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Title: Measuring the shock impedance mismatch between high-density carbon and deuterium at the National Ignition Facility

Abstract

Fine-grained diamond, or high-density carbon (HDC), is being used as an ablator for inertial confinement fusion (ICF) research at the National Ignition Facility (NIF). Accurate equation of state (EOS) knowledge over a wide range of phase space is critical in the design and analysis of integrated ICF experiments. Here in this paper, we report shock and release measurements of the shock impedance mismatch between HDC and liquid deuterium conducted during shock-timing experiments having a first shock in the ablator ranging between 8 and 14 Mbar. Using ultrafast Doppler imaging velocimetry to track the leading shock front, we characterize the shock velocity discontinuity upon the arrival of the shock at the HDC/liquid deuterium interface. Comparing the experimental data with tabular EOS models used to simulate integrated ICF experiments indicates the need for an improved multiphase EOS model for HDC in order to achieve a significant increase in neutron yield in indirect-driven ICF implosions with HDC ablators.

Authors:
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [2];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1] more »;  [1];  [1];  [3];  [1];  [3];  [4];  [1] « less
  1. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  2. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of Rochester, NY (United States). Lab. for Laser Energetics; Univ. of Rochester, NY (United States). Dept. of Mechanical Engineering, and Physics and Astronomy
  3. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of Rochester, NY (United States). Lab. for Laser Energetics
  4. Diamond Materials GmbH, Freiburg (Germany)
Publication Date:
Research Org.:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1455401
Alternate Identifier(s):
OSTI ID: 1433577
Report Number(s):
LLNL-JRNL-740027
Journal ID: ISSN 2469-9950; PRBMDO; 892349; TRN: US1901231
Grant/Contract Number:  
AC52-07NA27344
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 97; Journal Issue: 14; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION TECHNOLOGY; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Millot, M., Celliers, P. M., Sterne, P. A., Benedict, L. X., Correa, A. A., Hamel, S., Ali, S. J., Baker, K. L., Berzak Hopkins, L. F., Biener, J., Collins, G. W., Coppari, F., Divol, L., Fernandez-Panella, A., Fratanduono, D. E., Haan, S. W., Le Pape, S., Meezan, N. B., Moore, A. S., Moody, J. D., Ralph, J. E., Ross, J. S., Rygg, J. R., Thomas, C., Turnbull, D. P., Wild, C., and Eggert, J. H. Measuring the shock impedance mismatch between high-density carbon and deuterium at the National Ignition Facility. United States: N. p., 2018. Web. doi:10.1103/PhysRevB.97.144108.
Millot, M., Celliers, P. M., Sterne, P. A., Benedict, L. X., Correa, A. A., Hamel, S., Ali, S. J., Baker, K. L., Berzak Hopkins, L. F., Biener, J., Collins, G. W., Coppari, F., Divol, L., Fernandez-Panella, A., Fratanduono, D. E., Haan, S. W., Le Pape, S., Meezan, N. B., Moore, A. S., Moody, J. D., Ralph, J. E., Ross, J. S., Rygg, J. R., Thomas, C., Turnbull, D. P., Wild, C., & Eggert, J. H. Measuring the shock impedance mismatch between high-density carbon and deuterium at the National Ignition Facility. United States. https://doi.org/10.1103/PhysRevB.97.144108
Millot, M., Celliers, P. M., Sterne, P. A., Benedict, L. X., Correa, A. A., Hamel, S., Ali, S. J., Baker, K. L., Berzak Hopkins, L. F., Biener, J., Collins, G. W., Coppari, F., Divol, L., Fernandez-Panella, A., Fratanduono, D. E., Haan, S. W., Le Pape, S., Meezan, N. B., Moore, A. S., Moody, J. D., Ralph, J. E., Ross, J. S., Rygg, J. R., Thomas, C., Turnbull, D. P., Wild, C., and Eggert, J. H. Wed . "Measuring the shock impedance mismatch between high-density carbon and deuterium at the National Ignition Facility". United States. https://doi.org/10.1103/PhysRevB.97.144108. https://www.osti.gov/servlets/purl/1455401.
@article{osti_1455401,
title = {Measuring the shock impedance mismatch between high-density carbon and deuterium at the National Ignition Facility},
author = {Millot, M. and Celliers, P. M. and Sterne, P. A. and Benedict, L. X. and Correa, A. A. and Hamel, S. and Ali, S. J. and Baker, K. L. and Berzak Hopkins, L. F. and Biener, J. and Collins, G. W. and Coppari, F. and Divol, L. and Fernandez-Panella, A. and Fratanduono, D. E. and Haan, S. W. and Le Pape, S. and Meezan, N. B. and Moore, A. S. and Moody, J. D. and Ralph, J. E. and Ross, J. S. and Rygg, J. R. and Thomas, C. and Turnbull, D. P. and Wild, C. and Eggert, J. H.},
abstractNote = {Fine-grained diamond, or high-density carbon (HDC), is being used as an ablator for inertial confinement fusion (ICF) research at the National Ignition Facility (NIF). Accurate equation of state (EOS) knowledge over a wide range of phase space is critical in the design and analysis of integrated ICF experiments. Here in this paper, we report shock and release measurements of the shock impedance mismatch between HDC and liquid deuterium conducted during shock-timing experiments having a first shock in the ablator ranging between 8 and 14 Mbar. Using ultrafast Doppler imaging velocimetry to track the leading shock front, we characterize the shock velocity discontinuity upon the arrival of the shock at the HDC/liquid deuterium interface. Comparing the experimental data with tabular EOS models used to simulate integrated ICF experiments indicates the need for an improved multiphase EOS model for HDC in order to achieve a significant increase in neutron yield in indirect-driven ICF implosions with HDC ablators.},
doi = {10.1103/PhysRevB.97.144108},
journal = {Physical Review B},
number = 14,
volume = 97,
place = {United States},
year = {Wed Apr 18 00:00:00 EDT 2018},
month = {Wed Apr 18 00:00:00 EDT 2018}
}

