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Title: Transition of Femtosecond-Filament-Solid Interactions from Single to Multiple Filament Regime

Abstract

High-peak-power fs-laser filaments offer unique characteristics attractive to remote sensing via techniques such as remote laser-induced breakdown spectroscopy (R-LIBS). The dynamics of several ablation mechanisms following the interaction between a filament and a solid determines the emission strength and reproducibility of target plasma, which is of relevance for R-LIBS applications. Here, we investigate the space- and time-resolved dynamics of ionic and atomic emission from copper as well as the surrounding atmosphere in order to understand limitations of fs-filament-ablation for standoff energy delivery. Furthermore, we probe the shock front produced from filament-target interaction using time-resolved shadowgraphy and infer laser-material coupling efficiencies for both single and multiple filament regimes through analysis of shock expansion with the Sedov model for point detonation. The results provide insight into plasma structure for the range of peak powers up to 30 times the critical power for filamentation Pcr. Despite the stochastic nucleation of multiple filaments at peak-powers greater than 16 Pcr, emission of ionic and neutral species increases with pump beam intensity, and short-lived nitrogen emission originating from the ambient is consistently observed. Ultimately, results suggest favorable scaling of emission intensity from target species on the laser pump energy, furthering the prospects for use of filament-solidmore » interactions for remote sensing.« less

Authors:
 [1];  [1];  [1]
+ Show Author Affiliations
  1. Univ. of Michigan, Ann Arbor, MI (United States). Dept. of Nuclear Engineering and Radiological Sciences; Univ. of Michigan, Ann Arbor, MI (United States). Center for Ultrafast Optical Science
Publication Date:
Research Org.:
Univ. of Michigan, Ann Arbor, MI (United States)
Sponsoring Org.:
USDOE NA Office of Nonproliferation and Verification Research and Development (NA-22); USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1454792
Grant/Contract Number:  
NA0002534
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 7; Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
42 ENGINEERING

Citation Formats

Skrodzki, P. J., Burger, M., and Jovanovic, I. Transition of Femtosecond-Filament-Solid Interactions from Single to Multiple Filament Regime. United States: N. p., 2017. Web. doi:10.1038/s41598-017-13188-4.
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Skrodzki, P. J., Burger, M., & Jovanovic, I. Transition of Femtosecond-Filament-Solid Interactions from Single to Multiple Filament Regime. United States. doi:https://doi.org/10.1038/s41598-017-13188-4
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Skrodzki, P. J., Burger, M., and Jovanovic, I. Fri . "Transition of Femtosecond-Filament-Solid Interactions from Single to Multiple Filament Regime". United States. doi:https://doi.org/10.1038/s41598-017-13188-4. https://www.osti.gov/servlets/purl/1454792.
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@article{osti_1454792,
title = {Transition of Femtosecond-Filament-Solid Interactions from Single to Multiple Filament Regime},
author = {Skrodzki, P. J. and Burger, M. and Jovanovic, I.},
abstractNote = {High-peak-power fs-laser filaments offer unique characteristics attractive to remote sensing via techniques such as remote laser-induced breakdown spectroscopy (R-LIBS). The dynamics of several ablation mechanisms following the interaction between a filament and a solid determines the emission strength and reproducibility of target plasma, which is of relevance for R-LIBS applications. Here, we investigate the space- and time-resolved dynamics of ionic and atomic emission from copper as well as the surrounding atmosphere in order to understand limitations of fs-filament-ablation for standoff energy delivery. Furthermore, we probe the shock front produced from filament-target interaction using time-resolved shadowgraphy and infer laser-material coupling efficiencies for both single and multiple filament regimes through analysis of shock expansion with the Sedov model for point detonation. The results provide insight into plasma structure for the range of peak powers up to 30 times the critical power for filamentation Pcr. Despite the stochastic nucleation of multiple filaments at peak-powers greater than 16 Pcr, emission of ionic and neutral species increases with pump beam intensity, and short-lived nitrogen emission originating from the ambient is consistently observed. Ultimately, results suggest favorable scaling of emission intensity from target species on the laser pump energy, furthering the prospects for use of filament-solid interactions for remote sensing.},
doi = {10.1038/s41598-017-13188-4},
journal = {Scientific Reports},
number = 1,
volume = 7,
place = {United States},
year = {2017},
month = {10}
}
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DOI:  https://doi.org/10.1038/s41598-017-13188-4
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Cited by: 4 works
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Figures / Tables:

Figure 1 Figure 1: Initial detonation energy obtained from the predictive Sedov model. Focusing using an ordinary lens, resulting in random filament distribution in the multiple filament regime, is compared to focusing using a split lens, allowing induced multiple filament formation.
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Works referenced in this record:

