Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis
Abstract
In this study, lignin is an abundant biopolymer with a high carbon content and high aromaticity. Despite its potential as a raw material for the fuel and chemical industries, lignin remains the most poorly utilised of the lignocellulosic biopolymers. Effective valorisation of lignin requires careful fine-tuning of multiple “upstream” (i.e., lignin bioengineering, lignin isolation and “early-stage catalytic conversion of lignin”) and “downstream” (i.e., lignin depolymerisation and upgrading) process stages, demanding input and understanding from a broad array of scientific disciplines. This review provides a “beginning-to-end” analysis of the recent advances reported in lignin valorisation. Particular emphasis is placed on the improved understanding of ligninÏs biosynthesis and structure, differences in structure and chemical bonding between native and technical lignins, emerging catalytic valorisation strategies, and the relationships between lignin structure and catalyst performance.
- Authors:
-
[1];
[2];
- Department of Chemical Engineering, Imperial College London, South Kensington Campus London SW7 2AZ UK
- Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterials Science, Utrecht University, Universiteitsweg 99 3584 CG Utrecht The Netherlands
- Max-Planck-Institut für Kohlenforschung, Kaiser-Wilhelm-Platz 1 45470 Mülheim an der Ruhr Germany
- Department of Energy's Great Lakes Bioenergy Research Center, the Wisconsin Energy Institute, and Department of Biochemistry, University of Wisconsin, Madison WI 53726 USA
- Publication Date:
- Research Org.:
- Univ. of Wisconsin, Madison, WI (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Biological and Environmental Research (BER)
- OSTI Identifier:
- 1619413
- Alternate Identifier(s):
- OSTI ID: 1438202
- Grant/Contract Number:
- BER DE-FC02-07ER64494; FC02-07ER64494
- Resource Type:
- Published Article
- Journal Name:
- Angewandte Chemie (International Edition)
- Additional Journal Information:
- Journal Name: Angewandte Chemie (International Edition) Journal Volume: 55 Journal Issue: 29; Journal ID: ISSN 1433-7851
- Publisher:
- Wiley Blackwell (John Wiley & Sons)
- Country of Publication:
- Germany
- Language:
- English
- Subject:
- 59 BASIC BIOLOGICAL SCIENCES; bioengineering; biorefining; catalysis; lignin; lignocellulose
Citation Formats
Rinaldi, Roberto, Jastrzebski, Robin, Clough, Matthew T., Ralph, John, Kennema, Marco, Bruijnincx, Pieter C. A., and Weckhuysen, Bert M. Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis. Germany: N. p., 2016.
Web. doi:10.1002/anie.201510351.
Rinaldi, Roberto, Jastrzebski, Robin, Clough, Matthew T., Ralph, John, Kennema, Marco, Bruijnincx, Pieter C. A., & Weckhuysen, Bert M. Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis. Germany. https://doi.org/10.1002/anie.201510351
Rinaldi, Roberto, Jastrzebski, Robin, Clough, Matthew T., Ralph, John, Kennema, Marco, Bruijnincx, Pieter C. A., and Weckhuysen, Bert M. Fri .
"Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis". Germany. https://doi.org/10.1002/anie.201510351.
@article{osti_1619413,
title = {Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis},
author = {Rinaldi, Roberto and Jastrzebski, Robin and Clough, Matthew T. and Ralph, John and Kennema, Marco and Bruijnincx, Pieter C. A. and Weckhuysen, Bert M.},
abstractNote = {In this study, lignin is an abundant biopolymer with a high carbon content and high aromaticity. Despite its potential as a raw material for the fuel and chemical industries, lignin remains the most poorly utilised of the lignocellulosic biopolymers. Effective valorisation of lignin requires careful fine-tuning of multiple “upstream” (i.e., lignin bioengineering, lignin isolation and “early-stage catalytic conversion of lignin”) and “downstream” (i.e., lignin depolymerisation and upgrading) process stages, demanding input and understanding from a broad array of scientific disciplines. This review provides a “beginning-to-end” analysis of the recent advances reported in lignin valorisation. Particular emphasis is placed on the improved understanding of ligninÏs biosynthesis and structure, differences in structure and chemical bonding between native and technical lignins, emerging catalytic valorisation strategies, and the relationships between lignin structure and catalyst performance.},
doi = {10.1002/anie.201510351},
journal = {Angewandte Chemie (International Edition)},
number = 29,
volume = 55,
place = {Germany},
year = {Fri Jun 17 00:00:00 EDT 2016},
month = {Fri Jun 17 00:00:00 EDT 2016}
}
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