Traces of charge density waves in NbS2

Leroux, Maxime; Cario, Laurent; Bosak, Alexei; Rodiere, Pierre

doi:10.1103/PhysRevB.97.195140

Title: Traces of charge density waves in ${NbS}_{2}$

Abstract

Among transition metal dichalcogenides (TMD), NbS₂ is often considered as the archetypal compound that does not have a charge density wave (CDW) in any of its polytypes. By comparison, close isoelectronic compounds such as NbSe₂, TaS₂, and TaSe₂ all have CDW in at least one polytype. Here we report traces of CDW in the 2H polytype of NbS₂, using diffuse x-ray scattering measurements at 77 K and room temperature. We observe 12 extremely weak satellite peaks located at ±13.9° from ^→a* and ^→b* around each Bragg peak in the (h,k,0) plane. These satellite peaks are commensurate with the lattice via 3^→q–^→q'=^→a*, where ^→q' is the 120° rotation of ^→q, and define two √13a × √13a superlattices in real space. These commensurate wave vectors and tilt angle are identical to those of the CDW observed in the 1T polytype of TaS₂ and TaSe₂. In conclusion, to understand this similarity and the faintness of the peaks, we discuss possible sources of local 1T polytype environment in bulk 2H-NbS₂ crystals.

Authors:

^[1]; Cario, Laurent ^[2]; Bosak, Alexei ^[3]; Rodiere, Pierre ^[4]

Univ. Grenoble Alpes, Grenoble (France); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Institut des Materiaux de Nantes, Nantes (France)
The European Synchrotron, Grenoble (France)
Univ. Grenoble Alpes, Grenoble (France)

Publication Date:: Tue May 15 00:00:00 EDT 2018

Research Org.:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Org.:: Universities/Institutions; USDOE

OSTI Identifier:: 1440495

Report Number(s):: LA-UR-18-20468
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1900755

Grant/Contract Number:: AC52-06NA25396

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 97; Journal Issue: 19; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; Material Science

Citation Formats


                    Leroux, Maxime, Cario, Laurent, Bosak, Alexei, and Rodiere, Pierre. Traces of charge density waves in NbS2.  United States: N. p., 2018. 
Web.  doi:10.1103/PhysRevB.97.195140.

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                    Leroux, Maxime, Cario, Laurent, Bosak, Alexei, & Rodiere, Pierre. Traces of charge density waves in NbS2.  United States.  https://doi.org/10.1103/PhysRevB.97.195140

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                    Leroux, Maxime, Cario, Laurent, Bosak, Alexei, and Rodiere, Pierre. Tue .  
"Traces of charge density waves in NbS2".  United States.  https://doi.org/10.1103/PhysRevB.97.195140.  https://www.osti.gov/servlets/purl/1440495.

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@article{osti_1440495,

  title        = {Traces of charge density waves in NbS2},

  author       = {Leroux, Maxime and Cario, Laurent and Bosak, Alexei and Rodiere, Pierre},

  abstractNote = {Among transition metal dichalcogenides (TMD), NbS2 is often considered as the archetypal compound that does not have a charge density wave (CDW) in any of its polytypes. By comparison, close isoelectronic compounds such as NbSe2, TaS2, and TaSe2 all have CDW in at least one polytype. Here we report traces of CDW in the 2H polytype of NbS2, using diffuse x-ray scattering measurements at 77 K and room temperature. We observe 12 extremely weak satellite peaks located at ±13.9° from →a* and →b* around each Bragg peak in the (h,k,0) plane. These satellite peaks are commensurate with the lattice via 3→q–→q'=→a*, where →q' is the 120° rotation of →q, and define two √13a × √13a superlattices in real space. These commensurate wave vectors and tilt angle are identical to those of the CDW observed in the 1T polytype of TaS2 and TaSe2. In conclusion, to understand this similarity and the faintness of the peaks, we discuss possible sources of local 1T polytype environment in bulk 2H-NbS2 crystals.},

  doi          = {10.1103/PhysRevB.97.195140},

  journal      = {Physical Review B},

  number       = 19,

  volume       = 97,

  place        = {United States},

  year         = {Tue May 15 00:00:00 EDT 2018},

  month        = {Tue May 15 00:00:00 EDT 2018}

}

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https://doi.org/10.1103/PhysRevB.97.195140

