skip to main content
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Time-resolved ion imaging at free-electron lasers using TimepixCam

Abstract

In this paper, the application of a novel fast optical-imaging camera, TimepixCam, to molecular photoionization experiments using the velocity-map imaging technique at a free-electron laser is described. TimepixCam is a 256 × 256 pixel CMOS camera that is able to detect and time-stamp ion hits with 20 ns timing resolution, thus making it possible to record ion momentum images for all fragment ions simultaneously and avoiding the need to gate the detector on a single fragment. This allows the recording of significantly more data within a given amount of beam time and is particularly useful for pump–probe experiments, where drifts, for example, in the timing and pulse energy of the free-electron laser, severely limit the comparability of pump–probe scans for different fragments taken consecutively. Finally, in principle, this also allows ion–ion covariance or coincidence techniques to be applied to determine angular correlations between fragments.

Authors:
 [1];  [2];  [3];  [4];  [4];  [4];  [5];  [6];  [3]
+ Show Author Affiliations
  1. Brookhaven National Lab. (BNL), Upton, NY (United States); Princeton Univ., NJ (United States)
  2. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); European X-ray Free-Electron Laser (XFEL), Hamburg (Germany)
  3. Kansas State Univ., Manhattan, KS (United States). J. R. Macdonald Lab. Dept. of Physics
  4. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  5. CNRS Lab. of Physical Chemistry - Matter and Radiation (LCPMR), Paris (France)
  6. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Research Org.:
Kansas State Univ., Manhattan, KS (United States); Brookhaven National Lab. (BNL), Upton, NY (United States); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); BNL Laboratory Directed Research and Development (LDRD) Program; Helmholtz Association of German Research Centres
OSTI Identifier:
1430839
Report Number(s):
BNL-203364-2018-JAAM
Journal ID: ISSN 1600-5775; TRN: US1802624
Grant/Contract Number:  
SC0012704; FG02-86ER13491
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Synchrotron Radiation (Online)
Additional Journal Information:
Journal Name: Journal of Synchrotron Radiation (Online); Journal Volume: 25; Journal Issue: 2; Journal ID: ISSN 1600-5775
Publisher:
International Union of Crystallography
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; time-stamping camera; velocity map imaging; VMI; free-electron laser; FEL; ultrafast laser; pump-probe experiments; mass spectrometry

Citation Formats

Fisher-Levine, Merlin, Boll, Rebecca, Ziaee, Farzaneh, Bomme, Cedric, Erk, Benjamin, Rompotis, Dimitrios, Marchenko, Tatiana, Nomerotski, Andrei, and Rolles, Daniel. Time-resolved ion imaging at free-electron lasers using TimepixCam. United States: N. p., 2018. Web. doi:10.1107/S1600577517018306.
Copy to clipboard
Fisher-Levine, Merlin, Boll, Rebecca, Ziaee, Farzaneh, Bomme, Cedric, Erk, Benjamin, Rompotis, Dimitrios, Marchenko, Tatiana, Nomerotski, Andrei, & Rolles, Daniel. Time-resolved ion imaging at free-electron lasers using TimepixCam. United States. doi:10.1107/S1600577517018306.
Copy to clipboard
Fisher-Levine, Merlin, Boll, Rebecca, Ziaee, Farzaneh, Bomme, Cedric, Erk, Benjamin, Rompotis, Dimitrios, Marchenko, Tatiana, Nomerotski, Andrei, and Rolles, Daniel. Tue . "Time-resolved ion imaging at free-electron lasers using TimepixCam". United States. doi:10.1107/S1600577517018306. https://www.osti.gov/servlets/purl/1430839.
Copy to clipboard
@article{osti_1430839,
title = {Time-resolved ion imaging at free-electron lasers using TimepixCam},
author = {Fisher-Levine, Merlin and Boll, Rebecca and Ziaee, Farzaneh and Bomme, Cedric and Erk, Benjamin and Rompotis, Dimitrios and Marchenko, Tatiana and Nomerotski, Andrei and Rolles, Daniel},
abstractNote = {In this paper, the application of a novel fast optical-imaging camera, TimepixCam, to molecular photoionization experiments using the velocity-map imaging technique at a free-electron laser is described. TimepixCam is a 256 × 256 pixel CMOS camera that is able to detect and time-stamp ion hits with 20 ns timing resolution, thus making it possible to record ion momentum images for all fragment ions simultaneously and avoiding the need to gate the detector on a single fragment. This allows the recording of significantly more data within a given amount of beam time and is particularly useful for pump–probe experiments, where drifts, for example, in the timing and pulse energy of the free-electron laser, severely limit the comparability of pump–probe scans for different fragments taken consecutively. Finally, in principle, this also allows ion–ion covariance or coincidence techniques to be applied to determine angular correlations between fragments.},
doi = {10.1107/S1600577517018306},
journal = {Journal of Synchrotron Radiation (Online)},
number = 2,
volume = 25,
place = {United States},
year = {2018},
month = {2}
}
Copy to clipboard
Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI:  10.1107/S1600577517018306
Copyright Statement
Other availability
Search WorldCat Search WorldCat to find libraries that may hold this journal
Citation Metrics:
Cited by: 1 work
Citation information provided by
Web of Science
Save / Share:
Export Metadata
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.

