Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods
Abstract
Increased natural gas production in recent years has spurred intense interest in methane (CH4) emissions associated with its production, gathering, processing, transmission, and distribution. Gathering and processing facilities (G&P facilities) are unique in that the wide range of gas sources (shale, coal-bed, tight gas, conventional, etc.) results in a wide range of gas compositions, which in turn requires an array of technologies to prepare the gas for pipeline transmission and distribution. We present an overview and detailed description of the measurement method and analysis approach used during a 20-week field campaign studying CH4 emissions from the natural gas G&P facilities between October 2013 and April 2014. Dual-tracer flux measurements and on-site observations were used to address the magnitude and origins of CH4 emissions from these facilities. The use of a second tracer as an internal standard revealed plume-specific uncertainties in the measured emission rates of 20–47%, depending upon plume classification. Furthermore, combining downwind methane, ethane (C2H6), carbon monoxide (CO), carbon dioxide (CO2), and tracer gas measurements with on-site tracer gas release allows for quantification of facility emissions and in some cases a more detailed picture of source locations.
- Authors:
-
- Aerodyne Research Inc., Billerica, MA (United States)
- Carnegie Mellon Univ., Pittsburgh, PA (United States)
- Colorado State Univ., Fort Collins, CO (United States)
- Fort Lewis College, Durango, CO (United States)
- Publication Date:
- Research Org.:
- Aerodyne Research Inc., Billerica, MA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1455195
- Grant/Contract Number:
- SC0004578
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Atmospheric Measurement Techniques (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Measurement Techniques (Online); Journal Volume: 8; Journal Issue: 5; Journal ID: ISSN 1867-8548
- Publisher:
- European Geosciences Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 03 NATURAL GAS
Citation Formats
Roscioli, J. R., Yacovitch, T. I., Floerchinger, C., Mitchell, A. L., Tkacik, D. S., Subramanian, R., Martinez, D. M., Vaughn, T. L., Williams, L., Zimmerle, D., Robinson, A. L., Herndon, S. C., and Marchese, A. J. Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods. United States: N. p., 2015.
Web. doi:10.5194/amt-8-2017-2015.
Roscioli, J. R., Yacovitch, T. I., Floerchinger, C., Mitchell, A. L., Tkacik, D. S., Subramanian, R., Martinez, D. M., Vaughn, T. L., Williams, L., Zimmerle, D., Robinson, A. L., Herndon, S. C., & Marchese, A. J. Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods. United States. https://doi.org/10.5194/amt-8-2017-2015
Roscioli, J. R., Yacovitch, T. I., Floerchinger, C., Mitchell, A. L., Tkacik, D. S., Subramanian, R., Martinez, D. M., Vaughn, T. L., Williams, L., Zimmerle, D., Robinson, A. L., Herndon, S. C., and Marchese, A. J. Thu .
"Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods". United States. https://doi.org/10.5194/amt-8-2017-2015. https://www.osti.gov/servlets/purl/1455195.
@article{osti_1455195,
title = {Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods},
author = {Roscioli, J. R. and Yacovitch, T. I. and Floerchinger, C. and Mitchell, A. L. and Tkacik, D. S. and Subramanian, R. and Martinez, D. M. and Vaughn, T. L. and Williams, L. and Zimmerle, D. and Robinson, A. L. and Herndon, S. C. and Marchese, A. J.},
abstractNote = {Increased natural gas production in recent years has spurred intense interest in methane (CH4) emissions associated with its production, gathering, processing, transmission, and distribution. Gathering and processing facilities (G&P facilities) are unique in that the wide range of gas sources (shale, coal-bed, tight gas, conventional, etc.) results in a wide range of gas compositions, which in turn requires an array of technologies to prepare the gas for pipeline transmission and distribution. We present an overview and detailed description of the measurement method and analysis approach used during a 20-week field campaign studying CH4 emissions from the natural gas G&P facilities between October 2013 and April 2014. Dual-tracer flux measurements and on-site observations were used to address the magnitude and origins of CH4 emissions from these facilities. The use of a second tracer as an internal standard revealed plume-specific uncertainties in the measured emission rates of 20–47%, depending upon plume classification. Furthermore, combining downwind methane, ethane (C2H6), carbon monoxide (CO), carbon dioxide (CO2), and tracer gas measurements with on-site tracer gas release allows for quantification of facility emissions and in some cases a more detailed picture of source locations.},
doi = {10.5194/amt-8-2017-2015},
journal = {Atmospheric Measurement Techniques (Online)},
number = 5,
volume = 8,
place = {United States},
year = {Thu May 07 00:00:00 EDT 2015},
month = {Thu May 07 00:00:00 EDT 2015}
}
Web of Science
Works referenced in this record:
Collection of Leakage Statistics in the Natural Gas System by Tracer Methods
journal, July 1997
- Shorter, Joanne H.; McManus, J. Barry; Kolb, Charles E.
