuan Linda and Sun, Shuo and Burek, Michael J. and Dory, Constantin and Tzeng, Yan -Kai and Fischer, Kevin A. and Kelaita, Yousif and Lagoudakis, Konstantinos G. and Radulaski, Marina and Shen, Zhi -Xun and Melosh, Nicholas A. and Chu, Steven and Loncar, Marko and Vuckovic, Jelena},
abstractNote = {Quantum emitters are an integral component for a broad range of quantum technologies, including quantum communication, quantum repeaters, and linear optical quantum computation. Solid-state color centers are promising candidates for scalable quantum optics due to their long coherence time and small inhomogeneous broadening. However, once excited, color centers often decay through phonon-assisted processes, limiting the efficiency of single-photon generation and photon-mediated entanglement generation. Herein, we demonstrate strong enhancement of spontaneous emission rate of a single silicon-vacancy center in diamond embedded within a monolithic optical cavity, reaching a regime in which the excited-state lifetime is dominated by spontaneous emission into the cavity mode. We observe 10-fold lifetime reduction and 42-fold enhancement in emission intensity when the cavity is tuned into resonance with the optical transition of a single silicon-vacancy center, corresponding to 90% of the excited-state energy decay occurring through spontaneous emission into the cavity mode. Here, we also demonstrate the largest coupling strength (g/2π = 4.9 ± 0.3 GHz) and cooperativity (C = 1.4) to date for color-center-based cavity quantum electrodynamics systems, bringing the system closer to the strong coupling regime.},
doi = {10.1021/acs.nanolett.7b05075},
journal = {Nano Letters},
number = 2,
volume = 18,
place = {United States},
year = {Mon Jan 29 00:00:00 EST 2018},
month = {Mon Jan 29 00:00:00 EST 2018}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 94 works
Citation information provided by
Web of Science
Web of Science
Figures / Tables:
Figure 1: High-Q nanobeam photonic crystal cavity. (a) Scanning electron microscopy (SEM) images of a nanobeam photonic crystal (PhC) cavity fabricated from single crystal diamond, with the inset showing the angled-view of the cavity region. Scale bars in (a) and the inset: 5 μm and 1 μm respectively. (b) Electricmore »
All figures and tables
(5 total)
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Solid-state single-photon emitters
journal, September 2016
- Aharonovich, Igor; Englund, Dirk; Toth, Milos
- Nature Photonics, Vol. 10, Issue 10
Secure quantum key distribution
journal, July 2014
- Lo, Hoi-Kwong; Curty, Marcos; Tamaki, Kiyoshi
- Nature Photonics, Vol. 8, Issue 8
Linear optical quantum computing with photonic qubits
journal, January 2007
- Kok, Pieter; Munro, W. J.; Nemoto, Kae
- Reviews of Modern Physics, Vol. 79, Issue 1
Time-Bin-Encoded Boson Sampling with a Single-Photon Device
journal, May 2017
- He, Yu; Ding, X.; Su, Z. -E.
- Physical Review Letters, Vol. 118, Issue 19
Boson Sampling with Single-Photon Fock States from a Bright Solid-State Source
journal, March 2017
- Loredo, J. C.; Broome, M. A.; Hilaire, P.
- Physical Review Letters, Vol. 118, Issue 13
High-efficiency multiphoton boson sampling
journal, May 2017
- Wang, Hui; He, Yu; Li, Yu-Huai
- Nature Photonics, Vol. 11, Issue 6
Quantum key distribution over 120 km using ultrahigh purity single-photon source and superconducting single-photon detectors
journal, September 2015
- Takemoto, Kazuya; Nambu, Yoshihiro; Miyazawa, Toshiyuki
- Scientific Reports, Vol. 5, Issue 1
Quantum key distribution using quantum dot single-photon emitting diodes in the red and near infrared spectral range
journal, August 2012
- Heindel, Tobias; Kessler, Christian A.; Rau, Markus
- New Journal of Physics, Vol. 14, Issue 8
Room-temperature entanglement between single defect spins in diamond
journal, February 2013
- Dolde, F.; Jakobi, I.; Naydenov, B.
