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Title: Optimal control of orientation and entanglement for two dipole–dipole coupled quantum planar rotors

Abstract

Optimal control simulations are performed for orientation and entanglement of two dipole–dipole coupled identical quantum rotors.

Authors:
 [1];  [2]; ORCiD logo [2]
  1. State Key Laboratory of Precision, East China Normal University, Shanghai 200062, China, Department of Chemistry
  2. Department of Chemistry, Princeton University, Princeton, USA
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1435371
Grant/Contract Number:  
FG02-02ER15344
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Physical Chemistry Chemical Physics
Additional Journal Information:
Journal Name: Physical Chemistry Chemical Physics Journal Volume: 20 Journal Issue: 18; Journal ID: ISSN 1463-9076
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Yu, Hongling, Ho, Tak-San, and Rabitz, Herschel. Optimal control of orientation and entanglement for two dipole–dipole coupled quantum planar rotors. United Kingdom: N. p., 2018. Web. doi:10.1039/C8CP00231B.
Yu, Hongling, Ho, Tak-San, & Rabitz, Herschel. Optimal control of orientation and entanglement for two dipole–dipole coupled quantum planar rotors. United Kingdom. https://doi.org/10.1039/C8CP00231B
Yu, Hongling, Ho, Tak-San, and Rabitz, Herschel. Mon . "Optimal control of orientation and entanglement for two dipole–dipole coupled quantum planar rotors". United Kingdom. https://doi.org/10.1039/C8CP00231B.
@article{osti_1435371,
title = {Optimal control of orientation and entanglement for two dipole–dipole coupled quantum planar rotors},
author = {Yu, Hongling and Ho, Tak-San and Rabitz, Herschel},
abstractNote = {Optimal control simulations are performed for orientation and entanglement of two dipole–dipole coupled identical quantum rotors.},
doi = {10.1039/C8CP00231B},
journal = {Physical Chemistry Chemical Physics},
number = 18,
volume = 20,
place = {United Kingdom},
year = {Mon Jan 01 00:00:00 EST 2018},
month = {Mon Jan 01 00:00:00 EST 2018}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1039/C8CP00231B

Citation Metrics:
Cited by: 8 works
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Works referenced in this record:

Free-time and fixed end-point multi-target optimal control theory: Application to quantum computing
journal, January 2011


Optimal control of a charge qubit in a double quantum dot with a Coulomb impurity
journal, February 2017

  • Coden, Diego S. Acosta; Romero, Rodolfo H.; Ferrón, Alejandro
  • Physica E: Low-dimensional Systems and Nanostructures, Vol. 86
  • DOI: 10.1016/j.physe.2016.09.020

Monotonic convergent quantum optimal control method with exact equality constraints on the optimized control fields
journal, May 2016


Observation of Cumulative Spatial Focusing of Atoms
journal, December 2002


Exploring the control landscape for nonlinear quantum dynamics
journal, June 2014


Why do effective quantum controls appear easy to find?
journal, June 2006


Coherent Control of Quantum Dynamics: The Dream Is Alive
journal, March 1993


Essential entanglement for atomic and molecular physics
journal, September 2011

  • Tichy, Malte C.; Mintert, Florian; Buchleitner, Andreas
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 44, Issue 19
  • DOI: 10.1088/0953-4075/44/19/192001

Monotonically convergent optimization in quantum control using Krotov's method
journal, March 2012

  • Reich, Daniel M.; Ndong, Mamadou; Koch, Christiane P.
  • The Journal of Chemical Physics, Vol. 136, Issue 10
  • DOI: 10.1063/1.3691827

Deflection of Neutral Molecules using the Nonresonant Dipole Force
journal, October 1997


Robustness of adiabatic quantum computation
journal, December 2001


Molecular Orientation and Alignment by Intense Single-Cycle THz Pulses
journal, October 2011


Prospects for quantum computing with an array of ultracold polar paramagnetic molecules
journal, March 2016

  • Karra, Mallikarjun; Sharma, Ketan; Friedrich, Bretislav
  • The Journal of Chemical Physics, Vol. 144, Issue 9
  • DOI: 10.1063/1.4942928

Accurate time propagation for the Schrödinger equation with an explicitly time-dependent Hamiltonian
journal, May 2008

  • Kormann, Katharina; Holmgren, Sverker; Karlsson, Hans O.
  • The Journal of Chemical Physics, Vol. 128, Issue 18
  • DOI: 10.1063/1.2916581

Tridiagonal Toeplitz matrices: properties and novel applications: TRIDIAGONAL TOEPLITZ MATRICES
journal, March 2012

