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Title: Magnetodielectric Response from Spin-Orbital Interaction Occurring at Interface of Ferromagnetic Co and Organometal Halide Perovskite Layers via Rashba Effect

Abstract

The spin on a ferromagnetic Co surface can interact with the asymmetric orbital on an organometal halide perovskite surface, leading to an anisotropic magnetodielectric effect. Here, this study presents an opportunity to integrate ferromagnetic and semiconducting properties through the Rasbha effect for achieving spin–dependent electronic functionalities based on thin–film design.

Authors:
 [1]; ORCiD logo [1];  [1];  [2];  [1]; ORCiD logo [3];  [1];  [1]; ORCiD logo [3]; ORCiD logo [3];  [1];  [1]
  1. Univ. of Tennessee, Knoxville, TN (United States)
  2. Beijing Jiaotong Univ., Beijing (China)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1436051
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 29; Journal Issue: 6; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; magnetodielectric effect; Rashba effect; organometal halide perovskites; spin-orbital coupling

Citation Formats

Li, Mingxing, Li, Ling, Mukherjee, Rupam, Wang, Kai, Liu, Qing Gary, Zou, Qiang, Xu, Hengxing, Tisdale, Jeremy, Gai, Zheng, Ivanov, Ilia N., Mandrus, David, and Hu, Bin. Magnetodielectric Response from Spin-Orbital Interaction Occurring at Interface of Ferromagnetic Co and Organometal Halide Perovskite Layers via Rashba Effect. United States: N. p., 2016. Web. doi:10.1002/adma.201603667.
Li, Mingxing, Li, Ling, Mukherjee, Rupam, Wang, Kai, Liu, Qing Gary, Zou, Qiang, Xu, Hengxing, Tisdale, Jeremy, Gai, Zheng, Ivanov, Ilia N., Mandrus, David, & Hu, Bin. Magnetodielectric Response from Spin-Orbital Interaction Occurring at Interface of Ferromagnetic Co and Organometal Halide Perovskite Layers via Rashba Effect. United States. doi:10.1002/adma.201603667.
Li, Mingxing, Li, Ling, Mukherjee, Rupam, Wang, Kai, Liu, Qing Gary, Zou, Qiang, Xu, Hengxing, Tisdale, Jeremy, Gai, Zheng, Ivanov, Ilia N., Mandrus, David, and Hu, Bin. Mon . "Magnetodielectric Response from Spin-Orbital Interaction Occurring at Interface of Ferromagnetic Co and Organometal Halide Perovskite Layers via Rashba Effect". United States. doi:10.1002/adma.201603667. https://www.osti.gov/servlets/purl/1436051.
@article{osti_1436051,
title = {Magnetodielectric Response from Spin-Orbital Interaction Occurring at Interface of Ferromagnetic Co and Organometal Halide Perovskite Layers via Rashba Effect},
author = {Li, Mingxing and Li, Ling and Mukherjee, Rupam and Wang, Kai and Liu, Qing Gary and Zou, Qiang and Xu, Hengxing and Tisdale, Jeremy and Gai, Zheng and Ivanov, Ilia N. and Mandrus, David and Hu, Bin},
abstractNote = {The spin on a ferromagnetic Co surface can interact with the asymmetric orbital on an organometal halide perovskite surface, leading to an anisotropic magnetodielectric effect. Here, this study presents an opportunity to integrate ferromagnetic and semiconducting properties through the Rasbha effect for achieving spin–dependent electronic functionalities based on thin–film design.},
doi = {10.1002/adma.201603667},
journal = {Advanced Materials},
number = 6,
volume = 29,
place = {United States},
year = {2016},
month = {12}
}

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Works referenced in this record:

MAPbI3-xClx Mixed Halide Perovskite for Hybrid Solar Cells: The Role of Chloride as Dopant on the Transport and Structural Properties
journal, November 2013

  • Colella, Silvia; Mosconi, Edoardo; Fedeli, Paolo
  • Chemistry of Materials, Vol. 25, Issue 22, p. 4613-4618
  • DOI: 10.1021/cm402919x

Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites
journal, October 2012