Progress on the Critical Parameters for Lithium-Sulfur Batteries to be Practically Viable
Abstract
Lithium–sulfur batteries have great potential to satisfy the increasing demand of energy storage systems for portable devices, electric vehicles, and grid storage because of their extremely high specific capacity, cost-effectiveness, and environmental friendliness. In spite of all these merits, the practical utilization of lithium–sulfur batteries is impeded by commonly known challenges, such as low sulfur utilization (<80%), short life (<200 cycles), fast capacity fade, and severe self-discharge effect, which mainly result from the i) low conductivity of the active material, ii) serious polysulfide shuttling, iii) large volume changes, and iv) lithium–metal anode contamination/corrosion. Numerous approaches are reported to effectively mitigate these issues. Indeed, such approaches have shown enhanced lithium–sulfur battery performances. However, many reports overlook the critical parameters, including sulfur loading (<13 mg cm-2), sulfur content (<70 wt%), and electrolyte/sulfur ratio (>11 µL mg-1), that significantly affect the analyzed electrochemical characteristics, energy density, and practicality of lithium–sulfur batteries. This review highlights the trends and progress in making cells fulfilling these fabrication parameters and discuss the challenges of the amount of sulfur and electrolyte in fabricating cells with practically necessary parameters and with high electrochemical utilization and efficiency.
- Publication Date:
- Research Org.:
- Univ. of Texas, Austin, TX (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1488314
- Alternate Identifier(s):
- OSTI ID: 1439359; OSTI ID: 1488311; OSTI ID: 1488312; OSTI ID: 1488313
- Grant/Contract Number:
- EE0007218
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Functional Materials
- Additional Journal Information:
- Journal Volume: 28; Journal Issue: 28; Journal ID: ISSN 1616-301X
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; 36 MATERIALS SCIENCE; battery testing setting; cyclability; high loading; lithium–sulfur batteries; low electrolyte; sufficient sulfur content
Citation Formats
Chung, Sheng -Heng, Chang, Chi -Hao, and Manthiram, Arumugam. Progress on the Critical Parameters for Lithium-Sulfur Batteries to be Practically Viable. United States: N. p., 2018.
Web. doi:10.1002/adfm.201801188.
Chung, Sheng -Heng, Chang, Chi -Hao, & Manthiram, Arumugam. Progress on the Critical Parameters for Lithium-Sulfur Batteries to be Practically Viable. United States. https://doi.org/10.1002/adfm.201801188
Chung, Sheng -Heng, Chang, Chi -Hao, and Manthiram, Arumugam. Tue .
"Progress on the Critical Parameters for Lithium-Sulfur Batteries to be Practically Viable". United States. https://doi.org/10.1002/adfm.201801188. https://www.osti.gov/servlets/purl/1488314.
@article{osti_1488314,
title = {Progress on the Critical Parameters for Lithium-Sulfur Batteries to be Practically Viable},
author = {Chung, Sheng -Heng and Chang, Chi -Hao and Manthiram, Arumugam},
abstractNote = {Lithium–sulfur batteries have great potential to satisfy the increasing demand of energy storage systems for portable devices, electric vehicles, and grid storage because of their extremely high specific capacity, cost-effectiveness, and environmental friendliness. In spite of all these merits, the practical utilization of lithium–sulfur batteries is impeded by commonly known challenges, such as low sulfur utilization (<80%), short life (<200 cycles), fast capacity fade, and severe self-discharge effect, which mainly result from the i) low conductivity of the active material, ii) serious polysulfide shuttling, iii) large volume changes, and iv) lithium–metal anode contamination/corrosion. Numerous approaches are reported to effectively mitigate these issues. Indeed, such approaches have shown enhanced lithium–sulfur battery performances. However, many reports overlook the critical parameters, including sulfur loading (<13 mg cm-2), sulfur content (<70 wt%), and electrolyte/sulfur ratio (>11 µL mg-1), that significantly affect the analyzed electrochemical characteristics, energy density, and practicality of lithium–sulfur batteries. This review highlights the trends and progress in making cells fulfilling these fabrication parameters and discuss the challenges of the amount of sulfur and electrolyte in fabricating cells with practically necessary parameters and with high electrochemical utilization and efficiency.},
doi = {10.1002/adfm.201801188},
journal = {Advanced Functional Materials},
number = 28,
volume = 28,
place = {United States},
year = {Tue May 29 00:00:00 EDT 2018},
month = {Tue May 29 00:00:00 EDT 2018}
}
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Figure 1: Illustrations of the electrochemical reaction steps in lithium-sulfur cells: (a) discharge-charge voltage profiles and (b) cyclic voltammogram.
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