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Title: Dewetting in immiscible polymer bilayer films

 [1];  [2];  [3];  [4];  [5];  [6];  [7];  [8]
  1. Argonne National Lab. (ANL), Argonne, IL (United States). X-ray Science Division, and Intense Pulsed Neutron Source; Northern Illinois Univ., DeKalb, IL (United States). Dept. of Physics
  2. Argonne National Lab. (ANL), Argonne, IL (United States). Intense Pulsed Neutron Source
  3. Univ. of California, San Diego, CA (United States). Dept. of Physics
  4. Argonne National Lab. (ANL), Argonne, IL (United States). X-ray Science Division
  5. Brookhaven National Lab. (BNL), Upton, NY (United States). NSLS-II
  6. Argonne National Lab. (ANL), Argonne, IL (United States). Nanoscience and Technology Division
  7. Northern Illinois Univ., DeKalb, IL (United States). Dept. of Physics
  8. McGill Univ., Montreal, QC (Canada). Dept of Physics
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
Alternate Identifier(s):
OSTI ID: 1364220; OSTI ID: 1433945
Report Number(s):
Journal ID: ISSN 2475-9953; PRMHAR; 127301; TRN: US1802945
Grant/Contract Number:  
AC02-06CH11357; SC0012704
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Materials
Additional Journal Information:
Journal Volume: 1; Journal Issue: 1; Journal ID: ISSN 2475-9953
American Physical Society (APS)
Country of Publication:
United States

Citation Formats

Lal, J., Malkova, S., Mukhopadhyay, M. K., Narayanan, S., Fluerasu, A., Darling, S. B., Lurio, L. B., and Sutton, M. Dewetting in immiscible polymer bilayer films. United States: N. p., 2017. Web. doi:10.1103/PhysRevMaterials.1.015601.
Lal, J., Malkova, S., Mukhopadhyay, M. K., Narayanan, S., Fluerasu, A., Darling, S. B., Lurio, L. B., & Sutton, M. Dewetting in immiscible polymer bilayer films. United States. doi:10.1103/PhysRevMaterials.1.015601.
Lal, J., Malkova, S., Mukhopadhyay, M. K., Narayanan, S., Fluerasu, A., Darling, S. B., Lurio, L. B., and Sutton, M. Mon . "Dewetting in immiscible polymer bilayer films". United States. doi:10.1103/PhysRevMaterials.1.015601.
title = {Dewetting in immiscible polymer bilayer films},
author = {Lal, J. and Malkova, S. and Mukhopadhyay, M. K. and Narayanan, S. and Fluerasu, A. and Darling, S. B. and Lurio, L. B. and Sutton, M.},
abstractNote = {},
doi = {10.1103/PhysRevMaterials.1.015601},
journal = {Physical Review Materials},
number = 1,
volume = 1,
place = {United States},
year = {2017},
month = {6}

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Works referenced in this record:

Relaxation of Residual Stress and Reentanglement of Polymers in Spin-Coated Films
journal, July 2007

Final Stages of Spreading of Polymer Droplets on Smooth Solid Surfaces
journal, July 1988

The measurement of velocity gradients in laminar flow by homodyne light-scattering spectroscopy
journal, October 1980

  • Fuller, G. G.; Rallison, J. M.; Schmidt, R. L.
  • Journal of Fluid Mechanics, Vol. 100, Issue 03
  • DOI: 10.1017/S0022112080001280

Interface morphologies in liquid/liquid dewetting
journal, May 2011

  • Kostourou, Konstantina; Peschka, Dirk; Münch, Andreas
  • Chemical Engineering and Processing: Process Intensification, Vol. 50, Issue 5-6
  • DOI: 10.1016/j.cep.2010.10.006

Molecular layering in the spreading of wetting liquid drops
journal, April 1989

  • Heslot, F.; Fraysse, N.; Cazabat, A. M.
  • Nature, Vol. 338, Issue 6217
  • DOI: 10.1038/338640a0

