DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Ultrafast magnetization reversal by picosecond electrical pulses

Abstract

The field of spintronics involves the study of both spin and charge transport in solid-state devices. Ultrafast magnetism involves the use of femtosecond laser pulses to manipulate magnetic order on subpicosecond time scales. Here, we unite these phenomena by using picosecond charge current pulses to rapidly excite conduction electrons in magnetic metals. We observe deterministic, repeatable ultrafast reversal of the magnetization of a GdFeCo thin film with a single sub–10-ps electrical pulse. The magnetization reverses in ~10 ps, which is more than one order of magnitude faster than any other electrically controlled magnetic switching, and demonstrates a fundamentally new electrical switching mechanism that does not require spin-polarized currents or spin-transfer/orbit torques. The energy density required for switching is low, projecting to only 4 fJ needed to switch a (20 nm)3 cell. This discovery introduces a new field of research into ultrafast charge current–driven spintronic phenomena and devices.

Authors:
 [1];  [2];  [3];  [4];  [3]; ORCiD logo [3]
  1. Univ. of California, Berkeley, CA (United States). Dept. of Materials Science and Engineering
  2. Univ. of California, Riverside, CA (United States). Dept. of Materials Science and Engineering
  3. Univ. of California, Berkeley, CA (United States). Dept. of Electrical Engineering and Computer Sciences; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  4. Univ. of California, Berkeley, CA (United States). Dept. of Electrical Engineering and Computer Sciences
Publication Date:
Research Org.:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1432218
Grant/Contract Number:  
AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
Science Advances
Additional Journal Information:
Journal Volume: 3; Journal Issue: 11; Journal ID: ISSN 2375-2548
Publisher:
AAAS
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Yang, Yang, Wilson, Richard B., Gorchon, Jon, Lambert, Charles-Henri, Salahuddin, Sayeef, and Bokor, Jeffrey. Ultrafast magnetization reversal by picosecond electrical pulses. United States: N. p., 2017. Web. doi:10.1126/sciadv.1603117.
Yang, Yang, Wilson, Richard B., Gorchon, Jon, Lambert, Charles-Henri, Salahuddin, Sayeef, & Bokor, Jeffrey. Ultrafast magnetization reversal by picosecond electrical pulses. United States. https://doi.org/10.1126/sciadv.1603117
Yang, Yang, Wilson, Richard B., Gorchon, Jon, Lambert, Charles-Henri, Salahuddin, Sayeef, and Bokor, Jeffrey. Fri . "Ultrafast magnetization reversal by picosecond electrical pulses". United States. https://doi.org/10.1126/sciadv.1603117. https://www.osti.gov/servlets/purl/1432218.
@article{osti_1432218,
title = {Ultrafast magnetization reversal by picosecond electrical pulses},
author = {Yang, Yang and Wilson, Richard B. and Gorchon, Jon and Lambert, Charles-Henri and Salahuddin, Sayeef and Bokor, Jeffrey},
abstractNote = {The field of spintronics involves the study of both spin and charge transport in solid-state devices. Ultrafast magnetism involves the use of femtosecond laser pulses to manipulate magnetic order on subpicosecond time scales. Here, we unite these phenomena by using picosecond charge current pulses to rapidly excite conduction electrons in magnetic metals. We observe deterministic, repeatable ultrafast reversal of the magnetization of a GdFeCo thin film with a single sub–10-ps electrical pulse. The magnetization reverses in ~10 ps, which is more than one order of magnitude faster than any other electrically controlled magnetic switching, and demonstrates a fundamentally new electrical switching mechanism that does not require spin-polarized currents or spin-transfer/orbit torques. The energy density required for switching is low, projecting to only 4 fJ needed to switch a (20 nm)3 cell. This discovery introduces a new field of research into ultrafast charge current–driven spintronic phenomena and devices.},
doi = {10.1126/sciadv.1603117},
journal = {Science Advances},
number = 11,
volume = 3,
place = {United States},
year = {Fri Nov 03 00:00:00 EDT 2017},
month = {Fri Nov 03 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 91 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Crystallographically amorphous ferrimagnetic alloys: Comparing a localized atomistic spin model with experiments
journal, July 2011