Reflectivity of metals at high temperatures heated by pulsed laser
journal, May 1977

Stand-off filament-induced ablation of gallium arsenide
journal, July 2012

  • Weidman, Matthew; Lim, Khan; Ramme, Mark
  • Applied Physics Letters, Vol. 101, Issue 3
  • DOI: 10.1063/1.4734497

Understanding the advantage of remote femtosecond laser-induced breakdown spectroscopy of metallic targets
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  • Xu, H. L.; Bernhardt, J.; Mathieu, P.
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Shock wave and material vapour plume propagation during excimer laser ablation of aluminium samples
journal, September 1999

Experiment and simulations on the energy reservoir effect in femtosecond light filaments
journal, January 2005

Effect of laser parameters on laser ablation and laser-induced plasma formation: A numerical modeling investigation
journal, October 2005

  • Bogaerts, Annemie; Chen, Zhaoyang
  • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 60, Issue 9-10
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The White Light Supercontinuum Is Indeed an Ultrafast White Light Laser
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  • Japanese Journal of Applied Physics, Vol. 38, Issue Part 2, No. 2A
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Re-evaluation of the W value for electrons in dry air
journal, February 1987

Characterization of laser ablation sample introduction plasma plumes in fs-LA-ICP-MS
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White-Light Filaments for Atmospheric Analysis
journal, July 2003

Anomalous long-range propagation of femtosecond laser pulses through air:?moving focus or pulse self-guiding?
journal, January 1998

  • Lange, H. R.; Grillon, G.; Ripoche, J. -F.
  • Optics Letters, Vol. 23, Issue 2
  • DOI: 10.1364/OL.23.000120

Organizing Multiple Femtosecond Filaments in Air
journal, July 2004

Backward growth of plasma induced by long nanosecond laser pulse ablation
journal, August 2011

  • Zhou, Yun; Tao, Sha; Wu, Benxin
  • Applied Physics Letters, Vol. 99, Issue 5
  • DOI: 10.1063/1.3621855

Coulomb explosion in ultrashort pulsed laser ablation of Al 2 O 3
journal, November 2000

Spherical expansion of the vapor plume into ambient gas: an analytical model
journal, December 1999

  • Arnold, N.; Gruber, J.; Heitz, J.
  • Applied Physics A Materials Science & Processing, Vol. 69, Issue S1
  • DOI: 10.1007/s003399900183

Remote LIBS with ultrashort pulses: characteristics in picosecond and femtosecond regimes
journal, January 2004

  • Rohwetter, Ph.; Yu, J.; Méjean, G.
  • J. Anal. At. Spectrom., Vol. 19, Issue 4
  • DOI: 10.1039/b316343a

Phase explosion in atmospheric pressure infrared laser ablation from water-rich targets
journal, July 2006

  • Chen, Zhaoyang; Bogaerts, Annemie; Vertes, Akos
  • Applied Physics Letters, Vol. 89, Issue 4
  • DOI: 10.1063/1.2243961

Interaction of a single laser filament with a single water droplet
journal, April 2015

Filament-induced remote surface ablation for long range laser-induced breakdown spectroscopy operation
journal, August 2005

  • Rohwetter, Ph.; Stelmaszczyk, K.; Wöste, L.
  • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 60, Issue 7-8
  • DOI: 10.1016/j.sab.2005.03.017

Time-Resolved Shadowgraphs of Material Ejection in Intense Femtosecond Laser Ablation of Aluminum
journal, October 2007

The critical laser intensity of self-guided light filaments in air
journal, December 2000

  • Kasparian, J.; Sauerbrey, R.; Chin, S. L.
  • Applied Physics B, Vol. 71, Issue 6
  • DOI: 10.1007/s003400000463

Efficient non-gated remote filament-induced breakdown spectroscopy of metallic sample
journal, January 2007

  • Liu, W.; Xu, H. L.; Méjean, G.
  • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 62, Issue 1
  • DOI: 10.1016/j.sab.2007.01.001

Laser ablation of copper in different background gases: comparative study by numerical modeling and experiments
journal, January 2006

  • Bogaerts, Annemie; Chen, Zhaoyang; Bleiner, Davide
  • Journal of Analytical Atomic Spectrometry, Vol. 21, Issue 4
  • DOI: 10.1039/b514313f

Non-linear effects accompanying terawatt laser-pulse in air and their applications
conference, February 2012

  • Stelmaszczyk, Kamil; Rohwetter, Philipp; Ackermann, Roland
  • SPIE Proceedings
  • DOI: 10.1117/12.675772