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Works referenced in this record:

High-Precision Shock Wave Measurements of Deuterium: Evaluation of Exchange-Correlation Functionals at the Molecular-to-Atomic Transition
journal, January 2017


Line-imaging velocimeter for shock diagnostics at the OMEGA laser facility
journal, November 2004

  • Celliers, P. M.; Bradley, D. K.; Collins, G. W.
  • Review of Scientific Instruments, Vol. 75, Issue 11
  • DOI: 10.1063/1.1807008

Early time implosion symmetry from two-axis shock-timing measurements on indirect drive NIF experiments
journal, September 2014

  • Moody, J. D.; Robey, H. F.; Celliers, P. M.
  • Physics of Plasmas, Vol. 21, Issue 9
  • DOI: 10.1063/1.4893136

Raman Studies of Nano- and Ultra-nanocrystalline Diamond Films Grown by Hot-Filament CVD
journal, June 2010

  • Klauser, Frederik; Steinmüller-Nethl, Doris; Kaindl, Reinhard
  • Chemical Vapor Deposition, Vol. 16, Issue 4-6
  • DOI: 10.1002/cvde.200906827

First High-Convergence Cryogenic Implosion in a Near-Vacuum Hohlraum
journal, April 2015


Grain size dependent physical and chemical properties of thick CVD diamond films for high energy density physics experiments
journal, November 2013


Refractive index of lithium fluoride ramp compressed to 800 GPa
journal, June 2011

  • Fratanduono, D. E.; Boehly, T. R.; Barrios, M. A.
  • Journal of Applied Physics, Vol. 109, Issue 12
  • DOI: 10.1063/1.3599884

Shock-Wave Exploration of the High-Pressure Phases of Carbon
journal, December 2008