- Environmental Science & Technology, Vol. 31, Issue 7
Hydrocarbon emissions characterization in the Colorado Front Range: A pilot study: COLORADO FRONT RANGE EMISSIONS STUDY
journal, February 2012
- Pétron, Gabrielle; Frost, Gregory; Miller, Benjamin R.
- Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D4
Isoprene emission fluxes determined by an atmospheric tracer techniquE
journal, January 1986
- Lamb, B.; Westberg, H.; Allwine, G.
- Atmospheric Environment (1967), Vol. 20, Issue 1
Landfill methane emissions measured by enclosure and atmospheric tracer methods
journal, July 1996
- Czepiel, P. M.; Mosher, B.; Harriss, R. C.
- Journal of Geophysical Research: Atmospheres, Vol. 101, Issue D11
A high precision pulsed quantum cascade laser spectrometer for measurements of stable isotopes of carbon dioxide
journal, November 2005
- McManus, J. B.; Nelson, D. D.; Shorter, J. H.
- Journal of Modern Optics, Vol. 52, Issue 16
Atmospheric Hydrocarbon Emissions and Concentrations in the Barnett Shale Natural Gas Production Region
journal, April 2014
- Zavala-Araiza, Daniel; Sullivan, David W.; Allen, David T.
- Environmental Science & Technology, Vol. 48, Issue 9
Coupled weather research and forecasting–stochastic time-inverted lagrangian transport (WRF–STILT) model
journal, May 2010
- Nehrkorn, Thomas; Eluszkiewicz, Janusz; Wofsy, Steven C.
- Meteorology and Atmospheric Physics, Vol. 107, Issue 1-2
Methane Emissions from United States Natural Gas Gathering and Processing
journal, August 2015
- Marchese, Anthony J.; Vaughn, Timothy L.; Zimmerle, Daniel J.
- Environmental Science & Technology, Vol. 49, Issue 17
Characterization of urban pollutant emission fluxes and ambient concentration distributions using a mobile laboratory with rapid response instrumentation
journal, January 2005
- Herndon, Scott C.; Jayne, John T.; Zahniser, Mark S.
- Faraday Discussions, Vol. 130
Atmospheric Emission Characterization of Marcellus Shale Natural Gas Development Sites
journal, May 2015
- Goetz, J. Douglas; Floerchinger, Cody; Fortner, Edward C.
- Environmental Science & Technology, Vol. 49, Issue 11
Methane Emissions from the Natural Gas Transmission and Storage System in the United States
journal, July 2015
- Zimmerle, Daniel J.; Williams, Laurie L.; Vaughn, Timothy L.
- Environmental Science & Technology, Vol. 49, Issue 15
Demonstration of an Ethane Spectrometer for Methane Source Identification
journal, June 2014
- Yacovitch, Tara I.; Herndon, Scott C.; Roscioli, Joseph R.
- Environmental Science & Technology, Vol. 48, Issue 14
A cavity ring-down analyzer for measuring atmospheric levels of methane, carbon dioxide, and water vapor
journal, August 2008
- Crosson, E.R.
- Applied Physics B, Vol. 92, Issue 3, p. 403-408
Development of Atmospheric Tracer Methods To Measure Methane Emissions from Natural Gas Facilities and Urban Areas
journal, June 1995
- Lamb, Brian K.; McManus, J. B.; Shorter, Joanne H.
- Environmental Science & Technology, Vol. 29, Issue 6
Methane Emissions from Natural Gas Compressor Stations in the Transmission and Storage Sector: Measurements and Comparisons with the EPA Greenhouse Gas Reporting Program Protocol
journal, February 2015
- Subramanian, R.; Williams, Laurie L.; Vaughn, Timothy L.
- Environmental Science & Technology, Vol. 49, Issue 5
Industrial Flare Performance at Low Flow Conditions. 1. Study Overview
journal, March 2012
- Torres, Vincent M.; Herndon, Scott; Kodesh, Zach
- Industrial & Engineering Chemistry Research, Vol. 51, Issue 39
Direct Measurements Show Decreasing Methane Emissions from Natural Gas Local Distribution Systems in the United States
journal, March 2015
- Lamb, Brian K.; Edburg, Steven L.; Ferrara, Thomas W.
- Environmental Science & Technology, Vol. 49, Issue 8
Atmospheric trace gas measurements using a dual quantum-cascade laser mid-infrared absorption spectrometer
conference, April 2005
- Jimenez, Rodrigo; Herndon, Scott; Shorter, Joanne H.
- Integrated Optoelectronic Devices 2005, SPIE Proceedings
Measurements of Methane Emissions from Natural Gas Gathering Facilities and Processing Plants: Measurement Results
journal, February 2015
- Mitchell, Austin L.; Tkacik, Daniel S.; Roscioli, Joseph R.
- Environmental Science & Technology, Vol. 49, Issue 5
Amine Scrubbing for CO2 Capture
journal, September 2009
- Rochelle, G. T.