Laser-Induced Breakdown Spectroscopy in open-path configuration for the analysis of distant objects
journal, August 2007

  • Sallé, B.; Mauchien, P.; Maurice, S.
  • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 62, Issue 8
  • DOI: 10.1016/j.sab.2007.07.001

Efficient second- and third-harmonic radiation generation from relativistic laser-plasma interactions
journal, June 2015

  • Singh, Mamta; Gupta, D. N.; Suk, H.
  • Physics of Plasmas, Vol. 22, Issue 6
  • DOI: 10.1063/1.4922435

Standoff Detection of Uranium and its Isotopes by Femtosecond Filament Laser Ablation Molecular Isotopic Spectrometry
journal, March 2017

  • Hartig, Kyle C.; Ghebregziabher, Isaac; Jovanovic, Igor
  • Scientific Reports, Vol. 7, Issue 1
  • DOI: 10.1038/srep43852

Comparison between geometrically focused pulses versus filaments in femtosecond laser ablation of steel and titanium alloys
journal, December 2013

Laser ablation for analytical sampling: what can we learn from modeling?
journal, November 2003

  • Bogaerts, Annemie; Chen, Zhaoyang; Gijbels, Renaat
  • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 58, Issue 11
  • DOI: 10.1016/j.sab.2003.08.004

Femtosecond pulsed laser ablation dynamics and ablation morphology of nickel based superalloy CMSX-4
journal, May 2008

  • McDonald, Joel P.; Ma, Shuwei; Pollock, Tresa M.
  • Journal of Applied Physics, Vol. 103, Issue 9
  • DOI: 10.1063/1.2917418

Effect of beam diameter on the propagation of intense femtosecond laser pulses
journal, January 2005

Femtosecond laser ablation of copper at high laser fluence: Modeling and experimental comparison
journal, January 2016

Multiple Filamentation of Terawatt Laser Pulses in Air
journal, June 2004

Ultrashort pulse laser ablation of dielectrics: Thresholds, mechanisms, role of breakdown
journal, December 2016

  • Mirza, Inam; Bulgakova, Nadezhda M.; Tomáštík, Jan
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep39133

Role of spectroscopic diagnostics in studying nanosecond laser-plasma interaction
journal, May 2017

Ultraintense light filaments transmitted through clouds
journal, July 2003

  • Courvoisier, François; Boutou, Véronique; Kasparian, Jérôme
  • Applied Physics Letters, Vol. 83, Issue 2
  • DOI: 10.1063/1.1592615

Formation of a conducting channel in air by self-guided femtosecond laser pulses
journal, October 1999

Longitudinal compression of short laser pulses in air
journal, May 2004

  • Alexeev, I.; Ting, A.; Gordon, D. F.
  • Applied Physics Letters, Vol. 84, Issue 20
  • DOI: 10.1063/1.1753051

Self-channeling of high-peak-power femtosecond laser pulses in air
journal, January 1995

Time Resolved Shadowgraph Images of Silicon during Laser Ablation: Shockwaves and Particle Generation
journal, April 2007

Filament-induced breakdown remote spectroscopy in a polar environment
journal, November 2012

Propagation of intense short laser pulses in the atmosphere
journal, October 2002

Femtosecond Laser Filamentation for Atmospheric Sensing
journal, December 2010

Plasma temperature clamping in filamentation laser induced breakdown spectroscopy
journal, January 2015

  • Harilal, S. S.; Yeak, J.; Phillips, M. C.
  • Optics Express, Vol. 23, Issue 21
  • DOI: 10.1364/OE.23.027113

Propagation distance-resolved characteristics of filament-induced copper plasma
journal, January 2016

  • Ghebregziabher, Isaac; Hartig, Kyle C.; Jovanovic, Igor
  • Optics Express, Vol. 24, Issue 5
  • DOI: 10.1364/OE.24.005263
    [ × clear filter / sort ]

    Works referencing / citing this record:

    Spherical expansion of the vapor plume into ambient gas: an analytical model
    journal, December 1999

    • Arnold, N.; Gruber, J.; Heitz, J.
    • Applied Physics A Materials Science & Processing, Vol. 69, Issue S1
    • DOI: 10.1007/s003399900183

    Effect of beam diameter on the propagation of intense femtosecond laser pulses
    journal, January 2005

    Comparison between geometrically focused pulses versus filaments in femtosecond laser ablation of steel and titanium alloys
    journal, December 2013

    The critical laser intensity of self-guided light filaments in air
    journal, December 2000

    • Kasparian, J.; Sauerbrey, R.; Chin, S. L.
    • Applied Physics B, Vol. 71, Issue 6
    • DOI: 10.1007/s003400000463