Ramp compression of diamond to five terapascals
journal, July 2014

  • Smith, R. F.; Eggert, J. H.; Jeanloz, R.
  • Nature, Vol. 511, Issue 7509
  • DOI: 10.1038/nature13526

Systematic uncertainties in shock-wave impedance-match analysis and the high-pressure equation of state of Al
journal, December 2005

  • Celliers, P. M.; Collins, G. W.; Hicks, D. G.
  • Journal of Applied Physics, Vol. 98, Issue 11
  • DOI: 10.1063/1.2140077

First-principles multiphase equation of state of carbon under extreme conditions
journal, July 2008


High-density carbon ablator experiments on the National Ignition Facility
journal, May 2014

  • MacKinnon, A. J.; Meezan, N. B.; Ross, J. S.
  • Physics of Plasmas, Vol. 21, Issue 5
  • DOI: 10.1063/1.4876611

High-density carbon capsule experiments on the national ignition facility
journal, February 2015


Melting temperature of diamond at ultrahigh pressure
journal, November 2009

  • Eggert, J. H.; Hicks, D. G.; Celliers, P. M.
  • Nature Physics, Vol. 6, Issue 1
  • DOI: 10.1038/nphys1438

Generation and Beaming of Early Hot Electrons onto the Capsule in Laser-Driven Ignition Hohlraums
journal, February 2016


Temperature dependence of the refractive index of diamond up to 925 K
journal, December 2000


Optical constants and thermo-optic coefficients of nanocrystalline diamond films at 30–500°C
journal, August 2006

  • Hu, Z. G.; Hess, P.
  • Applied Physics Letters, Vol. 89, Issue 8
  • DOI: 10.1063/1.2243863

Growth of nanocrystalline diamond films deposited by microwave plasma CVD system at low substrate temperatures
journal, September 2006

  • Potocky, S.; Kromka, A.; Potmesil, J.
  • physica status solidi (a), Vol. 203, Issue 12
  • DOI: 10.1002/pssa.200671110

Strength effects in diamond under shock compression from 0.1 to 1 TPa
journal, January 2010


Laser-driven single shock compression of fluid deuterium from 45 to 220 GPa
journal, January 2009


Precision Shock Tuning on the National Ignition Facility
journal, May 2012


Equation of state of CH 1.36 : First-principles molecular dynamics simulations and shock-and-release wave speed measurements
journal, September 2012


Diamond spheres for inertial confinement fusion
journal, September 2009


Extended data set for the equation of state of warm dense hydrogen isotopes
journal, October 2012


Laser-shock compression of diamond and evidence of a negative-slope melting curve
journal, March 2007

  • Brygoo, Stéphanie; Henry, Emeric; Loubeyre, Paul
  • Nature Materials, Vol. 6, Issue 4
  • DOI: 10.1038/nmat1863

Shock Compressing Diamond to a Conducting Fluid
journal, November 2004


Analysis of laser shock experiments on precompressed samples using a quartz reference and application to warm dense hydrogen and helium
journal, November 2015

  • Brygoo, Stephanie; Millot, Marius; Loubeyre, Paul
  • Journal of Applied Physics, Vol. 118, Issue 19
  • DOI: 10.1063/1.4935295

Cryogenic tritium-hydrogen-deuterium and deuterium-tritium layer implosions with high density carbon ablators in near-vacuum hohlraums
journal, June 2015

  • Meezan, N. B.; Berzak Hopkins, L. F.; Le Pape, S.
  • Physics of Plasmas, Vol. 22, Issue 6
  • DOI: 10.1063/1.4921947

Carbon under extreme conditions: Phase boundaries and electronic properties from first-principles theory
journal, January 2006

  • Correa, A. A.; Bonev, S. A.; Galli, G.
  • Proceedings of the National Academy of Sciences, Vol. 103, Issue 5
  • DOI: 10.1073/pnas.0510489103