Spintronics: Fundamentals and applications
journal, April 2004


Transient ferromagnetic-like state mediating ultrafast reversal of antiferromagnetically coupled spins
journal, March 2011


Spin-Torque Switching with the Giant Spin Hall Effect of Tantalum
journal, May 2012


Novel STT-MTJ Device Enabling All-Metallic Logic Circuits
journal, November 2012

  • Bromberg, David M.; Morris, Daniel H.; Pileggi, Larry
  • IEEE Transactions on Magnetics, Vol. 48, Issue 11
  • DOI: 10.1109/TMAG.2012.2197186

Low Energy Magnetic Domain Wall Logic in Short, Narrow, Ferromagnetic Wires
journal, January 2012


All-optical magnetization reversal by circularly polarized laser pulses: Experiment and multiscale modeling
journal, March 2012


Characteristics of coplanar transmission lines on multilayer substrates: modeling and experiments
journal, June 1997

  • Erli Chen, ; Chou, S. Y.
  • IEEE Transactions on Microwave Theory and Techniques, Vol. 45, Issue 6
  • DOI: 10.1109/22.588606

Femtosecond control of electric currents in metallic ferromagnetic heterostructures
journal, February 2016

  • Huisman, T. J.; Mikhaylovskiy, R. V.; Costa, J. D.
  • Nature Nanotechnology, Vol. 11, Issue 5
  • DOI: 10.1038/nnano.2015.331

Ultrafast precessional magnetization reversal by picosecond magnetic field pulse shaping
journal, August 2002

  • Gerrits, Th.; van den Berg, H. A. M.; Hohlfeld, J.
  • Nature, Vol. 418, Issue 6897
  • DOI: 10.1038/nature00905

Subpicosecond carrier lifetime in GaAs grown by molecular beam epitaxy at low temperatures
journal, December 1991

  • Gupta, S.; Frankel, M. Y.; Valdmanis, J. A.
  • Applied Physics Letters, Vol. 59, Issue 25
  • DOI: 10.1063/1.105729

All-Optical Switching of Magnetic Tunnel Junctions with Single Subpicosecond Laser Pulses
journal, February 2017


Spin-orbit torques in ferrimagnetic GdFeCo alloys
journal, September 2016

  • Roschewsky, Niklas; Matsumura, Tomoya; Cheema, Suraj
  • Applied Physics Letters, Vol. 109, Issue 11
  • DOI: 10.1063/1.4962812

Electron diffusion in metals studied by picosecond ultrasonics
journal, June 1994


Role of Magnetic Circular Dichroism in All-Optical Magnetic Recording
journal, March 2012


Ultrafast magnetization switching by spin-orbit torques
journal, November 2014

  • Garello, Kevin; Avci, Can Onur; Miron, Ioan Mihai
  • Applied Physics Letters, Vol. 105, Issue 21
  • DOI: 10.1063/1.4902443

Ultrafast optical manipulation of magnetic order
journal, September 2010


Effect of resistance-area product on spin-transfer switching in MgO-based magnetic tunnel junction memory cells
journal, February 2011

  • Zeng, Z. M.; Khalili Amiri, P.; Rowlands, G.
  • Applied Physics Letters, Vol. 98, Issue 7
  • DOI: 10.1063/1.3556615

Electric current induced ultrafast demagnetization
journal, July 2017


Deep subnanosecond spin torque switching in magnetic tunnel junctions with combined in-plane and perpendicular polarizers
journal, March 2011

  • Rowlands, G. E.; Rahman, T.; Katine, J. A.
  • Applied Physics Letters, Vol. 98, Issue 10
  • DOI: 10.1063/1.3565162

Fast magnetization reversal of GdFeCo induced by femtosecond laser pulses
journal, December 2001


Ultrafast magnetic switching of GdFeCo with electronic heat currents
journal, May 2017


Athermal all-optical femtosecond magnetization reversal in GdFeCo
journal, April 2009

  • Hohlfeld, J.; Stanciu, C. D.; Rebei, A.
  • Applied Physics Letters, Vol. 94, Issue 15
  • DOI: 10.1063/1.3119313

