Radiation-driven rotational motion of nanoparticles
Abstract
Focused synchrotron beams can influence a studied sampleviaheating, or radiation pressure effects due to intensity gradients. The high angular sensitivity of rotational X-ray tracking of crystalline particlesviatheir Bragg reflections can detect extremely small forces such as those caused by field gradients. By tracking the rotational motion of single-crystal nanoparticles embedded in a viscous or viscoelastic medium, the effects of heating in a uniform gradient beam and radiation pressure in a Gaussian profile beam were observed. Changes in viscosity due to X-ray heating were measured for 42 µm crystals in glycerol, and angular velocities of 10–6 rad s–1due to torques of 10–24 N m were measured for 340 nm crystals in a colloidal gel matrix. Furthermore these results show the ability to quantify small forces using rotation motion of tracer particles.
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
- OSTI Identifier:
- 1434566
- Alternate Identifier(s):
- OSTI ID: 1433986; OSTI ID: 1466355
- Report Number(s):
- BNL-203527-2018-JAAM
Journal ID: ISSN 1600-5775; JSYRES; PII: S1600577518005039
- Grant/Contract Number:
- AC02-06CH11357; SC00112704; SC0012704
- Resource Type:
- Published Article
- Journal Name:
- Journal of Synchrotron Radiation (Online)
- Additional Journal Information:
- Journal Name: Journal of Synchrotron Radiation (Online) Journal Volume: 25 Journal Issue: 3; Journal ID: ISSN 1600-5775
- Publisher:
- International Union of Crystallography (IUCr)
- Country of Publication:
- Denmark
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; rotational X-ray tracking; radiation pressure; rotational dynamics; rotational x-ray tracking
Citation Formats
Liang, Mengning, Harder, Ross, and Robinson, Ian. Radiation-driven rotational motion of nanoparticles. Denmark: N. p., 2018.
Web. doi:10.1107/S1600577518005039.
Liang, Mengning, Harder, Ross, & Robinson, Ian. Radiation-driven rotational motion of nanoparticles. Denmark. https://doi.org/10.1107/S1600577518005039
Liang, Mengning, Harder, Ross, and Robinson, Ian. Wed .
"Radiation-driven rotational motion of nanoparticles". Denmark. https://doi.org/10.1107/S1600577518005039.
@article{osti_1434566,
title = {Radiation-driven rotational motion of nanoparticles},
author = {Liang, Mengning and Harder, Ross and Robinson, Ian},
abstractNote = {Focused synchrotron beams can influence a studied sampleviaheating, or radiation pressure effects due to intensity gradients. The high angular sensitivity of rotational X-ray tracking of crystalline particlesviatheir Bragg reflections can detect extremely small forces such as those caused by field gradients. By tracking the rotational motion of single-crystal nanoparticles embedded in a viscous or viscoelastic medium, the effects of heating in a uniform gradient beam and radiation pressure in a Gaussian profile beam were observed. Changes in viscosity due to X-ray heating were measured for 42 µm crystals in glycerol, and angular velocities of 10–6 rad s–1due to torques of 10–24 N m were measured for 340 nm crystals in a colloidal gel matrix. Furthermore these results show the ability to quantify small forces using rotation motion of tracer particles.},
doi = {10.1107/S1600577518005039},
journal = {Journal of Synchrotron Radiation (Online)},
number = 3,
volume = 25,
place = {Denmark},
year = {2018},
month = {4}
}
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https://doi.org/10.1107/S1600577518005039
https://doi.org/10.1107/S1600577518005039
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