  • Noschese, Silvia; Pasquini, Lionello; Reichel, Lothar
  • Numerical Linear Algebra with Applications, Vol. 20, Issue 2
  • DOI: 10.1002/nla.1811

Generalized monotonically convergent algorithms for solving quantum optimal control problems
journal, March 2004

  • Ohtsuki, Yukiyoshi; Turinici, Gabriel; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 120, Issue 12
  • DOI: 10.1063/1.1650297

Wavepacket dancing: Achieving chemical selectivity by shaping light pulses
journal, December 1989


Fast-kick-off monotonically convergent algorithm for searching optimal control fields
journal, September 2011


Free-time and fixed end-point optimal control theory in quantum mechanics: Application to entanglement generation
journal, January 2009

  • Mishima, K.; Yamashita, K.
  • The Journal of Chemical Physics, Vol. 130, Issue 3
  • DOI: 10.1063/1.3062860

Exploring the transition-probability-control landscape of open quantum systems: Application to a two-level case
journal, September 2013


Topology of classical molecular optimal control landscapes for multi-target objectives
journal, April 2015

  • Joe-Wong, Carlee; Ho, Tak-San; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 142, Issue 15
  • DOI: 10.1063/1.4918274

Optimal control of selective vibrational excitation in harmonic linear chain molecules
journal, June 1988

  • Shi, Shenghua; Woody, Andrea; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 88, Issue 11
  • DOI: 10.1063/1.454384

Whither the Future of Controlling Quantum Phenomena?
journal, May 2000


A High Phase-Space-Density Gas of Polar Molecules
journal, October 2008


Exploring the level sets of quantum control landscapes
journal, May 2006


Controlled dissociation of I2 via optical transitions between the X and B electronic states
journal, May 1993


Entanglement of angular momenta of atoms and molecules
journal, January 2008

  • Mishima, K.; Yamashita, K.
  • International Journal of Quantum Chemistry, Vol. 108, Issue 8
  • DOI: 10.1002/qua.21644

Laser-Field-Free Molecular Orientation
journal, June 2008


ANTHRAX INVESTIGATION: FBI Discusses Microbial Forensics--but Key Questions Remain Unanswered
journal, August 2008


Tailoring laser pulses with spectral and fluence constraints using optimal control theory
journal, September 2005

  • Werschnik, J.; Gross, E. K. U.
  • Journal of Optics B: Quantum and Semiclassical Optics, Vol. 7, Issue 10
  • DOI: 10.1088/1464-4266/7/10/014

Field-free molecular orientation by terahertz laser pulses at high temperature
journal, June 2012


Quantum Optimally Controlled Transition Landscapes
journal, March 2004


Orienting coupled quantum rotors by ultrashort laser pulses
journal, July 2004


Optimal control of quantum-mechanical systems: Existence, numerical approximation, and applications
journal, June 1988

  • Peirce, Anthony P.; Dahleh, Mohammed A.; Rabitz, Herschel
  • Physical Review A, Vol. 37, Issue 12, p. 4950-4964
  • DOI: 10.1103/PhysRevA.37.4950

Dielectric anomaly in coupled rotor systems
journal, January 2004


Field-Free Orientation of Molecules
journal, October 2001


Implementation of quantum logic gates using polar molecules in pendular states
journal, January 2013

  • Zhu, Jing; Kais, Sabre; Wei, Qi
  • The Journal of Chemical Physics, Vol. 138, Issue 2
  • DOI: 10.1063/1.4774058

Quantum phase gate and controlled entanglement with polar molecules
journal, March 2007


Quantum entanglement
journal, June 2009

  • Horodecki, Ryszard; Horodecki, Paweł; Horodecki, Michał
  • Reviews of Modern Physics, Vol. 81, Issue 2
  • DOI: 10.1103/RevModPhys.81.865

Photonic generation of microwave arbitrary waveforms
journal, July 2011


Review of high-power microwave source research
journal, November 1997

  • Gold, Steven H.; Nusinovich, Gregory S.
  • Review of Scientific Instruments, Vol. 68, Issue 11
  • DOI: 10.1063/1.1148382

Optimal local control of coherent dynamics in custom-made nanostructures
journal, June 2013


Quantum observable homotopy tracking control
journal, October 2005

  • Rothman, Adam; Ho, Tak-San; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 123, Issue 13
  • DOI: 10.1063/1.2042456

A Quantum Adiabatic Evolution Algorithm Applied to Random Instances of an NP-Complete Problem
journal, April 2001