Ultrafast switching in magnetic tunnel junction based orthogonal spin transfer devices
journal, December 2010

  • Liu, H.; Bedau, D.; Backes, D.
  • Applied Physics Letters, Vol. 97, Issue 24
  • DOI: 10.1063/1.3527962

A 45nm Logic Technology with High-k+Metal Gate Transistors, Strained Silicon, 9 Cu Interconnect Layers, 193nm Dry Patterning, and 100% Pb-free Packaging
conference, December 2007


All-Optical Magnetic Recording with Circularly Polarized Light
journal, July 2007


Role of electron and phonon temperatures in the helicity-independent all-optical switching of GdFeCo
journal, November 2016


Symmetry and magnitude of spin–orbit torques in ferromagnetic heterostructures
journal, July 2013

  • Garello, Kevin; Miron, Ioan Mihai; Avci, Can Onur
  • Nature Nanotechnology, Vol. 8, Issue 8
  • DOI: 10.1038/nnano.2013.145

Landau-Lifshitz-Bloch equation for ferrimagnetic materials
journal, September 2012


Proposal for an all-spin logic device with built-in memory
journal, February 2010

  • Behin-Aein, Behtash; Datta, Deepanjan; Salahuddin, Sayeef
  • Nature Nanotechnology, Vol. 5, Issue 4
  • DOI: 10.1038/nnano.2010.31

The Promise of Nanomagnetics and Spintronics for Future Logic and Universal Memory
journal, December 2010


Ultrafast heating as a sufficient stimulus for magnetization reversal in a ferrimagnet
journal, January 2012

  • Ostler, T. A.; Barker, J.; Evans, R. F. L.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms1666

Generation of subpicosecond electrical pulses on coplanar transmission lines
journal, March 1986

  • Ketchen, M. B.; Grischkowsky, D.; Chen, T. C.
  • Applied Physics Letters, Vol. 48, Issue 12
  • DOI: 10.1063/1.96709

Terahertz spin current pulses controlled by magnetic heterostructures
journal, March 2013

  • Kampfrath, T.; Battiato, M.; Maldonado, P.
  • Nature Nanotechnology, Vol. 8, Issue 4
  • DOI: 10.1038/nnano.2013.43

All-optical magnetization recording by tailoring optical excitation parameters
journal, December 2011


APPLIED PHYSICS: Toward a Universal Memory
journal, April 2005


Sub-200 ps spin transfer torque switching in in-plane magnetic tunnel junctions with interface perpendicular anisotropy
journal, December 2011


Spintronics: fundamentals and applications
text, January 2004

  • Zutic, Igor; Fabian, Jaroslav; Sarma, S. Das
  • Universität Regensburg
  • DOI: 10.5283/epub.1823

Athermal All-Optical Femtosecond Magnetization Reversal in GdFeCo
text, January 2009


The Landau-Lifshitz-Bloch equation for ferrimagnetic materials
text, January 2012


Spin-Orbit Torques in ferrimagnetic GdFeCo Alloys
text, January 2016


Electric Current Induced Ultrafast Demagnetization
text, January 2016


Ultrafast Magnetic Switching of GdFeCo with Electronic Heat Currents
text, January 2016


Ultrafast precessional magnetization reversal by picosecond magnetic field pulse shaping
journal, August 2002

  • Gerrits, Th.; van den Berg, H. A. M.; Hohlfeld, J.
  • Nature, Vol. 418, Issue 6897
  • DOI: 10.1038/nature00905

Transient ferromagnetic-like state mediating ultrafast reversal of antiferromagnetically coupled spins
journal, March 2011


Ultrafast heating as a sufficient stimulus for magnetization reversal in a ferrimagnet
journal, January 2012

  • Ostler, T. A.; Barker, J.; Evans, R. F. L.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms1666

Proposal for an all-spin logic device with built-in memory
journal, February 2010

  • Behin-Aein, Behtash; Datta, Deepanjan; Salahuddin, Sayeef
  • Nature Nanotechnology, Vol. 5, Issue 4
  • DOI: 10.1038/nnano.2010.31

Terahertz spin current pulses controlled by magnetic heterostructures
journal, March 2013