- Nature Physics, Vol. 9, Issue 3
Loophole-free Bell inequality violation using electron spins separated by 1.3 kilometres
journal, October 2015
- Hensen, B.; Bernien, H.; Dréau, A. E.
- Nature, Vol. 526, Issue 7575
Generation of heralded entanglement between distant hole spins
journal, December 2015
- Delteil, Aymeric; Sun, Zhe; Gao, Wei-bo
- Nature Physics, Vol. 12, Issue 3
Phase-Tuned Entangled State Generation between Distant Spin Qubits
journal, July 2017
- Stockill, R.; Stanley, M. J.; Huthmacher, L.
- Physical Review Letters, Vol. 119, Issue 1
Ultralong spin coherence time in isotopically engineered diamond
journal, April 2009
- Balasubramanian, Gopalakrishnan; Neumann, Philipp; Twitchen, Daniel
- Nature Materials, Vol. 8, Issue 5
Room-Temperature Quantum Bit Memory Exceeding One Second
journal, June 2012
- Maurer, P. C.; Kucsko, G.; Latta, C.
- Science, Vol. 336, Issue 6086
Coherent control of single spins in silicon carbide at room temperature
journal, December 2014
- Widmann, Matthias; Lee, Sang-Yun; Rendler, Torsten
- Nature Materials, Vol. 14, Issue 2
Room temperature coherent control of defect spin qubits in silicon carbide
journal, November 2011
- Koehl, William F.; Buckley, Bob B.; Heremans, F. Joseph
- Nature, Vol. 479, Issue 7371
Multiple intrinsically identical single-photon emitters in the solid state
journal, August 2014
- Rogers, L. J.; Jahnke, K. D.; Teraji, T.
- Nature Communications, Vol. 5, Issue 1
One- and two-dimensional photonic crystal microcavities in single crystal diamond
journal, November 2011
- Riedrich-Möller, Janine; Kipfstuhl, Laura; Hepp, Christian
- Nature Nanotechnology, Vol. 7, Issue 1
Deterministic coupling of delta-doped nitrogen vacancy centers to a nanobeam photonic crystal cavity
journal, December 2014
- Lee, Jonathan C.; Bracher, David O.; Cui, Shanying
- Applied Physics Letters, Vol. 105, Issue 26
Coupling of Nitrogen-Vacancy Centers to Photonic Crystal Cavities in Monocrystalline Diamond
journal, July 2012
- Faraon, Andrei; Santori, Charles; Huang, Zhihong
- Physical Review Letters, Vol. 109, Issue 3
Resonant enhancement of the zero-phonon emission from a colour centre in a diamond cavity
journal, April 2011
- Faraon, Andrei; Barclay, Paul E.; Santori, Charles
- Nature Photonics, Vol. 5, Issue 5
Coupling of NV Centers to Photonic Crystal Nanobeams in Diamond
journal, November 2013
- Hausmann, B. J. M.; Shields, B. J.; Quan, Q.
- Nano Letters, Vol. 13, Issue 12
Deterministic Coupling of a Single Silicon-Vacancy Color Center to a Photonic Crystal Cavity in Diamond
journal, August 2014
- Riedrich-Möller, Janine; Arend, Carsten; Pauly, Christoph
- Nano Letters, Vol. 14, Issue 9
An integrated diamond nanophotonics platform for quantum-optical networks
journal, October 2016
- Sipahigil, A.; Evans, R. E.; Sukachev, D. D.
- Science, Vol. 354, Issue 6314
Fiber-Coupled Diamond Quantum Nanophotonic Interface
journal, August 2017
- Burek, Michael J.; Meuwly, Charles; Evans, Ruffin E.
- Physical Review Applied, Vol. 8, Issue 2
Selective Purcell enhancement of two closely linked zero-phonon transitions of a silicon carbide color center
journal, April 2017
- Bracher, David O.; Zhang, Xingyu; Hu, Evelyn L.