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Cited by: 27 works

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FIG. 1: Cristallographic structures of the three known polytypes of NbS₂: 1T reported only in thin film⁷ or monolayer form⁸, and 2H and 3R found in bulk crystals form⁹. In the 1T polytype, the transition metal atom is in octahedral coordination and layers are stacked without rotation or in-plane translation.more »

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Works referenced in this record:

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Works referencing / citing this record:

Optical Properties of 2D 3R Phase Niobium Disulfide and Its Applications as a Saturable Absorber
journal, December 2019

Sun, Xiaoli; Shi, Bingnan; Wang, Haoyuan
Advanced Optical Materials, Vol. 8, Issue 4
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Niobium disulphide (NbS ₂ )-based (heterogeneous) electrocatalysts for an efficient hydrogen evolution reaction
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Najafi, Leyla; Bellani, Sebastiano; Oropesa-Nuñez, Reinier
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Coexistence of the Kondo effect and spin glass physics in Fe-doped NbS ₂
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Nobukane, H.; Tabata, Y.; Kurosawa, T.
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Impact ionization dynamics in small band-gap two-dimensional materials from a coherent phonon mechanism
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Michael, Stephan; Schneider, Hans Christian
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Niobium disulphide (NbS$_2$)-based (heterogeneous) electrocatalysts for an efficient hydrogen evolution reaction
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Similar Records

Title: Traces of charge density waves in NbS 2

Abstract

Citation Formats

Figures / Tables:

Studies on two-gap superconductivity in 2H–NbS2 journal, December 2010

Phase engineering of transition metal dichalcogenides journal, January 2015

Stacking disorder in 2H-NbS2 and its intercalation compounds Kx(H2O)yNbS2 I. Description and model calculations of stacking faults in the host lattice NbS2 journal, January 2002

Spin density wave instabilities in the NbS 2 monolayer journal, March 2016

Stoichiometry, structure, and physical properties of niobium disulfide journal, January 1980

In-plane magnetic penetration depth in NbS 2 journal, August 2011

Strongly enhanced charge-density-wave order in monolayer NbSe2 journal, July 2015

Electronics and optoelectronics of two-dimensional transition metal dichalcogenides journal, November 2012

Electron diffraction study of the charge-density wave superlattice in 2H-NbSe2 journal, February 1984

Origin of Superconductivity and Latent Charge Density Wave in NbS 2 journal, August 2017

Phonon spectroscopy by inelastic x-ray scattering journal, January 2000

Novel high pressure structures and superconductivity of niobium disulfide journal, October 2014

Pressure Effect on Superconducting Nb Se 2 and Nb S 2 journal, August 1972

Anisotropy of Upper Critical Field in Superconducting 2 H -NbS 2 journal, July 1978

Charge-Density Waves in Metallic, Layered, Transition-Metal Dichalcogenides journal, April 1974

Charge-density waves and superlattices in the metallic layered transition metal dichalcogenides journal, March 1975

Origin of hydrogen evolution activity on MS 2 (M = Mo or Nb) monolayers journal, January 2015

Landau theory of charge-density waves in transition-metal dichalcogenides journal, August 1975

Two-Gap Superconductivity in 2H-NbS 2 journal, November 2010

Two-dimensional layered transition-metal dichalcogenides for versatile properties and applications journal, July 2015

Crystal structure studies of the 3R-Nb1.09S2 and the 2H-NbSe2 compounds: correlation between nonstoichiometry and stacking type (= polytypism) journal, July 2001

Electronic properties of intercalation complexes of the transition metal dichalcogenides journal, January 1987

Anharmonic suppression of charge density waves in 2 H -NbS 2 journal, October 2012

Orbital textures and charge density waves in transition metal dichalcogenides journal, March 2015

Superconducting Density of States and Vortex Cores of 2H- NbS 2 journal, October 2008

Anisotropy and temperature dependence of the first critical field in 2H–NbS2 journal, June 2012

Effect of dimensionality on the charge-density wave in few-layer 2 H -NbSe 2 journal, December 2009

Electrical Transport Properties in 2 H -NbS 2 , -NbSe 2 , -TaS 2 and -TaSe 2 journal, January 1982

The role of charge density waves in structural transformations of 1T TaS 2 journal, February 1975

Extended Phonon Collapse and the Origin of the Charge-Density Wave in 2 H − NbSe 2 journal, September 2011

