Three-dimensional strain engineering in epitaxial vertically aligned nanocomposite thin films with tunable magnetotransport properties
Abstract
Three-dimensional (3D) frameworks have been successfully constructed by interlayering La0.7Sr0.3MnO3 (LSMO)–CeO2 based epitaxial vertically aligned nanocomposite (VAN) thin films with pure CeO2 (or LSMO) layers. Such 3D interconnected CeO2 scaffolds integrate the lateral film strain by the interlayers with the vertical strain in VAN layers, and thus achieve the maximized strain tuning in LSMO. More importantly, by varying the types of the interlayers (i.e., CeO2 or LSMO) and the number of interlayers from 1 to 3 layers, such 3D framework nanostructures effectively tune the electrical transport properties of LSMO, e.g., from a 3D insulating CeO2 framework with integrated magnetic tunnel junction structures, to a 3D conducting LSMO framework, where the magnetoresistance (MR) peak values have been tuned systematically to a record high of 66% at 56 K and enhanced MR properties at high temperatures above room temperature (~325 K). This new 3D framed design provides a novel approach in maximizing film strain, enhancing strain-driven functionalities, and manipulating the electrical transport properties effectively.
- Authors:
-
- School of Materials Engineering, Purdue University, West Lafayette, USA
- Department of Materials Science and Metallurgy, University of Cambridge, Cambridge, UK
- Sandia National Laboratories, Albuquerque, USA
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1432400
- Alternate Identifier(s):
- OSTI ID: 1477313
- Report Number(s):
- SAND-2018-10376J
Journal ID: ISSN 2051-6347; MHAOAL
- Grant/Contract Number:
- AC02-05CH11231; AC04-94AL85000
- Resource Type:
- Published Article
- Journal Name:
- Materials Horizons
- Additional Journal Information:
- Journal Name: Materials Horizons Journal Volume: 5 Journal Issue: 3; Journal ID: ISSN 2051-6347
- Publisher:
- Royal Society of Chemistry (RSC)
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Sun, Xing, Huang, Jijie, Jian, Jie, Fan, Meng, Wang, Han, Li, Qiang, Mac Manus-Driscoll, Judith L., Lu, Ping, Zhang, Xinghang, and Wang, Haiyan. Three-dimensional strain engineering in epitaxial vertically aligned nanocomposite thin films with tunable magnetotransport properties. United Kingdom: N. p., 2018.
Web. doi:10.1039/C8MH00216A.
Sun, Xing, Huang, Jijie, Jian, Jie, Fan, Meng, Wang, Han, Li, Qiang, Mac Manus-Driscoll, Judith L., Lu, Ping, Zhang, Xinghang, & Wang, Haiyan. Three-dimensional strain engineering in epitaxial vertically aligned nanocomposite thin films with tunable magnetotransport properties. United Kingdom. https://doi.org/10.1039/C8MH00216A
Sun, Xing, Huang, Jijie, Jian, Jie, Fan, Meng, Wang, Han, Li, Qiang, Mac Manus-Driscoll, Judith L., Lu, Ping, Zhang, Xinghang, and Wang, Haiyan. Mon .
"Three-dimensional strain engineering in epitaxial vertically aligned nanocomposite thin films with tunable magnetotransport properties". United Kingdom. https://doi.org/10.1039/C8MH00216A.
@article{osti_1432400,
title = {Three-dimensional strain engineering in epitaxial vertically aligned nanocomposite thin films with tunable magnetotransport properties},
author = {Sun, Xing and Huang, Jijie and Jian, Jie and Fan, Meng and Wang, Han and Li, Qiang and Mac Manus-Driscoll, Judith L. and Lu, Ping and Zhang, Xinghang and Wang, Haiyan},
abstractNote = {Three-dimensional (3D) frameworks have been successfully constructed by interlayering La0.7Sr0.3MnO3 (LSMO)–CeO2 based epitaxial vertically aligned nanocomposite (VAN) thin films with pure CeO2 (or LSMO) layers. Such 3D interconnected CeO2 scaffolds integrate the lateral film strain by the interlayers with the vertical strain in VAN layers, and thus achieve the maximized strain tuning in LSMO. More importantly, by varying the types of the interlayers (i.e., CeO2 or LSMO) and the number of interlayers from 1 to 3 layers, such 3D framework nanostructures effectively tune the electrical transport properties of LSMO, e.g., from a 3D insulating CeO2 framework with integrated magnetic tunnel junction structures, to a 3D conducting LSMO framework, where the magnetoresistance (MR) peak values have been tuned systematically to a record high of 66% at 56 K and enhanced MR properties at high temperatures above room temperature (~325 K). This new 3D framed design provides a novel approach in maximizing film strain, enhancing strain-driven functionalities, and manipulating the electrical transport properties effectively.},
doi = {10.1039/C8MH00216A},
journal = {Materials Horizons},
number = 3,
volume = 5,
place = {United Kingdom},
year = {Mon Jan 01 00:00:00 EST 2018},
month = {Mon Jan 01 00:00:00 EST 2018}
}
https://doi.org/10.1039/C8MH00216A
Web of Science
Figures / Tables:
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