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 16
Vertical-Substrate MPCVD Epitaxial Nanodiamond Growth
journal, February 2017
- Tzeng, Yan-Kai; Zhang, Jingyuan Linda; Lu, Haiyu
- Nano Letters, Vol. 17, Issue 3
Complete coherent control of silicon vacancies in diamond nanopillars containing single defect centers
journal, January 2017
- Zhang, Jingyuan Linda; Lagoudakis, Konstantinos G.; Tzeng, Yan-Kai
- Optica, Vol. 4, Issue 11
Narrow-Linewidth Homogeneous Optical Emitters in Diamond Nanostructures via Silicon Ion Implantation
journal, April 2016
- Evans, Ruffin E.; Sipahigil, Alp; Sukachev, Denis D.
- Physical Review Applied, Vol. 5, Issue 4
Hybrid Group IV Nanophotonic Structures Incorporating Diamond Silicon-Vacancy Color Centers
journal, December 2015
- Zhang, Jingyuan Linda; Ishiwata, Hitoshi; Babinec, Thomas M.
- Nano Letters, Vol. 16, Issue 1
Faraday cage angled-etching of nanostructures in bulk dielectrics
journal, July 2016
- Latawiec, Pawel; Burek, Michael J.; Sohn, Young-Ik
- Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 34, Issue 4
Free-Standing Mechanical and Photonic Nanostructures in Single-Crystal Diamond
journal, February 2012
- Burek, Michael J.; de Leon, Nathalie P.; Shields, Brendan J.
- Nano Letters, Vol. 12, Issue 12, p. 6084-6089
Fabrication of triangular nanobeam waveguide networks in bulk diamond using single-crystal silicon hard masks
journal, November 2014
- Bayn, I.; Mouradian, S.; Li, L.
- Applied Physics Letters, Vol. 105, Issue 21
High quality factor photonic crystal nanobeam cavities
journal, March 2009
- Deotare, Parag B.; McCutcheon, Murray W.; Frank, Ian W.
- Applied Physics Letters, Vol. 94, Issue 12
Cavity-Enhanced Single-Photon Source Based on the Silicon-Vacancy Center in Diamond
journal, February 2017
- Benedikter, Julia; Kaupp, Hanno; Hümmer, Thomas
- Physical Review Applied, Vol. 7, Issue 2
Coherent spin control of a nanocavity-enhanced qubit in diamond
journal, January 2015
- Li, Luozhou; Schröder, Tim; Chen, Edward H.
- Nature Communications, Vol. 6, Issue 1
Hybrid Nanocavity Resonant Enhancement of Color Center Emission in Diamond
journal, September 2011
- Barclay, Paul E.; Fu, Kai-Mei C.; Santori, Charles
- Physical Review X, Vol. 1, Issue 1
Spontaneous emission and collection efficiency enhancement of single emitters in diamond via plasmonic cavities and gratings
journal, October 2013
- Choy, Jennifer T.; Bulu, Irfan; Hausmann, Birgit J. M.
- Applied Physics Letters, Vol. 103, Issue 16
Coupling of silicon-vacancy centers to a single crystal diamond cavity
journal, January 2012
- Lee, Jonathan C.; Aharonovich, Igor; Magyar, Andrew P.
- Optics Express, Vol. 20, Issue 8
Enhanced single-photon emission from a diamond–silver aperture
journal, October 2011
- Choy, Jennifer T.; Hausmann, Birgit J. M.; Babinec, Thomas M.
- Nature Photonics, Vol. 5, Issue 12
Deterministic Coupling of a Single Nitrogen Vacancy Center to a Photonic Crystal Cavity
journal, October 2010
- Englund, Dirk; Shields, Brendan; Rivoire, Kelley
- Nano Letters, Vol. 10, Issue 10
Deterministic Enhancement of Coherent Photon Generation from a Nitrogen-Vacancy Center in Ultrapure Diamond
journal, September 2017
- Riedel, Daniel; Söllner, Immo; Shields, Brendan J.
