Wafer-scale growth of large arrays of perovskite microplate crystals for functional electronics and optoelectronics

Wang, Gongming; Li, Dehui; Cheng, Hung -Chieh; Li, Yongja; Chen, Chih -Yen; Yin, Anxiang; Zhao, Zipeng; Lin, Zhaoyang; Wu, Hao; He, Qiyuan; Ding, Mengning; Liu, Yuan; Huang, Yu; Duan, Xiangfeng

doi:10.1126/sciadv.1500613

Title: Wafer-scale growth of large arrays of perovskite microplate crystals for functional electronics and optoelectronics

Journal Article · 01 October 2015 · Science Advances

DOI: https://doi.org/10.1126/sciadv.1500613 · OSTI ID:1437930

Wang, Gongming ^[1]; Li, Dehui ^[2]; Cheng, Hung -Chieh ^[2]; Li, Yongja ^[2]; Chen, Chih -Yen ^[2]; Yin, Anxiang ^[2]; Zhao, Zipeng ^[2]; Lin, Zhaoyang ^[2]; Wu, Hao ^[2]; He, Qiyuan ^[2]; Ding, Mengning ^[2]; Liu, Yuan ^[2]; Huang, Yu ^[2]; Duan, Xiangfeng ^[2]

Univ. of California, Los Angeles, CA (United States); Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA
Univ. of California, Los Angeles, CA (United States)

Methylammonium lead iodide perovskite has attracted intensive interest for its diverse optoelectronic applications. However, most studies to date have been limited to bulk thin films that are difficult to implement for integrated device arrays because of their incompatibility with typical lithography processes. We report the first patterned growth of regular arrays of perovskite microplate crystals for functional electronics and optoelectronics. We show that large arrays of lead iodide microplates can be grown from an aqueous solution through a seeded growth process and can be further intercalated with methylammonium iodide to produce perovskite crystals. Structural and optical characterizations demonstrate that the resulting materials display excellent crystalline quality and optical properties. We further show that perovskite crystals can be selectively grown on prepatterned electrode arrays to create independently addressable photodetector arrays and functional field effect transistors. Furthermore, the ability to grow perovskite microplates and to precisely place them at specific locations offers a new material platform for the fundamental investigation of the electronic and optical properties of perovskite materials and opens a pathway for integrated electronic and optoelectronic systems.

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Research Organization:: Univ. of California, Los Angeles, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0008055

