Phase separation and large deviations of lattice active matter
Abstract
Off-lattice active Brownian particles form clusters and undergo phase separation even in the absence of attractions or velocity-alignment mechanisms. Arguments that explain this phenomenon appeal only to the ability of particles to move persistently in a direction that fluctuates, but existing lattice models of hard particles that account for this behavior do not exhibit phase separation. Here we present a lattice model of active matter that exhibits motility-induced phase separation in the absence of velocity alignment. Using direct and rare-event sampling of dynamical trajectories, we show that clustering and phase separation are accompanied by pronounced fluctuations of static and dynamic order parameters. In conclusion, this model provides a complement to off-lattice models for the study of motility-induced phase separation.
- Authors:
-
[2];
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Univ. of California, Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1462977
- Alternate Identifier(s):
- OSTI ID: 1434178
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Chemical Physics
- Additional Journal Information:
- Journal Volume: 148; Journal Issue: 15; Related Information: © 2018 Author(s).; Journal ID: ISSN 0021-9606
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Whitelam, Stephen, Klymko, Katherine, and Mandal, Dibyendu. Phase separation and large deviations of lattice active matter. United States: N. p., 2018.
Web. doi:10.1063/1.5023403.
Whitelam, Stephen, Klymko, Katherine, & Mandal, Dibyendu. Phase separation and large deviations of lattice active matter. United States. https://doi.org/10.1063/1.5023403
Whitelam, Stephen, Klymko, Katherine, and Mandal, Dibyendu. Fri .
"Phase separation and large deviations of lattice active matter". United States. https://doi.org/10.1063/1.5023403. https://www.osti.gov/servlets/purl/1462977.
@article{osti_1462977,
title = {Phase separation and large deviations of lattice active matter},
author = {Whitelam, Stephen and Klymko, Katherine and Mandal, Dibyendu},
abstractNote = {Off-lattice active Brownian particles form clusters and undergo phase separation even in the absence of attractions or velocity-alignment mechanisms. Arguments that explain this phenomenon appeal only to the ability of particles to move persistently in a direction that fluctuates, but existing lattice models of hard particles that account for this behavior do not exhibit phase separation. Here we present a lattice model of active matter that exhibits motility-induced phase separation in the absence of velocity alignment. Using direct and rare-event sampling of dynamical trajectories, we show that clustering and phase separation are accompanied by pronounced fluctuations of static and dynamic order parameters. In conclusion, this model provides a complement to off-lattice models for the study of motility-induced phase separation.},
doi = {10.1063/1.5023403},
journal = {Journal of Chemical Physics},
number = 15,
volume = 148,
place = {United States},
year = {Fri Apr 20 00:00:00 EDT 2018},
month = {Fri Apr 20 00:00:00 EDT 2018}
}
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FIG. 1.: (a) Rates for the motion of isolated lattice-based active particles (particles may not move to an occupied site), and the color scheme used in pictures: particles that point toward nearest-neighbor particles are shown in red, and those that do not are shown in blue. (b) Time-ordered configurations formore »
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