    Reflectivity of metals at high temperatures heated by pulsed laser
    journal, May 1977

    Femtosecond laser ablation of copper at high laser fluence: Modeling and experimental comparison
    journal, January 2016

    Laser ablation for analytical sampling: what can we learn from modeling?
    journal, November 2003

    • Bogaerts, Annemie; Chen, Zhaoyang; Gijbels, Renaat
    • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 58, Issue 11
    • DOI: 10.1016/j.sab.2003.08.004

    Filament-induced remote surface ablation for long range laser-induced breakdown spectroscopy operation
    journal, August 2005

    • Rohwetter, Ph.; Stelmaszczyk, K.; Wöste, L.
    • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 60, Issue 7-8
    • DOI: 10.1016/j.sab.2005.03.017

    Effect of laser parameters on laser ablation and laser-induced plasma formation: A numerical modeling investigation
    journal, October 2005

    • Bogaerts, Annemie; Chen, Zhaoyang
    • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 60, Issue 9-10
    • DOI: 10.1016/j.sab.2005.06.009

    Efficient non-gated remote filament-induced breakdown spectroscopy of metallic sample
    journal, January 2007

    • Liu, W.; Xu, H. L.; Méjean, G.
    • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 62, Issue 1
    • DOI: 10.1016/j.sab.2007.01.001

    Laser-Induced Breakdown Spectroscopy in open-path configuration for the analysis of distant objects
    journal, August 2007

    • Sallé, B.; Mauchien, P.; Maurice, S.
    • Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 62, Issue 8
    • DOI: 10.1016/j.sab.2007.07.001

    Ultrashort pulse laser ablation of dielectrics: Thresholds, mechanisms, role of breakdown
    journal, December 2016

    • Mirza, Inam; Bulgakova, Nadezhda M.; Tomáštík, Jan
    • Scientific Reports, Vol. 6, Issue 1
    • DOI: 10.1038/srep39133

    Standoff Detection of Uranium and its Isotopes by Femtosecond Filament Laser Ablation Molecular Isotopic Spectrometry
    journal, March 2017

    • Hartig, Kyle C.; Ghebregziabher, Isaac; Jovanovic, Igor
    • Scientific Reports, Vol. 7, Issue 1
    • DOI: 10.1038/srep43852

    Remote LIBS with ultrashort pulses: characteristics in picosecond and femtosecond regimes
    journal, January 2004

    • Rohwetter, Ph.; Yu, J.; Méjean, G.
    • J. Anal. At. Spectrom., Vol. 19, Issue 4
    • DOI: 10.1039/b316343a

    Laser ablation of copper in different background gases: comparative study by numerical modeling and experiments
    journal, January 2006

    • Bogaerts, Annemie; Chen, Zhaoyang; Bleiner, Davide
    • Journal of Analytical Atomic Spectrometry, Vol. 21, Issue 4
    • DOI: 10.1039/b514313f

    Characterization of laser ablation sample introduction plasma plumes in fs-LA-ICP-MS
    journal, January 2014

    • LaHaye, N. L.; Harilal, S. S.; Diwakar, P. K.
    • J. Anal. At. Spectrom., Vol. 29, Issue 12
    • DOI: 10.1039/c4ja00200h

    Ultraintense light filaments transmitted through clouds
    journal, July 2003

    • Courvoisier, François; Boutou, Véronique; Kasparian, Jérôme
    • Applied Physics Letters, Vol. 83, Issue 2
    • DOI: 10.1063/1.1592615

    Longitudinal compression of short laser pulses in air
    journal, May 2004

    • Alexeev, I.; Ting, A.; Gordon, D. F.
    • Applied Physics Letters, Vol. 84, Issue 20
    • DOI: 10.1063/1.1753051

    Phase explosion in atmospheric pressure infrared laser ablation from water-rich targets
    journal, July 2006

    • Chen, Zhaoyang; Bogaerts, Annemie; Vertes, Akos
    • Applied Physics Letters, Vol. 89, Issue 4
    • DOI: 10.1063/1.2243961

    Understanding the advantage of remote femtosecond laser-induced breakdown spectroscopy of metallic targets
    journal, February 2007

    • Xu, H. L.; Bernhardt, J.; Mathieu, P.
    • Journal of Applied Physics, Vol. 101, Issue 3
    • DOI: 10.1063/1.2437580

    Femtosecond pulsed laser ablation dynamics and ablation morphology of nickel based superalloy CMSX-4
    journal, May 2008

    • McDonald, Joel P.; Ma, Shuwei; Pollock, Tresa M.
    • Journal of Applied Physics, Vol. 103, Issue 9
    • DOI: 10.1063/1.2917418