Optical Properties of 2D 3R Phase Niobium Disulfide and Its Applications as a Saturable Absorber journal, December 2019

Niobium disulphide (NbS 2 )-based (heterogeneous) electrocatalysts for an efficient hydrogen evolution reaction journal, January 2019

Coexistence of the Kondo effect and spin glass physics in Fe-doped NbS 2 journal, January 2020

Impact ionization dynamics in small band-gap two-dimensional materials from a coherent phonon mechanism journal, July 2019

Niobium disulphide (NbS$_2$)-based (heterogeneous) electrocatalysts for an efficient hydrogen evolution reaction text, January 2020

Title: Traces of charge density waves in ${NbS}_{2}$

Studies on two-gap superconductivity in 2H–NbS2
journal, December 2010

Phase engineering of transition metal dichalcogenides
journal, January 2015

Stacking disorder in 2H-NbS2 and its intercalation compounds Kx(H2O)yNbS2 I. Description and model calculations of stacking faults in the host lattice NbS2
journal, January 2002

Spin density wave instabilities in the ${NbS}_{2}$ monolayer
journal, March 2016

Stoichiometry, structure, and physical properties of niobium disulfide
journal, January 1980

In-plane magnetic penetration depth in NbS $_{2}$
journal, August 2011

Strongly enhanced charge-density-wave order in monolayer NbSe₂
journal, July 2015

Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
journal, November 2012

Electron diffraction study of the charge-density wave superlattice in 2H-NbSe2
journal, February 1984

Origin of Superconductivity and Latent Charge Density Wave in ${NbS}_{2}$
journal, August 2017

Phonon spectroscopy by inelastic x-ray scattering
journal, January 2000

Novel high pressure structures and superconductivity of niobium disulfide
journal, October 2014

Pressure Effect on Superconducting Nb ${Se}_{2}$ and Nb $S_{2}$
journal, August 1972

Anisotropy of Upper Critical Field in Superconducting 2 H -NbS ₂
journal, July 1978

Charge-Density Waves in Metallic, Layered, Transition-Metal Dichalcogenides
journal, April 1974

Charge-density waves and superlattices in the metallic layered transition metal dichalcogenides
journal, March 1975

Origin of hydrogen evolution activity on MS ₂ (M = Mo or Nb) monolayers
journal, January 2015

Landau theory of charge-density waves in transition-metal dichalcogenides
journal, August 1975

Two-Gap Superconductivity in 2H-NbS ₂
journal, November 2010

Two-dimensional layered transition-metal dichalcogenides for versatile properties and applications
journal, July 2015

Crystal structure studies of the 3R-Nb1.09S2 and the 2H-NbSe2 compounds: correlation between nonstoichiometry and stacking type (= polytypism)
journal, July 2001

Electronic properties of intercalation complexes of the transition metal dichalcogenides
journal, January 1987

Anharmonic suppression of charge density waves in 2 $H$ -NbS $_{2}$
journal, October 2012

Orbital textures and charge density waves in transition metal dichalcogenides
journal, March 2015

Superconducting Density of States and Vortex Cores of 2H- ${NbS}_{2}$
journal, October 2008

Anisotropy and temperature dependence of the first critical field in 2H–NbS2
journal, June 2012

Effect of dimensionality on the charge-density wave in few-layer $2 {H -NbSe}_{2}$
journal, December 2009

Electrical Transport Properties in 2 H -NbS ₂ , -NbSe ₂ , -TaS ₂ and -TaSe ₂
journal, January 1982

The role of charge density waves in structural transformations of 1T TaS ₂
journal, February 1975

Extended Phonon Collapse and the Origin of the Charge-Density Wave in $2 H − {NbSe}_{2}$
journal, September 2011

Optical Properties of 2D 3R Phase Niobium Disulfide and Its Applications as a Saturable Absorber
journal, December 2019

Niobium disulphide (NbS ₂ )-based (heterogeneous) electrocatalysts for an efficient hydrogen evolution reaction
journal, January 2019

Coexistence of the Kondo effect and spin glass physics in Fe-doped NbS ₂
journal, January 2020

Impact ionization dynamics in small band-gap two-dimensional materials from a coherent phonon mechanism
journal, July 2019

Niobium disulphide (NbS$_2$)-based (heterogeneous) electrocatalysts for an efficient hydrogen evolution reaction
text, January 2020