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Title: Incommensurate to commensurate antiferromagnetism in CeRhAl 4 Si 2 : An Al 27 NMR study

27Al nuclear magnetic resonance (NMR) experiments have been performed on a single crystal of CeRhAl 4Si 2, which is an antiferromagnetic Kondo-lattice compound with successive antiferromagnetic transitions of T N1 = 14 K and T N2 = 9 K at zero external field. In the paramagnetic state, the Knight shifts, quadrupolar frequency, and asymmetric parameter of electrical field gradient on the Al sites have been determined, which have local orthorhombic symmetry. The transferred hyperfine coupling constants are also determined. Here, analysis of the NMR spectra indicates that a commensurate antiferromagnetic structure exists below T N2, but an incommensurate modulation of antiferromagnetic moments is present in the antiferromagnetic state between T N1 and T N2. The spin-lattice relaxation rate suggests that the 4f electrons behave as local moments at temperatures above T N1.
Authors:
 [1] ;  [1] ;  [1] ;  [1] ;  [2] ; ORCiD logo [2] ; ORCiD logo [2] ; ORCiD logo [2]
  1. Japan Atomic Energy Agency (JAEA), Tokai (Japan). Advanced Science Research Center
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Publication Date:
Report Number(s):
LA-UR-17-22948
Journal ID: ISSN 2469-9950; PRBMDO
Grant/Contract Number:
AC52-06NA25396
Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 93; Journal Issue: 1; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Research Org:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org:
USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22); USDOE
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; High Magnetic Field Science
OSTI Identifier:
1454995
Alternate Identifier(s):
OSTI ID: 1234136

Sakai, Hironori, Hattori, T., Tokunaga, Y., Kambe, Shin, Ghimire, N. J., Ronning, Filip, Bauer, Eric Dietzgen, and Thompson, Joe David. Incommensurate to commensurate antiferromagnetism in CeRhAl4Si2 : An Al27 NMR study. United States: N. p., Web. doi:10.1103/PhysRevB.93.014402.
Sakai, Hironori, Hattori, T., Tokunaga, Y., Kambe, Shin, Ghimire, N. J., Ronning, Filip, Bauer, Eric Dietzgen, & Thompson, Joe David. Incommensurate to commensurate antiferromagnetism in CeRhAl4Si2 : An Al27 NMR study. United States. doi:10.1103/PhysRevB.93.014402.
Sakai, Hironori, Hattori, T., Tokunaga, Y., Kambe, Shin, Ghimire, N. J., Ronning, Filip, Bauer, Eric Dietzgen, and Thompson, Joe David. 2016. "Incommensurate to commensurate antiferromagnetism in CeRhAl4Si2 : An Al27 NMR study". United States. doi:10.1103/PhysRevB.93.014402. https://www.osti.gov/servlets/purl/1454995.
@article{osti_1454995,
title = {Incommensurate to commensurate antiferromagnetism in CeRhAl4Si2 : An Al27 NMR study},
author = {Sakai, Hironori and Hattori, T. and Tokunaga, Y. and Kambe, Shin and Ghimire, N. J. and Ronning, Filip and Bauer, Eric Dietzgen and Thompson, Joe David},
abstractNote = {27Al nuclear magnetic resonance (NMR) experiments have been performed on a single crystal of CeRhAl4Si2, which is an antiferromagnetic Kondo-lattice compound with successive antiferromagnetic transitions of TN1 = 14 K and TN2 = 9 K at zero external field. In the paramagnetic state, the Knight shifts, quadrupolar frequency, and asymmetric parameter of electrical field gradient on the Al sites have been determined, which have local orthorhombic symmetry. The transferred hyperfine coupling constants are also determined. Here, analysis of the NMR spectra indicates that a commensurate antiferromagnetic structure exists below TN2, but an incommensurate modulation of antiferromagnetic moments is present in the antiferromagnetic state between TN1 and TN2. The spin-lattice relaxation rate suggests that the 4f electrons behave as local moments at temperatures above TN1.},
doi = {10.1103/PhysRevB.93.014402},
journal = {Physical Review B},
number = 1,
volume = 93,
place = {United States},
year = {2016},
month = {1}
}

Works referenced in this record:

Generalized Gradient Approximation Made Simple
journal, October 1996
  • Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
  • Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
  • DOI: 10.1103/PhysRevLett.77.3865