Shock timing measurements and analysis in deuterium-tritium-ice layered capsule implosions on NIF
journal, February 2014

  • Robey, H. F.; Celliers, P. M.; Moody, J. D.
  • Physics of Plasmas, Vol. 21, Issue 2
  • DOI: 10.1063/1.4863975

Hugoniot and release measurements in diamond shocked up to 26 Mbar
journal, April 2017


High-precision measurements of the diamond Hugoniot in and above the melt region
journal, November 2008


Experimental evidence for a phase transition in magnesium oxide at exoplanet pressures
journal, September 2013

  • Coppari, F.; Smith, R. F.; Eggert, J. H.
  • Nature Geoscience, Vol. 6, Issue 11
  • DOI: 10.1038/ngeo1948

Shock compression of stishovite and melting of silica at planetary interior conditions
journal, January 2015


�ber Brechungsindizes und Absorptionskonstanten des Diamanten zwischen 644 und 226 m?
journal, December 1923


Multiphase equation of state for carbon addressing high pressures and temperatures
journal, June 2014


Shock timing experiments on the National Ignition Facility: Initial results and comparison with simulation
journal, April 2012

  • Robey, H. F.; Boehly, T. R.; Celliers, P. M.
  • Physics of Plasmas, Vol. 19, Issue 4
  • DOI: 10.1063/1.3694122

Near-vacuum hohlraums for driving fusion implosions with high density carbon ablatorsa)
journal, May 2015

  • Berzak Hopkins, L. F.; Le Pape, S.; Divol, L.
  • Physics of Plasmas, Vol. 22, Issue 5
  • DOI: 10.1063/1.4921151

Optical properties of nanocrystalline diamond films from mid-infrared to ultraviolet using reflectometry and ellipsometry
journal, March 2007

  • Hu, Z. G.; Prunici, P.; Hess, P.
  • Journal of Materials Science: Materials in Electronics, Vol. 18, Issue S1
  • DOI: 10.1007/s10854-007-9175-y

Temperature and pressure variation of the refractive index of diamond
journal, January 1977

  • Fontanella, John; Johnston, Richard L.; Colwell, Jack H.
  • Applied Optics, Vol. 16, Issue 11
  • DOI: 10.1364/AO.16.002949

Symmetry control of an indirectly driven high-density-carbon implosion at high convergence and high velocity
journal, May 2017

  • Divol, L.; Pak, A.; Berzak Hopkins, L. F.
  • Physics of Plasmas, Vol. 24, Issue 5
  • DOI: 10.1063/1.4982215

Multiphase equation of state of hydrogen from ab initio calculations in the range 0.2 to 5 g/cc up to 10 eV
journal, March 2011


X-ray preheating of window materials in direct-drive shock-wave timing experiments
journal, December 2006

  • Theobald, W.; Miller, J. E.; Boehly, T. R.
  • Physics of Plasmas, Vol. 13, Issue 12
  • DOI: 10.1063/1.2397581

Hugoniot measurement of diamond under laser shock compression up to 2TPa
journal, May 2006

  • Nagao, H.; Nakamura, K. G.; Kondo, K.
  • Physics of Plasmas, Vol. 13, Issue 5
  • DOI: 10.1063/1.2205194

Examining the radiation drive asymmetries present in the high foot series of implosion experiments at the National Ignition Facility
journal, May 2017

  • Pak, A.; Divol, L.; Kritcher, A. L.
  • Physics of Plasmas, Vol. 24, Issue 5
  • DOI: 10.1063/1.4979192

Works referencing / citing this record:

Three-dimensional modeling and hydrodynamic scaling of National Ignition Facility implosions
journal, May 2019

  • Clark, D. S.; Weber, C. R.; Milovich, J. L.
  • Physics of Plasmas, Vol. 26, Issue 5
  • DOI: 10.1063/1.5091449