OSTI ID:: 1437930

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 9 Vol. 1; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Templated growth of oriented layered hybrid perovskites on 3D-like perovskites Wang, Jifei; Luo, Shiqiang; Lin, Yun Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-019-13856-1	journal	January 2020
Synthesis of centimeter-size free-standing perovskite nanosheets from single-crystal lead bromide for optoelectronic devices Zheng, Jian-Yao; Manning, Hugh G.; Zhang, Yanhui Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-47902-1	journal	August 2019
Perovskite-based photodetectors: materials and devices Wang, Huan; Kim, Dong Ha Chemical Society Reviews, Vol. 46, Issue 17 https://doi.org/10.1039/c6cs00896h	journal	January 2017
Poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate)(PEDOT:PSS)–molybdenum oxide composite films as hole conductors for efficient planar perovskite solar cells Jiang, Yurong; Li, Chen; Liu, Hairui Journal of Materials Chemistry A, Vol. 4, Issue 25 https://doi.org/10.1039/c6ta03658a	journal	January 2016
Two-dimensional halide perovskite nanomaterials and heterostructures Shi, Enzheng; Gao, Yao; Finkenauer, Blake P. Chemical Society Reviews, Vol. 47, Issue 16 https://doi.org/10.1039/c7cs00886d	journal	January 2018
Growth, characterization, and thin film transistor application of CH ₃ NH ₃ PbI ₃ perovskite on polymeric gate dielectric layers Ngai, Jenner H. L.; Ho, Johnny K. W.; Chan, Rocky K. H. RSC Adv., Vol. 7, Issue 78 https://doi.org/10.1039/c7ra08699g	journal	January 2017
A formamidinium–methylammonium lead iodide perovskite single crystal exhibiting exceptional optoelectronic properties and long-term stability Li, Wen-Guang; Rao, Hua-Shang; Chen, Bai-Xue Journal of Materials Chemistry A, Vol. 5, Issue 36 https://doi.org/10.1039/c7ta04608a	journal	January 2017
Controllable growth of two-dimensional perovskite microstructures Fang, Chen; Li, Junze; Wang, Jun CrystEngComm, Vol. 20, Issue 41 https://doi.org/10.1039/c8ce01087k	journal	January 2018
A fractional crystallization technique towards pure mega-size CsPb ₂ Br ₅ single crystal films Yin, Jian; Zhang, Guodong; Tao, Xutang CrystEngComm, Vol. 21, Issue 9 https://doi.org/10.1039/c8ce02191k	journal	January 2019
Structural effects on optoelectronic properties of halide perovskites Chen, Kun; Schünemann, Stefan; Song, Seulki Chemical Society Reviews, Vol. 47, Issue 18 https://doi.org/10.1039/c8cs00212f	journal	January 2018
2D library beyond graphene and transition metal dichalcogenides: a focus on photodetection Wang, Feng; Wang, Zhenxing; Yin, Lei Chemical Society Reviews, Vol. 47, Issue 16 https://doi.org/10.1039/c8cs00255j	journal	January 2018
Transforming bulk alloys into nanoporous lanthanum-based perovskite oxides with high specific surface areas and enhanced electrocatalytic activities Si, Conghui; Zhang, Chi; Sunarso, Jaka Journal of Materials Chemistry A, Vol. 6, Issue 41 https://doi.org/10.1039/c8ta07182a	journal	January 2018
Incorporating deep electron traps into perovskite devices: towards high efficiency solar cells and fast photodetectors Zhang, Dezhong; Liu, Chunyu; Li, Zhiqi Journal of Materials Chemistry A, Vol. 6, Issue 42 https://doi.org/10.1039/c8ta08499h	journal	January 2018
Synthesis of ultrathin two-dimensional organic–inorganic hybrid perovskite nanosheets for polymer field-effect transistors Zhu, Lijie; Zhang, Huaye; Lu, Qipeng Journal of Materials Chemistry C, Vol. 6, Issue 15 https://doi.org/10.1039/c8tc00289d	journal	January 2018
Two-step vapor deposition of self-catalyzed large-size PbI ₂ nanobelts for high-performance photodetectors Han, Mingming; Sun, Jiamin; Bian, Luozhen Journal of Materials Chemistry C, Vol. 6, Issue 21 https://doi.org/10.1039/c8tc01180j	journal	January 2018
Recent progress on highly sensitive perovskite photodetectors Miao, Jianli; Zhang, Fujun Journal of Materials Chemistry C, Vol. 7, Issue 7 https://doi.org/10.1039/c8tc06089d	journal	January 2019
Monocrystalline perovskite wafers/thin films for photovoltaic and transistor applications Wang, Kai; Wu, Congcong; Hou, Yuchen Journal of Materials Chemistry A, Vol. 7, Issue 43 https://doi.org/10.1039/c9ta08823g	journal	January 2019
2D perovskite microsheets for high-performance photodetectors Qian, Liu; Sun, Yilin; Sun, Mengxing Journal of Materials Chemistry C, Vol. 7, Issue 18 https://doi.org/10.1039/c9tc00138g	journal	January 2019
In situ localized formation of cesium lead bromide nanocomposites for fluorescence micro-patterning technology achieved by organic solvent polymerization Zhang, Louwen; Liu, Yanan; Gan, Zongsong Journal of Materials Chemistry C, Vol. 8, Issue 10 https://doi.org/10.1039/c9tc06687j	journal	January 2020
Toward air-stable field-effect transistors with a tin iodide-based hybrid perovskite semiconductor Matsushima, Toshinori; Terakawa, Shinobu; Leyden, Matthew R. Journal of Applied Physics, Vol. 125, Issue 23 https://doi.org/10.1063/1.5097433	journal	June 2019
Manipulating the assembly of perovskites onto soft nanoimprinted titanium dioxide templates Baca, Alfred J.; Roberts, M. Joseph; Stenger-Smith, John Nanotechnology, Vol. 29, Issue 25 https://doi.org/10.1088/1361-6528/aabac2	journal	April 2018
Synthesis and optical applications of low dimensional metal-halide perovskites Liu, Jingying; Chen, Keqiang; Khan, Sayed Ali Nanotechnology, Vol. 31, Issue 15 https://doi.org/10.1088/1361-6528/ab5a19	journal	January 2020
Synthesis and Characterization of Methylammonium Lead Iodide Perovskite and its Application in Planar Hetero-junction Devices Upadhyaya, Aditi; Negi, Chandra Mohan Singh; Yadav, Anjali Semiconductor Science and Technology, Vol. 33, Issue 6 https://doi.org/10.1088/1361-6641/aac066	journal	May 2018
Understanding charge transport in lead iodide perovskite thin-film field-effect transistors Senanayak, Satyaprasad P.; Yang, Bingyan; Thomas, Tudor H. Science Advances, Vol. 3, Issue 1 https://doi.org/10.1126/sciadv.1601935	journal	January 2017
A general printing approach for scalable growth of perovskite single-crystal films Gu, Zhenkun; Huang, Zhandong; Li, Chang Science Advances, Vol. 4, Issue 6 https://doi.org/10.1126/sciadv.aat2390	journal	June 2018
Understanding charge transport in lead iodide perovskite thin-film field-effect transistors Senanayak, Satyaprasad; Yang, B.; Thomas, Tudor Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.7594	text	January 2017
Controllable Synthesis of 2D Perovskite on Different Substrates and Its Application as Photodetector Xue, Yunzhou; Yuan, Jian; Liu, Jingying Nanomaterials, Vol. 8, Issue 8 https://doi.org/10.3390/nano8080591	journal	August 2018
Impact of Grain Boundaries on Efficiency and Stability of Organic-Inorganic Trihalide Perovskites Chu, Zhaodong; Yang, Mengjin; Schulz, Philip arXiv https://doi.org/10.48550/arxiv.1610.00755	text	January 2016

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