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Title: Insight into selectivity: uptake studies of radionuclides 90 Sr 2+ , 137 Cs + , and 233 UO 2 2+ with bis-amidoxime polymers

Density functional theory and separation experiments combine to demonstrate the selectivity of bis-amidoxime polymer for uranyl extraction from aqueous solution.
Authors:
ORCiD logo [1] ;  [2] ; ORCiD logo [2]
  1. Chemical Sciences and Engineering Division, Argonne National Laboratory, Argonne, USA, Department of Chemistry
  2. Chemical Sciences and Engineering Division, Argonne National Laboratory, Argonne, USA
Publication Date:
Grant/Contract Number:
AC02-06CH11357
Type:
Publisher's Accepted Manuscript
Journal Name:
Dalton Transactions
Additional Journal Information:
Journal Name: Dalton Transactions Journal Volume: 47 Journal Issue: 15; Journal ID: ISSN 1477-9226
Publisher:
Royal Society of Chemistry (RSC)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United Kingdom
Language:
English
OSTI Identifier:
1434157

Piechowicz, Marek, Chiarizia, R., and Soderholm, L.. Insight into selectivity: uptake studies of radionuclides 90 Sr 2+ , 137 Cs + , and 233 UO 2 2+ with bis-amidoxime polymers. United Kingdom: N. p., Web. doi:10.1039/C7DT04935H.
Piechowicz, Marek, Chiarizia, R., & Soderholm, L.. Insight into selectivity: uptake studies of radionuclides 90 Sr 2+ , 137 Cs + , and 233 UO 2 2+ with bis-amidoxime polymers. United Kingdom. doi:10.1039/C7DT04935H.
Piechowicz, Marek, Chiarizia, R., and Soderholm, L.. 2018. "Insight into selectivity: uptake studies of radionuclides 90 Sr 2+ , 137 Cs + , and 233 UO 2 2+ with bis-amidoxime polymers". United Kingdom. doi:10.1039/C7DT04935H.
@article{osti_1434157,
title = {Insight into selectivity: uptake studies of radionuclides 90 Sr 2+ , 137 Cs + , and 233 UO 2 2+ with bis-amidoxime polymers},
author = {Piechowicz, Marek and Chiarizia, R. and Soderholm, L.},
abstractNote = {Density functional theory and separation experiments combine to demonstrate the selectivity of bis-amidoxime polymer for uranyl extraction from aqueous solution.},
doi = {10.1039/C7DT04935H},
journal = {Dalton Transactions},
number = 15,
volume = 47,
place = {United Kingdom},
year = {2018},
month = {1}
}

Works referenced in this record:

Density‚Äźfunctional thermochemistry. III. The role of exact exchange
journal, April 1993
  • Becke, Axel D.
  • The Journal of Chemical Physics, Vol. 98, Issue 7, p. 5648-5652
  • DOI: 10.1063/1.464913