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Title: Nucleation and phase transformation pathways in electrolyte solutions investigated by in situ microscopy techniques

Identification of crystal nucleation and growth pathways is of fundamental importance for synthesis of functional materials, which requires control over size, orientation, polymorph, and hierarchical structure, often in the presence of additives used to tune the energy landscape defining these pathways. Furthermore we summarize the recent progress in application of in situ TEM and AFM techniques to monitor or even tune the pathway of crystal nucleation and growth.
Authors:
 [1] ;  [2] ;  [3]
  1. Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
  2. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  3. Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Univ. of Washington, Seattle, WA (United States)
Publication Date:
Grant/Contract Number:
AC05–76RL01830; AC52-07NA27344
Type:
Accepted Manuscript
Journal Name:
Current Opinion in Colloid & Interface Science
Additional Journal Information:
Journal Volume: 34; Journal Issue: C; Journal ID: ISSN 1359-0294
Publisher:
Elsevier
Research Org:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Nucleation; Phase transformation; In situ TEM; In situ AFM
OSTI Identifier:
1437026

Tao, Jinhui, Nielsen, Michael H., and De Yoreo, James J.. Nucleation and phase transformation pathways in electrolyte solutions investigated by in situ microscopy techniques. United States: N. p., Web. doi:10.1016/j.cocis.2018.04.002.
Tao, Jinhui, Nielsen, Michael H., & De Yoreo, James J.. Nucleation and phase transformation pathways in electrolyte solutions investigated by in situ microscopy techniques. United States. doi:10.1016/j.cocis.2018.04.002.
Tao, Jinhui, Nielsen, Michael H., and De Yoreo, James J.. 2018. "Nucleation and phase transformation pathways in electrolyte solutions investigated by in situ microscopy techniques". United States. doi:10.1016/j.cocis.2018.04.002.
@article{osti_1437026,
title = {Nucleation and phase transformation pathways in electrolyte solutions investigated by in situ microscopy techniques},
author = {Tao, Jinhui and Nielsen, Michael H. and De Yoreo, James J.},
abstractNote = {Identification of crystal nucleation and growth pathways is of fundamental importance for synthesis of functional materials, which requires control over size, orientation, polymorph, and hierarchical structure, often in the presence of additives used to tune the energy landscape defining these pathways. Furthermore we summarize the recent progress in application of in situ TEM and AFM techniques to monitor or even tune the pathway of crystal nucleation and growth.},
doi = {10.1016/j.cocis.2018.04.002},
journal = {Current Opinion in Colloid & Interface Science},
number = C,
volume = 34,
place = {United States},
year = {2018},
month = {4}
}