Control landscapes are almost always trap free: a geometric assessment
journal, April 2017

  • Russell, Benjamin; Rabitz, Herschel; Wu, Re-Bing
  • Journal of Physics A: Mathematical and Theoretical, Vol. 50, Issue 20
  • DOI: 10.1088/1751-8121/aa6b77

Suppression of strong-field ionization by optimal pulse shaping: Application to hydrogen and the hydrogen molecular ion
journal, February 2015


Surface plasmon enhanced substrate mediated photochemistry on roughened silver
journal, November 2000

  • Kidd, Robert T.; Lennon, David; Meech, Stephen R.
  • The Journal of Chemical Physics, Vol. 113, Issue 18
  • DOI: 10.1063/1.1316106

New formulations of monotonically convergent quantum control algorithms
journal, May 2003

  • Maday, Yvon; Turinici, Gabriel
  • The Journal of Chemical Physics, Vol. 118, Issue 18
  • DOI: 10.1063/1.1564043

Controlling polar molecules in optical lattices
journal, April 2006


Orientations of two coupled molecules
journal, November 2004


Rapidly convergent iteration methods for quantum optimal control of population
journal, February 1998

  • Zhu, Wusheng; Botina, Jair; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 108, Issue 5
  • DOI: 10.1063/1.475576

Angular Focusing, Squeezing, and Rainbow Formation in a Strongly Driven Quantum Rotor
journal, September 2001


Adiabatic approximation with exponential accuracy for many-body systems and quantum computation
journal, October 2009

  • Lidar, Daniel A.; Rezakhani, Ali T.; Hamma, Alioscia
  • Journal of Mathematical Physics, Vol. 50, Issue 10
  • DOI: 10.1063/1.3236685

High-order harmonic generation in the presence of a resonance
journal, July 2011


Topology of optimally controlled quantum mechanical transition probability landscapes
journal, July 2006


Rotational entangled states between two coupled molecules
journal, December 2005

  • Liao, Y. Y.; Chen, Y. N.; Li, C. M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 39, Issue 2
  • DOI: 10.1088/0953-4075/39/2/016

Quantum optimal control of isomerization dynamics of a one-dimensional reaction-path model dominated by a competing dissociation channel
journal, July 2009

  • Kurosaki, Yuzuru; Artamonov, Maxim; Ho, Tak-San
  • The Journal of Chemical Physics, Vol. 131, Issue 4
  • DOI: 10.1063/1.3185565

Optimal Control Simulation of Field-Free Molecular Orientation: Alignment-Enhanced Molecular Orientation
journal, August 2012

  • Nakajima, Katsuhiro; Abe, Hiroya; Ohtsuki, Yukiyoshi
  • The Journal of Physical Chemistry A, Vol. 116, Issue 46
  • DOI: 10.1021/jp3052054

Microwave photonics combines two worlds
journal, June 2007


Quantum computing using rotational modes of two polar molecules
journal, June 2009


Numerical modelling of the excitation energy dependence of adsorbate photochemistry at metal surfaces
journal, October 2001


Accelerated monotonic convergence of optimal control over quantum dynamics
journal, August 2010


Optimal Control of Multiphoton Ionization Processes in Aligned I 2 Molecules with Time-Dependent Polarization Pulses
journal, April 2004


Optimal molecular alignment and orientation through rotational ladder climbing
journal, October 2005

  • Salomon, Julien; Dion, Claude M.; Turinici, Gabriel
  • The Journal of Chemical Physics, Vol. 123, Issue 14
  • DOI: 10.1063/1.2049270

Nanometer Resolution and Coherent Optical Dipole Coupling of Two Individual Molecules
journal, September 2002


Observable-preserving control of quantum dynamics over a family of related systems
journal, August 2005


Maximum attainable field-free molecular orientation of a thermal ensemble with near–single-cycle THz pulses
journal, January 2013


A rapid monotonically convergent iteration algorithm for quantum optimal control over the expectation value of a positive definite operator
journal, July 1998

  • Zhu, Wusheng; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 109, Issue 2
  • DOI: 10.1063/1.476575

Two-State Wave Packet for Strong Field-Free Molecular Orientation
journal, March 2015


Microwave Spectra of Molecules of Astrophysical Interest VI. Carbonyl Sulfide and Hydrogen Cyanide
journal, January 1974

  • Maki, Arthur G.
  • Journal of Physical and Chemical Reference Data, Vol. 3, Issue 1
  • DOI: 10.1063/1.3253139