  • Kampfrath, T.; Battiato, M.; Maldonado, P.
  • Nature Nanotechnology, Vol. 8, Issue 4
  • DOI: 10.1038/nnano.2013.43

Femtosecond control of electric currents in metallic ferromagnetic heterostructures
journal, February 2016

  • Huisman, T. J.; Mikhaylovskiy, R. V.; Costa, J. D.
  • Nature Nanotechnology, Vol. 11, Issue 5
  • DOI: 10.1038/nnano.2015.331

Electron thermalization in gold
journal, November 1992


Interplay of heating and helicity in all-optical magnetization switching
journal, March 2012


Ultrafast Spin Dynamics in Ferromagnetic Nickel
journal, May 1996


Subpicosecond Magnetization Reversal across Ferrimagnetic Compensation Points
journal, November 2007


Spin-Torque Switching with the Giant Spin Hall Effect of Tantalum
journal, May 2012


Symmetry and magnitude of spin-orbit torques in ferromagnetic heterostructures
text, January 2013


Spin-Orbit Torques in ferrimagnetic GdFeCo Alloys
text, January 2016


Works referencing / citing this record:

Single-Shot Multi-Level All-Optical Magnetization Switching Mediated by Spin Transport
journal, October 2018


Quantum Landauer erasure with a molecular nanomagnet
journal, March 2018


Beyond CMOS computing with spin and polarization
journal, April 2018


Forming individual magnetic biskyrmions by merging two skyrmions in a centrosymmetric nanodisk
journal, July 2019


Electrical writing, deleting, reading, and moving of magnetic skyrmioniums in a racetrack device
journal, August 2019


Giant localised spin-Peltier effect due to ultrafast domain wall motion in antiferromagnetic metals
journal, February 2020


Ultrafast double magnetization switching in GdFeCo with two picosecond-delayed femtosecond pump pulses
journal, August 2018

  • Atxitia, U.; Ostler, T. A.
  • Applied Physics Letters, Vol. 113, Issue 6
  • DOI: 10.1063/1.5044272

Artifact-free optical spin–orbit torque magnetometry
journal, May 2019

  • Kim, Joo-Sung; Park, Yong-Keun; Whang, Hyun-Seok
  • Applied Physics Letters, Vol. 114, Issue 18
  • DOI: 10.1063/1.5087743

Ultrafast spin dynamics in ferrimagnets with compensation point
journal, October 2019

  • Davydova, M. D.; Zvezdin, K. A.; Kimel, A. V.
  • Journal of Physics: Condensed Matter, Vol. 32, Issue 1
  • DOI: 10.1088/1361-648x/ab42fa

From single to multiple pulse all-optical switching in GdFeCo thin films
journal, August 2019


Finite-size effects in ultrafast remagnetization dynamics of FePt
journal, December 2019


Anomalously Damped Heat-Assisted Route for Precessional Magnetization Reversal in an Iron Garnet
journal, January 2019


Giant localised spin-Peltier effect due to ultrafast domain wall motion in antiferromagnetic metals
text, January 2020

  • Otxoa, R. M.; Atxitia, U.; Roy, P. E.
  • Apollo - University of Cambridge Repository
  • DOI: 10.17863/cam.64952

Giant localised spin-Peltier effect due to ultrafast domain wall motion in antiferromagnetic metals
text, January 2020

  • Otxoa, R. M.; Atxitia, U.; Roy, P. E.
  • Apollo - University of Cambridge Repository
  • DOI: 10.17863/cam.64335

Electrical writing, deleting, reading, and moving of magnetic skyrmioniums in a racetrack device
text, January 2019


Forming individual magnetic biskyrmions by merging two skyrmions in a centrosymmetric nanodisk
text, January 2019


Finite size effects on the ultrafast remagnetization dynamics of FePt
text, January 2019


Optically Tunable Magnetoresistance Effect: From Mechanism to Novel Device Application
journal, December 2017


Understanding all-optical spin switching: Comparison between experiment and theory
text, January 2018


Electrical writing, deleting, reading, and moving of magnetic skyrmioniums in a racetrack device
text, January 2019