Engineered Transport in Microporous Materials and Membranes for Clean Energy Technologies

Li, Changyi; Meckler, Stephen M.; Smith, Zachary P.; Bachman, Jonathan E.; Maserati, Lorenzo; Long, Jeffrey R.; Helms, Brett A.

doi:10.1002/adma.201704953

Title: Engineered Transport in Microporous Materials and Membranes for Clean Energy Technologies

Journal Article · 08 January 2018 · Advanced Materials

DOI: https://doi.org/10.1002/adma.201704953 · OSTI ID:1454496

Li, Changyi ^[1]; Meckler, Stephen M. ^[2]; Smith, Zachary P. ^[3]; Bachman, Jonathan E. ^[1]; Maserati, Lorenzo ^[4]; Long, Jeffrey R. ^[5];

^[6]

Univ. of California, Berkeley, CA (United States). Dept. of Chemical and Biomolecular Engineering
Univ. of California, Berkeley, CA (United States). Dept. of Chemistry
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Chemical Engineering
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
Univ. of California, Berkeley, CA (United States). Dept. of Chemical and Biomolecular Engineering and Dept. of Chemistry; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division and Molecular Foundry

Many forward-looking clean-energy technologies hinge on the development of scalable and efficient membrane-based separations. Ongoing investment in the basic research of microporous materials is beginning to pay dividends in membrane technology maturation. Specifically, improvements in membrane selectivity, permeability, and durability are being leveraged for more efficient carbon capture, desalination, and energy storage, and the market adoption of membranes in those areas appears to be on the horizon. Herein, an overview of the microporous materials chemistry driving advanced membrane development, the clean-energy separations employing them, and the theoretical underpinnings tying membrane performance to membrane structure across multiple length scales is provided. The interplay of pore architecture and chemistry for a given set of analytes emerges as a critical design consideration dictating mass transport outcomes. Also discussed are opportunities and outstanding challenges in the field, including high-flux 2D molecular-sieving membranes, phase-change adsorbents as performance-enhancing components in composite membranes, and the need for quantitative metrologies for understanding mass transport in heterophasic materials and in micropores with unusual chemical interactions with analytes of interest.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Center for Gas Separations Relevant to Clean Energy Technologies (CGS); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-05CH11231; SC0001015

OSTI ID:: 1454496

Alternate ID(s):: OSTI ID: 1416396

Journal Information:: Advanced Materials, Vol. 30, Issue 8; Related Information: © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 81 works

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