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Title: Synthesis and radiometric evaluation of diglycolamide functionalized mesoporous silica for the chromatographic separation of actinides Th, Pa and U

Grafting of DGA on mesoporous silica affords a sorbent with the potential to separate U from Pa and Th.
Authors:
 [1] ;  [1] ; ORCiD logo [2] ;  [3] ;  [1] ;  [1] ;  [1] ; ORCiD logo [1] ; ORCiD logo [2] ; ORCiD logo [1]
  1. Chemistry Division, Los Alamos National Laboratory, Los Alamos, USA
  2. Faculty of Chemistry, Department of Inorganic Chemistry - Functional Materials, University of Vienna, 1090 Wien, Austria
  3. Nuclear Security and Isotope Technology Division, Oak Ridge National Laboratory, Oak Ridge, USA
Publication Date:
Grant/Contract Number:
FOA LAB 14-1099
Type:
Publisher's Accepted Manuscript
Journal Name:
Dalton Transactions
Additional Journal Information:
Journal Name: Dalton Transactions Journal Volume: 47 Journal Issue: 15; Journal ID: ISSN 1477-9226
Publisher:
Royal Society of Chemistry (RSC)
Sponsoring Org:
USDOE
Country of Publication:
United Kingdom
Language:
English
OSTI Identifier:
1434126

Hopkins, Philip D., Mastren, Tara, Florek, Justyna, Copping, Roy, Brugh, Mark, John, Kevin D., Nortier, Meiring F., Birnbaum, Eva R., Kleitz, Freddy, and Fassbender, Michael E.. Synthesis and radiometric evaluation of diglycolamide functionalized mesoporous silica for the chromatographic separation of actinides Th, Pa and U. United Kingdom: N. p., Web. doi:10.1039/C8DT00404H.
Hopkins, Philip D., Mastren, Tara, Florek, Justyna, Copping, Roy, Brugh, Mark, John, Kevin D., Nortier, Meiring F., Birnbaum, Eva R., Kleitz, Freddy, & Fassbender, Michael E.. Synthesis and radiometric evaluation of diglycolamide functionalized mesoporous silica for the chromatographic separation of actinides Th, Pa and U. United Kingdom. doi:10.1039/C8DT00404H.
Hopkins, Philip D., Mastren, Tara, Florek, Justyna, Copping, Roy, Brugh, Mark, John, Kevin D., Nortier, Meiring F., Birnbaum, Eva R., Kleitz, Freddy, and Fassbender, Michael E.. 2018. "Synthesis and radiometric evaluation of diglycolamide functionalized mesoporous silica for the chromatographic separation of actinides Th, Pa and U". United Kingdom. doi:10.1039/C8DT00404H.
@article{osti_1434126,
title = {Synthesis and radiometric evaluation of diglycolamide functionalized mesoporous silica for the chromatographic separation of actinides Th, Pa and U},
author = {Hopkins, Philip D. and Mastren, Tara and Florek, Justyna and Copping, Roy and Brugh, Mark and John, Kevin D. and Nortier, Meiring F. and Birnbaum, Eva R. and Kleitz, Freddy and Fassbender, Michael E.},
abstractNote = {Grafting of DGA on mesoporous silica affords a sorbent with the potential to separate U from Pa and Th.},
doi = {10.1039/C8DT00404H},
journal = {Dalton Transactions},
number = 15,
volume = 47,
place = {United Kingdom},
year = {2018},
month = {1}
}

Works referenced in this record:

Adsorption of Gases in Multimolecular Layers
journal, February 1938
  • Brunauer, Stephen; Emmett, P. H.; Teller, Edward
  • Journal of the American Chemical Society, Vol. 60, Issue 2, p. 309-319
  • DOI: 10.1021/ja01269a023

Application of ion exchange and extraction chromatography to the separation of actinium from proton-irradiated thorium metal for analytical purposes
journal, February 2015