- Physical Review X, Vol. 7, Issue 3
Purcell-Enhanced Single-Photon Emission from Nitrogen-Vacancy Centers Coupled to a Tunable Microcavity
journal, November 2016
- Kaupp, Hanno; Hümmer, Thomas; Mader, Matthias
- Physical Review Applied, Vol. 6, Issue 5
Nanophotonic coherent light–matter interfaces based on rare-earth-doped crystals
journal, September 2015
- Zhong, Tian; Kindem, Jonathan M.; Miyazono, Evan
- Nature Communications, Vol. 6, Issue 1
Dipole Induced Transparency in Drop-Filter Cavity-Waveguide Systems
journal, April 2006
- Waks, Edo; Vuckovic, Jelena
- Physical Review Letters, Vol. 96, Issue 15
Electron–phonon processes of the silicon-vacancy centre in diamond
journal, April 2015
- Jahnke, Kay D.; Sipahigil, Alp; Binder, Jan M.
- New Journal of Physics, Vol. 17, Issue 4
Electronic Structure of the Silicon Vacancy Color Center in Diamond
journal, January 2014
- Hepp, Christian; Müller, Tina; Waselowski, Victor
- Physical Review Letters, Vol. 112, Issue 3
Quantum Nonlinear Optics with a Germanium-Vacancy Color Center in a Nanoscale Diamond Waveguide
journal, May 2017
- Bhaskar, M. K.; Sukachev, D. D.; Sipahigil, A.
- Physical Review Letters, Vol. 118, Issue 22
Optical and microwave control of germanium-vacancy center spins in diamond
journal, August 2017
- Siyushev, Petr; Metsch, Mathias H.; Ijaz, Aroosa
- Physical Review B, Vol. 96, Issue 8
Rectangular photonic crystal nanobeam cavities in bulk diamond
journal, July 2017
- Mouradian, Sara; Wan, Noel H.; Schröder, Tim
- Applied Physics Letters, Vol. 111, Issue 2
Interfacing broadband photonic qubits to on-chip cavity-protected rare-earth ensembles
journal, January 2017
- Zhong, Tian; Kindem, Jonathan M.; Rochman, Jake
- Nature Communications, Vol. 8, Issue 1
Observation of normal-mode splitting for an atom in an optical cavity
journal, February 1992
- Thompson, R. J.; Rempe, G.; Kimble, H. J.
- Physical Review Letters, Vol. 68, Issue 8
Photon blockade in two-emitter-cavity systems
journal, July 2017
- Radulaski, Marina; Fischer, Kevin A.; Lagoudakis, Konstantinos G.
- Physical Review A, Vol. 96, Issue 1
Interfacing broadband photonic qubits to on-chip cavity-protected rare-earth ensembles
journal, January 2017
- Zhong, Tian; Kindem, Jonathan M.; Rochman, Jake
- Nature Communications, Vol. 8, Issue 1
Resonant enhancement of the zero-phonon emission from a colour centre in a diamond cavity
journal, April 2011
- Faraon, Andrei; Barclay, Paul E.; Santori, Charles
- Nature Photonics, Vol. 5, Issue 5
High Quality factor photonic crystal nanobeam cavities
text, January 2009
- Deotare, Parag B.; McCutcheon, Murray W.; Frank, Ian W.
- arXiv
Spontaneous emission and collection efficiency enhancement of single emitters in diamond via plasmonic cavities and gratings
text, January 2013
- Choy, Jennifer T.; Bulu, Irfan; Hausmann, Birgit J. M.
- arXiv
Faraday cage angled-etching of nanostructures in bulk dielectrics
preprint, January 2016
- Latawiec, Pawel; Burek, Michael J.; Sohn, Young-Ik
- arXiv
Rectangular Photonic Crystal Nanobeam Cavities in Bulk Diamond
text, January 2017
- Mouradian, Sara; Wan, Noel H.; Schröder, Tim
- arXiv
Dipole induced transparency in drop-filter cavity-waveguide systems
text, January 2005
- Waks, Edo; Vuckovic, Jelena
- arXiv
Purcell-Enhanced Single-Photon Emission from Nitrogen-Vacancy Centers Coupled to a Tunable Microcavity
text, January 2016
- Kaupp, Hanno; Hümmer, Thomas; Mader, Matthias
- Karlsruhe
Works referencing / citing this record:
Nanodiamond Integration with Photonic Devices
journal, July 2019
- Radulaski, Marina; Zhang, Jingyuan Linda; Tzeng, Yan‐Kai
- Laser & Photonics Reviews, Vol. 13, Issue 8
Diamond as a Platform for Integrated Quantum Photonics
journal, October 2018
- Lenzini, Francesco; Gruhler, Nico; Walter, Nicolai
- Advanced Quantum Technologies, Vol. 1, Issue 3
Photon-mediated interactions between quantum emitters in a diamond nanocavity
journal, September 2018
- Evans, R. E.; Bhaskar, M. K.; Sukachev, D. D.