Observation of nano-dewetting structures
journal, December 1997

  • Müller-Buschbaum, P.; Vanhoorne, P.; Scheumann, V.
  • Europhysics Letters (EPL), Vol. 40, Issue 6
  • DOI: 10.1209/epl/i1997-00519-4

Dewetting at the Liquid-Liquid Interface
journal, February 1996

Resonantly enhanced off-specular X-ray scattering from polymer/polymer interfaces⋆
journal, July 2005

Dewetting of Highly Elastic Thin Polymer Films
journal, October 2001

Dewetting of Supported Viscoelastic Polymer Films:  Birth of Rims
journal, February 1997

  • Brochard-Wyart, F.; Debregeas, G.; Fondecave, R.
  • Macromolecules, Vol. 30, Issue 4
  • DOI: 10.1021/ma960929x

Capillarity and Wetting Phenomena: Drops, Bubbles, Pearls, Waves
book, January 2004

Wetting: statics and dynamics
journal, July 1985

The spreading dynamics of a liquid drop on a viscoelastic solid
journal, June 1988

Dynamics of Rims and the Onset of Spinodal Dewetting at Liquid/Liquid Interfaces
journal, February 1999

  • Segalman, Rachel A.; Green, Peter F.
  • Macromolecules, Vol. 32, Issue 3
  • DOI: 10.1021/ma981208w

Using coherence to measure two-time correlation functions
journal, January 2003

  • Sutton, Mark; Laaziri, Khalid; Livet, F.
  • Optics Express, Vol. 11, Issue 19
  • DOI: 10.1364/OE.11.002268

Influence of chain interdiffusion between immiscible polymers on dewetting dynamics
journal, January 2011

  • Coppée, Séverine; Gabriele, Sylvain; Jonas, Alain M.
  • Soft Matter, Vol. 7, Issue 21
  • DOI: 10.1039/c1sm05486d

Dewetting of thin viscoelastic polymer films on slippery substrates
journal, December 2005

Residual stresses in thin polymer films cause rupture and dominate early stages of dewetting
journal, September 2005

  • Reiter, Günter; Hamieh, Moustafa; Damman, Pascal
  • Nature Materials, Vol. 4, Issue 10
  • DOI: 10.1038/nmat1484

Transient Cooperative Processes in Dewetting Polymer Melts
journal, February 2016

Dewetting of thin polymer films: Influence of interface evolution
journal, May 2009

Aging of Thin Polymer Films Cast from a Near-Theta Solvent
journal, November 2010

Reduced Interfacial Entanglement Density Affects the Boundary Conditions of Polymer Flow
journal, December 2009

Interfacial Instability Driven by Dispersive Forces: The Early Stages of Spinodal Dewetting of a Thin Polymer Film on a Polymer Substrate
journal, December 1998

Effect of an Interactive Surface on the Equilibrium Contact Angles in Bilayer Polymer Films
journal, March 2000

  • Slep, D.; Asselta, J.; Rafailovich, M. H.
  • Langmuir, Vol. 16, Issue 5
  • DOI: 10.1021/la990031b

Surface Tension and Surface Roughness of Supported Polystyrene Films
journal, July 2003

  • Lurio, Laurence; Kim, Hyunjung; Rühm, Adrian
  • Macromolecules, Vol. 36, Issue 15
  • DOI: 10.1021/ma034189l

Observation of a low-viscosity interface between immiscible polymer layers
journal, July 2006

Bulk and surface characterization of a dewetting thin film polymer bilayer
journal, December 1998

  • Ade, H.; Winesett, D. A.; Smith, A. P.
  • Applied Physics Letters, Vol. 73, Issue 25
  • DOI: 10.1063/1.122891

Dewetting near the Glass Transition: Transition from a Capillary Force Dominated to a Dissipation Dominated Regime
journal, November 2003

Liquid/liquid dewetting
journal, December 1993

  • Wyart, Francoise Brochard; Martin, Pascal; Redon, Claude
  • Langmuir, Vol. 9, Issue 12
  • DOI: 10.1021/la00036a053