- Science, Vol. 325, Issue 5948
Methane emissions estimate from airborne measurements over a western United States natural gas field: CH
journal, August 2013
- Karion, Anna; Sweeney, Colm; Pétron, Gabrielle
- Geophysical Research Letters, Vol. 40, Issue 16
Methane Emissions at Nine Landfill Sites in the Northeastern United States
journal, June 1999
- Mosher, Byard W.; Czepiel, Peter M.; Harriss, Robert C.
- Environmental Science & Technology, Vol. 33, Issue 12
Measurements of methane emissions at natural gas production sites in the United States
journal, September 2013
- Allen, D. T.; Torres, V. M.; Thomas, J.
- Proceedings of the National Academy of Sciences, Vol. 110, Issue 44
Reply to comment on “Hydrocarbon emissions characterization in the Colorado Front Range-A pilot study” by Michael A. Levi: PéTRON ET AL.
journal, January 2013
- Pétron, Gabrielle; Frost, Gregory J.; Trainer, Michael K.
- Journal of Geophysical Research: Atmospheres, Vol. 118, Issue 1
Correlation of Natural Gases with Their Sources
book, January 1994
- Whiticar, Michael J.
- The Petroleum System—From Source to Trap
Works referencing / citing this record:
Atmospheric Implications of Large C 2 ‐C 5 Alkane Emissions From the U.S. Oil and Gas Industry
journal, January 2019
- Tzompa‐Sosa, Z. A.; Henderson, B. H.; Keller, C. A.
- Journal of Geophysical Research: Atmospheres, Vol. 124, Issue 2
Characterization of methane emissions from five cold heavy oil production with sands (CHOPS) facilities
journal, May 2018
- Roscioli, Joseph R.; Herndon, Scott C.; Yacovitch, Tara I.
- Journal of the Air & Waste Management Association, Vol. 68, Issue 7
A review of close-range and screening technologies for mitigating fugitive methane emissions in upstream oil and gas
journal, April 2019
- Fox, Thomas A.; Barchyn, Thomas E.; Risk, David
- Environmental Research Letters, Vol. 14, Issue 5
Exploring the endocrine activity of air pollutants associated with unconventional oil and gas extraction
journal, March 2018
- Bolden, Ashley L.; Schultz, Kim; Pelch, Katherine E.
- Environmental Health, Vol. 17, Issue 1
A Near-Field Gaussian Plume Inversion Flux Quantification Method, Applied to Unmanned Aerial Vehicle Sampling
journal, July 2019
- Shah, Adil; Allen, Grant; Pitt, Joseph R.
- Atmosphere, Vol. 10, Issue 7
Constraining sector-specific CO 2 and CH 4 emissions in the US
journal, January 2017
- Miller, Scot M.; Michalak, Anna M.
- Atmospheric Chemistry and Physics, Vol. 17, Issue 6
Quantifying uncertainties from mobile-laboratory-derived emissions of well pads using inverse Gaussian methods
journal, January 2018
- Caulton, Dana R.; Li, Qi; Bou-Zeid, Elie
- Atmospheric Chemistry and Physics, Vol. 18, Issue 20
Methane and ethane emission scenarios for potential shale gas production in Europe
journal, January 2018
- Visschedijk, Antoon J. H.; Denier van der Gon, Hugo A. C.; Doornenbal, Hans C.
- Advances in Geosciences, Vol. 45
Using the tracer flux ratio method with flight measurements to estimate dairy farm CH4 emissions in central California
journal, January 2019
- Daube, Conner; Conley, Stephen; Faloona, Ian C.
- Atmospheric Measurement Techniques, Vol. 12, Issue 4
Constraining the accuracy of flux estimates using OTM 33A
journal, January 2020
- Edie, Rachel; Robertson, Anna M.; Field, Robert A.
- Atmospheric Measurement Techniques, Vol. 13, Issue 1
Characterization of methane emissions from five cold heavy oil production with sands (CHOPS) facilities
text, January 2018
- Roscioli, Joseph R.; Herndon, Scott C.; Yacovitch, Tara I.
- Taylor & Francis
Exploring the endocrine activity of air pollutants associated with unconventional oil and gas extraction
journal, March 2018
- Bolden, Ashley L.; Schultz, Kim; Pelch, Katherine E.
- Environmental Health, Vol. 17, Issue 1
Comparing facility-level methane emission rate estimates at natural gas gathering and boosting stations
journal, February 2017
- Vaughn, Timothy L.; Bell, Clay S.; Yacovitch, Tara I.
- Elem Sci Anth, Vol. 5, Issue 0
Comparison of methane emission estimates from multiple measurement techniques at natural gas production pads
journal, February 2017
- Bell, Clay Samuel; Vaughn, Timothy L.; Zimmerle, Daniel
- Elem Sci Anth, Vol. 5, Issue 0