    Backward growth of plasma induced by long nanosecond laser pulse ablation
    journal, August 2011

    • Zhou, Yun; Tao, Sha; Wu, Benxin
    • Applied Physics Letters, Vol. 99, Issue 5
    • DOI: 10.1063/1.3621855

    Stand-off filament-induced ablation of gallium arsenide
    journal, July 2012

    • Weidman, Matthew; Lim, Khan; Ramme, Mark
    • Applied Physics Letters, Vol. 101, Issue 3
    • DOI: 10.1063/1.4734497

    Efficient second- and third-harmonic radiation generation from relativistic laser-plasma interactions
    journal, June 2015

    • Singh, Mamta; Gupta, D. N.; Suk, H.
    • Physics of Plasmas, Vol. 22, Issue 6
    • DOI: 10.1063/1.4922435

    Shock wave and material vapour plume propagation during excimer laser ablation of aluminium samples
    journal, September 1999

    Re-evaluation of the W value for electrons in dry air
    journal, February 1987

    Time Resolved Shadowgraph Images of Silicon during Laser Ablation: Shockwaves and Particle Generation
    journal, April 2007

    Interaction of a single laser filament with a single water droplet
    journal, April 2015

    Coulomb explosion in ultrashort pulsed laser ablation of Al 2 O 3
    journal, November 2000

    Formation of a conducting channel in air by self-guided femtosecond laser pulses
    journal, October 1999

    Propagation of intense short laser pulses in the atmosphere
    journal, October 2002

    Multiple Filamentation of Terawatt Laser Pulses in Air
    journal, June 2004

    Organizing Multiple Femtosecond Filaments in Air
    journal, July 2004

    Time-Resolved Shadowgraphs of Material Ejection in Intense Femtosecond Laser Ablation of Aluminum
    journal, October 2007

    Non-linear effects accompanying terawatt laser-pulse in air and their applications
    conference, February 2012

    • Stelmaszczyk, Kamil; Rohwetter, Philipp; Ackermann, Roland
    • SPIE Proceedings
    • DOI: 10.1117/12.675772

    White-Light Filaments for Atmospheric Analysis
    journal, July 2003

    Filament-induced breakdown remote spectroscopy in a polar environment
    journal, November 2012

    Role of spectroscopic diagnostics in studying nanosecond laser-plasma interaction
    journal, May 2017

    The White Light Supercontinuum Is Indeed an Ultrafast White Light Laser
    journal, February 1999

    • Chin, See Leang; Petit, Stéphane; Borne, Frédéric
    • Japanese Journal of Applied Physics, Vol. 38, Issue Part 2, No. 2A
    • DOI: 10.1143/jjap.38.l126

    Plasma temperature clamping in filamentation laser induced breakdown spectroscopy
    journal, January 2015

    • Harilal, S. S.; Yeak, J.; Phillips, M. C.
    • Optics Express, Vol. 23, Issue 21
    • DOI: 10.1364/oe.23.027113

    Propagation distance-resolved characteristics of filament-induced copper plasma
    journal, January 2016

    • Ghebregziabher, Isaac; Hartig, Kyle C.; Jovanovic, Igor
    • Optics Express, Vol. 24, Issue 5
    • DOI: 10.1364/oe.24.005263

    Self-channeling of high-peak-power femtosecond laser pulses in air
    journal, January 1995

    Anomalous long-range propagation of femtosecond laser pulses through air:?moving focus or pulse self-guiding?
    journal, January 1998

    • Lange, H. R.; Grillon, G.; Ripoche, J. -F.
    • Optics Letters, Vol. 23, Issue 2
    • DOI: 10.1364/ol.23.000120

    Experiment and simulations on the energy reservoir effect in femtosecond light filaments
    journal, January 2005

    Femtosecond Laser Filamentation for Atmospheric Sensing
    journal, December 2010

    Ultrafast dynamics observation during femtosecond laser-material interaction
    journal, September 2019

    • Guo, Baoshan; Sun, Jingya; Lu, YongFeng
    • International Journal of Extreme Manufacturing, Vol. 1, Issue 3
    • DOI: 10.1088/2631-7990/ab3a24

    Optical emission from ultrafast laser filament-produced air plasmas in the multiple filament regime
    journal, January 2018

    • Finney, L. A.; Skrodzki, P. J.; Burger, M.
    • Optics Express, Vol. 26, Issue 22
    • DOI: 10.1364/oe.26.029110

    Electrical conductance of near-infrared femtosecond air filaments in the multi-filament regime
    journal, January 2018

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