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Title: Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals

Abstract

Asymmetric nanophotonic structures enable a wide range of opportunities in optical nanotechnology because they support efficient optical nonlinearities mediated by multiple plasmon resonances over a broad spectral range. The Archimedean nanospiral is a canonical example of a chiral plasmonic structure because it supports even-order nonlinearities that are not generally accessible in locally symmetric geometries. However, the complex spiral response makes nanoscale experimental characterization of the plasmonic near-field structure highly desirable. Here we employ high-efficiency, high-spatial-resolution cathodoluminescence imaging in a scanning transmission electron microscope to describe the spatial, spectral, and polarization response of plasmon modes in the nanospiral geometry.

Authors:
ORCiD logo [1];  [2]; ORCiD logo [3]; ORCiD logo [1]; ORCiD logo [1];  [4]; ORCiD logo [1];  [2]
+ Show Author Affiliations
  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  2. Vanderbilt Univ., Nashville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Univ. of North Carolina, Chapel Hill, NC (United States)
  4. Vanderbilt Univ., Nashville, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Vanderbilt Univ., Nashville, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1435311
Alternate Identifier(s):
OSTI ID: 1420366; OSTI ID: 1597874
Grant/Contract Number:  
AC05-00OR22725; FG02-01ER45916; FG02-09ER4655; FG02-09ER46554
Resource Type:
Accepted Manuscript
Journal Name:
Optics Letters
Additional Journal Information:
Journal Volume: 43; Journal Issue: 4; Journal ID: ISSN 0146-9592
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Surface plasmons; Cathodoluminescence; Subwavelength structures, nano-structures; Polarization-selective devices

Citation Formats

Hachtel, Jordan A., Davidson, II, Roderick B., Kovalik, Elena R., Retterer, Scott T., Lupini, Andrew R., Haglund, Jr., Richard F., Lawrie, Benjamin J., and Pantelides, Sokrates T. Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals. United States: N. p., 2018. Web. doi:10.1364/OL.43.000927.
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Hachtel, Jordan A., Davidson, II, Roderick B., Kovalik, Elena R., Retterer, Scott T., Lupini, Andrew R., Haglund, Jr., Richard F., Lawrie, Benjamin J., & Pantelides, Sokrates T. Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals. United States. https://doi.org/10.1364/OL.43.000927
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Hachtel, Jordan A., Davidson, II, Roderick B., Kovalik, Elena R., Retterer, Scott T., Lupini, Andrew R., Haglund, Jr., Richard F., Lawrie, Benjamin J., and Pantelides, Sokrates T. Thu . "Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals". United States. https://doi.org/10.1364/OL.43.000927. https://www.osti.gov/servlets/purl/1435311.
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@article{osti_1435311,
title = {Polarization- and wavelength-resolved near-field imaging of complex plasmonic modes in Archimedean nanospirals},
author = {Hachtel, Jordan A. and Davidson, II, Roderick B. and Kovalik, Elena R. and Retterer, Scott T. and Lupini, Andrew R. and Haglund, Jr., Richard F. and Lawrie, Benjamin J. and Pantelides, Sokrates T.},
abstractNote = {Asymmetric nanophotonic structures enable a wide range of opportunities in optical nanotechnology because they support efficient optical nonlinearities mediated by multiple plasmon resonances over a broad spectral range. The Archimedean nanospiral is a canonical example of a chiral plasmonic structure because it supports even-order nonlinearities that are not generally accessible in locally symmetric geometries. However, the complex spiral response makes nanoscale experimental characterization of the plasmonic near-field structure highly desirable. Here we employ high-efficiency, high-spatial-resolution cathodoluminescence imaging in a scanning transmission electron microscope to describe the spatial, spectral, and polarization response of plasmon modes in the nanospiral geometry.},
doi = {10.1364/OL.43.000927},
journal = {Optics Letters},
number = 4,
volume = 43,
place = {United States},
year = {Thu Feb 15 00:00:00 EST 2018},
month = {Thu Feb 15 00:00:00 EST 2018}
}
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Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1364/OL.43.000927
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Cited by: 11 works
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Figures / Tables:

Fig. 1 Fig. 1: Imaging the Plasmonic Response of Nanospirals with Cathodoluminescence. (a) Schematic of Archimedean nanospiral. (b.c) Finite-difference time-domain (FDTD) simulations of the focusing plasmon mode in the near-infrared (NIR) at 850 nm (b) and hourglass plasmon mode in the visible at 601 nm (c) that is strongly dependent on themore » polarization of the exciting source. (d) Schematic diagram for scanning transmission electron microscope (STEM) apparatus designed for cathodoluminescence (CL).« less
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Works referenced in this record:

Probing plasmons in three dimensions by combining complementary spectroscopies in a scanning transmission electron microscope
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Periodically Varying Height in Metal Nano-pillars for Enhanced Generation of Localized Surface Plasmon Field
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Direct Write Protein Patterns for Multiplexed Cytokine Detection from Live Cells Using Electron Beam Lithography
journal, December 2015

Complex Polarization Response in Plasmonic Nanospirals
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Tailoring MoS 2 Exciton–Plasmon Interaction by Optical Spin–Orbit Coupling
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    Works referencing / citing this record:

    Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators
    journal, March 2019

    • Hachtel, Jordan A.; Cho, Sang-Yeon; Davidson, Roderick B.
    • Light: Science & Applications, Vol. 8, Issue 1
    • DOI: 10.1038/s41377-019-0136-z
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      Figures / Tables found in this record:

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