Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in LaBr 3 and LaBr 3 :Ce

Li, Peiyun; Gridin, Sergii; Ucer, K. Burak; Williams, Richard T.; Menge, Peter R.

doi:10.1103/PhysRevB.97.144303

Title: Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in ${LaBr}_{3}$ and ${LaBr}_{3}$ :Ce

Authors:: Li, Peiyun; Gridin, Sergii; Ucer, K. Burak; Williams, Richard T.; Menge, Peter R.

Publication Date:: 2018-04-18

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA)

OSTI Identifier:: 1433567

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Name: Physical Review B Journal Volume: 97 Journal Issue: 14; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Li, Peiyun, Gridin, Sergii, Ucer, K. Burak, Williams, Richard T., and Menge, Peter R. Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in LaBr 3 and LaBr 3 :Ce.  United States: N. p., 2018. 
Web.  doi:10.1103/PhysRevB.97.144303.

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                    Li, Peiyun, Gridin, Sergii, Ucer, K. Burak, Williams, Richard T., & Menge, Peter R. Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in LaBr 3 and LaBr 3 :Ce.  United States.  https://doi.org/10.1103/PhysRevB.97.144303

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                    Li, Peiyun, Gridin, Sergii, Ucer, K. Burak, Williams, Richard T., and Menge, Peter R. Wed .  
"Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in LaBr 3 and LaBr 3 :Ce".  United States.  https://doi.org/10.1103/PhysRevB.97.144303.

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@article{osti_1433567,

  title        = {Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in LaBr 3 and LaBr 3 :Ce},

  author       = {Li, Peiyun and Gridin, Sergii and Ucer, K. Burak and Williams, Richard T. and Menge, Peter R.},

  abstractNote = {},

  doi          = {10.1103/PhysRevB.97.144303},

  journal      = {Physical Review B},

  number       = 14,

  volume       = 97,

  place        = {United States},

  year         = {2018},

  month        = {4}

}

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https://doi.org/10.1103/PhysRevB.97.144303

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Title: Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in LaBr 3 and LaBr 3 :Ce

Citation Formats

Energy-Dependent Scintillation Pulse Shape and Proportionality of Decay Components for CsI:Tl: Modeling with Transport and Rate Equations journal, January 2017

Luminescence of LaBr 3 :Ce,Hf scintillation crystals under UV-VUV and X-ray excitation journal, December 2013

Electron Spin Resonance of V 1 -Centers journal, September 1955

Lanthanide 4f-electron binding energies and the nephelauxetic effect in wide band gap compounds journal, April 2013

High-energy-resolution scintillator: Ce3+ activated LaBr3 journal, September 2001

Luminescence and scintillation properties of the small band gap compound LaI3:Ce3+ journal, January 2005

Kinetics of Self-Trapped Holes in Alkali-Halide Crystals: Experiments in NaI(Tl) and KI(Tl) journal, December 1973

Investigation of the PGNAA using the LaBr3 scintillation detector journal, April 2010

The scintillation mechanism in LaCl 3 :Ce 3 journal, February 2003

Short-pulse optical studies of exciton relaxation and F -center formation in NaCl, KCl, and NaBr journal, December 1978

Fundamental Limitations in the Performance of ${\rm Ce}^{3+}$–, ${\rm Pr}^{3+}$–, and ${\rm Eu}^{2+}$–Activated Scintillators journal, June 2010

Transient absorption due to self-trapped excitons in NaBr and NaI journal, March 1993

Magnetic resonance investigations of LaCl 3 :Ce 3+ scintillators journal, January 2002

Improvement of LaBr 3 :5%Ce scintillation properties by Li + , Na + , Mg 2+ , Ca 2+ , Sr 2+ , and Ba 2+ co-doping journal, June 2013

Decay time measurements of intrinsic luminescence in alkali halides using single-bunched light pulses from UVSOR journal, January 1990

Excited-state absorption spectroscopy of self-trapped excitons in alkali halides journal, February 1974

Subpicosecond spectroscopy of hole and exciton self-trapping in alkali-halide crystals journal, October 1997

Theory of the Self-Trapped Hole in the Alkali Halides journal, August 1969

Effects of Ce concentration on scintillation properties of LaBr/sub 3/:Ce journal, October 2005

Electron thermalization and trapping rates in pure and doped alkali and alkaline-earth iodide crystals studied by picosecond optical absorption journal, April 2014

Comparative Study of Nonproportionality and Electronic Band Structures Features in Scintillator Materials journal, October 2009

Time-resolved spectroscopy of self-trapped excitons in fluorite crystals journal, July 1976

Absorption Spectra of F 2 − , Cl 2 − , Br 2 − , and I 2 − in the Alkali Halides journal, February 1961

The electronic level structure of lanthanide impurities in REPO 4 , REBO 3 , REAlO 3 , and RE 2 O 3 (RE = La, Gd, Y, Lu, Sc) compounds journal, May 2013

Electronic structure of LaBr 3 from quasiparticle self-consistent G W calculations journal, March 2012

A Theory of Sensitized Luminescence in Solids journal, May 1953

Relaxation of the 2s Hot Excitons in Alkali Iodides journal, September 1983

First-principles search for efficient activators for LaI3 journal, August 2016

From Luminescence Non-Linearity to Scintillation Non-Proportionality journal, June 2008

Off-center self-trapped excitons and creation of lattice defects in alkali halide crystals journal, May 1986

ENDOR of the self-trapped exciton in KCl journal, October 1978

Optical Absorption and X-Ray Photoemission Spectra of Lanthanum and Cerium Halides journal, September 1976