- Science, Vol. 362, Issue 6415
Manipulating spontaneous emission spectra using two-dimensional elliptical microcavities
journal, January 2019
- Xu, Kaiyuan; Jiang, Chun
- Journal of the Optical Society of America B, Vol. 36, Issue 12
Fabrication of highly dense arrays of nanocrystalline diamond nanopillars with integrated silicon-vacancy color centers during the growth
journal, January 2019
- Schmidt, Alexander; Naydenov, Boris; Jelezko, Fedor
- Optical Materials Express, Vol. 9, Issue 12
Deterministic coupling of site-controlled quantum emitters in monolayer WSe2 to plasmonic nanocavities
journal, October 2018
- Luo, Yue; Shepard, Gabriella D.; Ardelean, Jenny V.
- Nature Nanotechnology, Vol. 13, Issue 12
Developing a time-domain method for simulating statistical behavior of many-emitter systems in the presence of electromagnetic field
journal, January 2020
- Hashemi, A. R.; Hosseini-Farzad, M.
- Physical Review E, Vol. 101, Issue 1
Optical coherence of implanted silicon vacancy centers in thin diamond membranes
journal, January 2019
- Lekavicius, Ignas; Wang, Hailin
- Optics Express, Vol. 27, Issue 22
Direct writing of single germanium vacancy center arrays in diamond
journal, December 2018
- Zhou, Yu; Mu, Zhao; Adamo, Giorgio
- New Journal of Physics, Vol. 20, Issue 12
Inverse-designed diamond photonics
journal, July 2019
- Dory, Constantin; Vercruysse, Dries; Yang, Ki Youl
- Nature Communications, Vol. 10, Issue 1
Advances in quantum light emission from 2D materials
journal, August 2019
- Chakraborty, Chitraleema; Vamivakas, Nick; Englund, Dirk
- Nanophotonics, Vol. 8, Issue 11
Enhanced spin state readout of nitrogen-vacancy centers in diamond using infrared fluorescence
journal, September 2019
- Meirzada, I.; Wolf, S. A.; Naiman, A.
- Physical Review B, Vol. 100, Issue 12
Building Blocks for Quantum Network Based on Group‐IV Split‐Vacancy Centers in Diamond
journal, October 2019
- Chen, Disheng; Zheludev, Nikolay; Gao, Wei‐bo
- Advanced Quantum Technologies, Vol. 3, Issue 2
Fabrication of highly dense arrays of nanocrystalline diamond nanopillars with integrated silicon-vacancy color centers during the growth
text, January 2019
- Schmidt, Alexander; Naydenov, Boris; Jelezko, Fedor
- Universität Kassel
Nanodiamond integration with photonic devices
preprint, January 2016
- Radulaski, Marina; Zhang, Jingyuan Linda; Tzeng, Yan-Kai
- arXiv
Strain engineering of the silicon-vacancy center in diamond
text, January 2018
- Meesala, Srujan; Sohn, Young-Ik; Pingault, Benjamin
- arXiv
Inverse-Designed Diamond Photonics
text, January 2018
- Dory, Constantin; Vercruysse, Dries; Yang, Ki Youl
- arXiv
Enhanced spin state readout of Nitrogen-Vacancy centers in diamond using IR fluorescence
text, January 2019
- Meirzada, Idan; Wolf, Sigal A.; Naiman, Alex
- arXiv
Developing a time-domain method for simulating statistical behaviour of many-emitter systems in the presence of electromagnetic field
text, January 2019
- Hashemi, Ali Reza; Hosseini-Farzad, Mahmood
- arXiv
Inverse-Designed Diamond Photonics
text, January 2018
- Dory, Constantin; Vercruysse, Dries; Yang, Ki Youl
- arXiv
Figures / Tables found in this record:
Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.