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Title: Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures

Abstract

A novel synthesis route to the formation of vertically aligned single–crystalline oxide nanostructures is found by precisely controlling the nonequilibrium pulsed laser deposition process. Here, the columnar nanostructures with deep crevices offering a large surface area are generated owing to the diffusion limited geometric shadowing effect.

Authors:
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1]
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  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1436958
Alternate Identifier(s):
OSTI ID: 1401742
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Materials Interfaces
Additional Journal Information:
Journal Volume: 4; Journal Issue: 3; Journal ID: ISSN 2196-7350
Publisher:
Wiley-VCH
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; vertical oxide nanostructures; pulsed laser deposition; diffusion limited aggregation; binary oxides; porous nanostructures

Citation Formats

Lee, Dongkyu, Gao, Xiang, Fan, Lisha, Guo, Er-Jia, Farmer, Thomas O., Heller, William T., Ward, T. Z., Eres, Gyula, Fitzsimmons, Michael R., Chisholm, Matthew F., and Lee, Ho Nyung. Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures. United States: N. p., 2017. Web. doi:10.1002/admi.201601034.
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Lee, Dongkyu, Gao, Xiang, Fan, Lisha, Guo, Er-Jia, Farmer, Thomas O., Heller, William T., Ward, T. Z., Eres, Gyula, Fitzsimmons, Michael R., Chisholm, Matthew F., & Lee, Ho Nyung. Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures. United States. https://doi.org/10.1002/admi.201601034
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Lee, Dongkyu, Gao, Xiang, Fan, Lisha, Guo, Er-Jia, Farmer, Thomas O., Heller, William T., Ward, T. Z., Eres, Gyula, Fitzsimmons, Michael R., Chisholm, Matthew F., and Lee, Ho Nyung. Fri . "Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures". United States. https://doi.org/10.1002/admi.201601034. https://www.osti.gov/servlets/purl/1436958.
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@article{osti_1436958,
title = {Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures},
author = {Lee, Dongkyu and Gao, Xiang and Fan, Lisha and Guo, Er-Jia and Farmer, Thomas O. and Heller, William T. and Ward, T. Z. and Eres, Gyula and Fitzsimmons, Michael R. and Chisholm, Matthew F. and Lee, Ho Nyung},
abstractNote = {A novel synthesis route to the formation of vertically aligned single–crystalline oxide nanostructures is found by precisely controlling the nonequilibrium pulsed laser deposition process. Here, the columnar nanostructures with deep crevices offering a large surface area are generated owing to the diffusion limited geometric shadowing effect.},
doi = {10.1002/admi.201601034},
journal = {Advanced Materials Interfaces},
number = 3,
volume = 4,
place = {United States},
year = {2017},
month = {1}
}
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https://doi.org/10.1002/admi.201601034
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