Shift current bulk photovoltaic effect in polar materials—hybrid and oxide perovskites and beyond
Abstract
Here, the bulk photovoltaic effect (BPVE) refers to the generation of a steady photocurrent and above-bandgap photovoltage in a single-phase homogeneous material lacking inversion symmetry. The mechanism of BPVE is decidedly different from the typical p–n junction-based photovoltaic mechanism in heterogeneous materials. Recently, there has been renewed interest in ferroelectric materials for solar energy conversion, inspired by the discovery of above-bandgap photovoltages in ferroelectrics, the invention of low bandgap ferroelectric materials and the rapidly improving power conversion efficiency of metal halide perovskites. However, as long as the nature of the BPVE and its dependence on composition and structure remain poorly understood, materials engineering and the realisation of its true potential will be hampered. In this review article, we survey the history, development and recent progress in understanding the mechanisms of BPVE, with a focus on the shift current mechanism, an intrinsic BPVE that is universal to all materials lacking inversion symmetry. In addition to explaining the theory of shift current, materials design opportunities and challenges will be discussed for future applications of the BPVE.
- Authors:
-
[1];
[3];
- Univ. of Pennsylvania, Philadelphia, PA (United States)
- United States Naval Research Lab., Washington, D.C. (United States)
- Carnegie Institution of Science, Washington, D.C. (United States)
- Publication Date:
- Research Org.:
- Univ. of Pennsylvania, Philadelphia, PA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Advanced Scientific Computing Research (ASCR)
- OSTI Identifier:
- 1434900
- Grant/Contract Number:
- FG02-07ER46431
- Resource Type:
- Accepted Manuscript
- Journal Name:
- npj Computational Materials
- Additional Journal Information:
- Journal Volume: 2; Journal Issue: 1; Journal ID: ISSN 2057-3960
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; Electronic properties and materials; Electronic structure; Nonlinear optics; Solar cells
Citation Formats
Tan, Liang Z., Zheng, Fan, Young, Steve M., Wang, Fenggong, Liu, Shi, and Rappe, Andrew M. Shift current bulk photovoltaic effect in polar materials—hybrid and oxide perovskites and beyond. United States: N. p., 2016.
Web. doi:10.1038/npjcompumats.2016.26.
Tan, Liang Z., Zheng, Fan, Young, Steve M., Wang, Fenggong, Liu, Shi, & Rappe, Andrew M. Shift current bulk photovoltaic effect in polar materials—hybrid and oxide perovskites and beyond. United States. https://doi.org/10.1038/npjcompumats.2016.26
Tan, Liang Z., Zheng, Fan, Young, Steve M., Wang, Fenggong, Liu, Shi, and Rappe, Andrew M. Fri .
"Shift current bulk photovoltaic effect in polar materials—hybrid and oxide perovskites and beyond". United States. https://doi.org/10.1038/npjcompumats.2016.26. https://www.osti.gov/servlets/purl/1434900.
@article{osti_1434900,
title = {Shift current bulk photovoltaic effect in polar materials—hybrid and oxide perovskites and beyond},
author = {Tan, Liang Z. and Zheng, Fan and Young, Steve M. and Wang, Fenggong and Liu, Shi and Rappe, Andrew M.},
abstractNote = {Here, the bulk photovoltaic effect (BPVE) refers to the generation of a steady photocurrent and above-bandgap photovoltage in a single-phase homogeneous material lacking inversion symmetry. The mechanism of BPVE is decidedly different from the typical p–n junction-based photovoltaic mechanism in heterogeneous materials. Recently, there has been renewed interest in ferroelectric materials for solar energy conversion, inspired by the discovery of above-bandgap photovoltages in ferroelectrics, the invention of low bandgap ferroelectric materials and the rapidly improving power conversion efficiency of metal halide perovskites. However, as long as the nature of the BPVE and its dependence on composition and structure remain poorly understood, materials engineering and the realisation of its true potential will be hampered. In this review article, we survey the history, development and recent progress in understanding the mechanisms of BPVE, with a focus on the shift current mechanism, an intrinsic BPVE that is universal to all materials lacking inversion symmetry. In addition to explaining the theory of shift current, materials design opportunities and challenges will be discussed for future applications of the BPVE.},
doi = {10.1038/npjcompumats.2016.26},
journal = {npj Computational Materials},
number = 1,
volume = 2,
place = {United States},
year = {Fri Aug 26 00:00:00 EDT 2016},
month = {Fri Aug 26 00:00:00 EDT 2016}
}
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Releasing the hidden shift current in the TTF-CA organic molecular solid via symmetry lowering
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Large Bulk Photovoltaic Response by Symmetry-Breaking Structural Transformation in Ferroelectric [ ] 0.5 [( ] 0.5
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The Narrowest Band Gap Ever Observed in Molecular Ferroelectrics: Hexane-1,6-diammonium Pentaiodobismuth(III)
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Wannier90 as a community code: New features and applications
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Spatio-temporal dynamics of shift current quantum pumping by femtosecond light pulse
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Ab initio calculation of the shift photocurrent by Wannier interpolation
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Impact of electrodes on the extraction of shift current from a ferroelectric semiconductor SbSI
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Ultrafast Spin-To-Charge Conversion at the Surface of Topological Insulator Thin Films
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Theory for shift current of bosons: Photogalvanic spin current in ferrimagnetic and antiferromagnetic insulators
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Non-equilibrium nature of non-linear optical response: Application to the bulk photo voltaic effect
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Giant photovoltaic response in band engineered ferroelectric perovskite
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