The Self-trapped Hole in CaF 2 journal, June 1962

Origin of the 4.1-eV luminescence in pure CsI scintillator journal, January 1995

Coupled rate and transport equations modeling proportionality of light yield in high-energy electron tracks: CsI at 295 K and 100 K; CsI:Tl at 295 K journal, September 2015

Design of a lanthanum bromide detector for time-of-flight PET journal, October 2004

Resonance Luminescence Lines of Free Excitons in Alkali Iodide Single Crystals journal, July 1977

Evidence and Consequences of Ce$^{4+}$ in LYSO:Ce,Ca and LYSO:Ce,Mg Single Crystals for Medical Imaging Applications journal, August 2013

Level location and spectroscopy of , , , and in journal, April 2006

Charge carrier and exciton dynamics in LaBr 3 : Ce 3 + scintillators: Experiment and model journal, May 2007

Title: Picosecond absorption spectroscopy of self-trapped excitons and transient Ce states in ${LaBr}_{3}$ and ${LaBr}_{3}$ :Ce

Energy-Dependent Scintillation Pulse Shape and Proportionality of Decay Components for CsI:Tl: Modeling with Transport and Rate Equations
journal, January 2017

Luminescence of LaBr ₃ :Ce,Hf scintillation crystals under UV-VUV and X-ray excitation
journal, December 2013

Electron Spin Resonance of $V_{1}$ -Centers
journal, September 1955

Lanthanide 4f-electron binding energies and the nephelauxetic effect in wide band gap compounds
journal, April 2013

High-energy-resolution scintillator: Ce³⁺ activated LaBr₃
journal, September 2001

Luminescence and scintillation properties of the small band gap compound LaI₃:Ce³⁺
journal, January 2005

Kinetics of Self-Trapped Holes in Alkali-Halide Crystals: Experiments in NaI(Tl) and KI(Tl)
journal, December 1973

Investigation of the PGNAA using the LaBr3 scintillation detector
journal, April 2010

The scintillation mechanism in LaCl ₃ :Ce ³
journal, February 2003

Short-pulse optical studies of exciton relaxation and $F$ -center formation in NaCl, KCl, and NaBr
journal, December 1978

Fundamental Limitations in the Performance of ${\rm Ce}^{3+}$–, ${\rm Pr}^{3+}$–, and ${\rm Eu}^{2+}$–Activated Scintillators
journal, June 2010

Transient absorption due to self-trapped excitons in NaBr and NaI
journal, March 1993

Magnetic resonance investigations of LaCl 3 :Ce 3+ scintillators
journal, January 2002

Improvement of LaBr ₃ :5%Ce scintillation properties by Li ⁺ , Na ⁺ , Mg ²⁺ , Ca ²⁺ , Sr ²⁺ , and Ba ²⁺ co-doping
journal, June 2013

Decay time measurements of intrinsic luminescence in alkali halides using single-bunched light pulses from UVSOR
journal, January 1990

Excited-state absorption spectroscopy of self-trapped excitons in alkali halides
journal, February 1974

Subpicosecond spectroscopy of hole and exciton self-trapping in alkali-halide crystals
journal, October 1997

Theory of the Self-Trapped Hole in the Alkali Halides
journal, August 1969

Effects of Ce concentration on scintillation properties of LaBr/sub 3/:Ce
journal, October 2005

Electron thermalization and trapping rates in pure and doped alkali and alkaline-earth iodide crystals studied by picosecond optical absorption
journal, April 2014

Comparative Study of Nonproportionality and Electronic Band Structures Features in Scintillator Materials
journal, October 2009

Time-resolved spectroscopy of self-trapped excitons in fluorite crystals
journal, July 1976

Absorption Spectra of $F_{2}^{-}$ , ${Cl}_{2}^{-}$ , ${Br}_{2}^{-}$ , and $I_{2}^{-}$ in the Alkali Halides
journal, February 1961

The electronic level structure of lanthanide impurities in REPO ₄ , REBO ₃ , REAlO ₃ , and RE ₂ O ₃ (RE = La, Gd, Y, Lu, Sc) compounds
journal, May 2013

Electronic structure of LaBr $_{3}$ from quasiparticle self-consistent $G W$ calculations
journal, March 2012

A Theory of Sensitized Luminescence in Solids
journal, May 1953

Relaxation of the 2s Hot Excitons in Alkali Iodides
journal, September 1983

First-principles search for efficient activators for LaI3
journal, August 2016

From Luminescence Non-Linearity to Scintillation Non-Proportionality
journal, June 2008

Off-center self-trapped excitons and creation of lattice defects in alkali halide crystals
journal, May 1986

ENDOR of the self-trapped exciton in KCl
journal, October 1978

Optical Absorption and X-Ray Photoemission Spectra of Lanthanum and Cerium Halides
journal, September 1976

The Self-trapped Hole in CaF ₂
journal, June 1962

Origin of the 4.1-eV luminescence in pure CsI scintillator
journal, January 1995

Coupled rate and transport equations modeling proportionality of light yield in high-energy electron tracks: CsI at 295 K and 100 K; CsI:Tl at 295 K
journal, September 2015

Design of a lanthanum bromide detector for time-of-flight PET
journal, October 2004

Resonance Luminescence Lines of Free Excitons in Alkali Iodide Single Crystals
journal, July 1977

Evidence and Consequences of Ce$^{4+}$ in LYSO:Ce,Ca and LYSO:Ce,Mg Single Crystals for Medical Imaging Applications
journal, August 2013

Level location and spectroscopy of , , , and in
journal, April 2006

Charge carrier and exciton dynamics in ${LaBr}_{3} : {Ce}^{3 +}$ scintillators: Experiment and model
journal, May 2007