Works referenced in this record:

Identification of absolute geometries of cis and trans molecular isomers by Coulomb Explosion Imaging
journal, December 2016

  • Ablikim, Utuq; Bomme, Cédric; Xiong, Hui
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep38202

Operation of a free-electron laser from the extreme ultraviolet to the water window
journal, June 2007

Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet
journal, September 2012

Two-colour pump–probe experiments with a twin-pulse-seed extreme ultraviolet free-electron laser
journal, September 2013

  • Allaria, E.; Bencivenga, F.; Borghes, R.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3476

Three-dimensional imaging of carbonyl sulfide and ethyl iodide photodissociation using the pixel imaging mass spectrometry camera
journal, October 2015

  • Amini, K.; Blake, S.; Brouard, M.
  • Review of Scientific Instruments, Vol. 86, Issue 10
  • DOI: 10.1063/1.4934544

Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera
journal, July 2017

  • Amini, Kasra; Boll, Rebecca; Lauer, Alexandra
  • The Journal of Chemical Physics, Vol. 147, Issue 1
  • DOI: 10.1063/1.4982220

Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses
journal, March 2016

  • Boll, Rebecca; Erk, Benjamin; Coffee, Ryan
  • Structural Dynamics, Vol. 3, Issue 4
  • DOI: 10.1063/1.4944344

Coulomb-explosion imaging of concurrent CH 2 BrI photodissociation dynamics
journal, October 2017

The generation, characterization and applications of broadband isolated attosecond pulses
journal, February 2014

Multimass Velocity-Map Imaging with the Pixel Imaging Mass Spectrometry (PImMS) Sensor: An Ultra-Fast Event-Triggered Camera for Particle Imaging
journal, November 2012

  • Clark, Andrew T.; Crooks, Jamie P.; Sedgwick, Iain
  • The Journal of Physical Chemistry A, Vol. 116, Issue 45
  • DOI: 10.1021/jp309860t

Cold Target Recoil Ion Momentum Spectroscopy: a ‘momentum microscope’ to view atomic collision dynamics
journal, June 2000

Development of experimental techniques for the characterization of ultrashort photon pulses of extreme ultraviolet free-electron lasers
journal, December 2014

  • Düsterer, S.; Rehders, M.; Al-Shemmary, A.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 17, Issue 12
  • DOI: 10.1103/PhysRevSTAB.17.120702

First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010

Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen
journal, September 1997

  • Eppink, André T. J. B.; Parker, David H.
  • Review of Scientific Instruments, Vol. 68, Issue 9
  • DOI: 10.1063/1.1148310

Imaging charge transfer in iodomethane upon x-ray photoabsorption
journal, July 2014

FLASH—the first soft x-ray free electron laser (FEL) user facility
journal, September 2010

TimepixCam: a fast optical imager with time-stamping
journal, March 2016

High photon flux table-top coherent extreme-ultraviolet source
journal, September 2014

A compact X-ray free-electron laser emitting in the sub-ångström region
journal, June 2012

PImMS, a fast event-triggered monolithic pixel detector with storage of multiple timestamps
journal, August 2012

Detection systems for mass spectrometry imaging: A perspective on novel developments with a focus on active pixel detectors: Detection systems for MSI
journal, December 2012

  • Jungmann, Julia H.; Heeren, Ron M. A.
  • Rapid Communications in Mass Spectrometry, Vol. 27, Issue 1
  • DOI: 10.1002/rcm.6418

Fast, High Resolution Mass Spectrometry Imaging Using a Medipix Pixelated Detector
journal, December 2010

  • Jungmann, Julia H.; MacAleese, Luke; Buijs, Ronald
  • Journal of the American Society for Mass Spectrometry, Vol. 21, Issue 12
  • DOI: 10.1016/j.jasms.2010.08.014

Timepix, a 65k programmable pixel readout chip for arrival time, energy and/or photon counting measurements
journal, October 2007

  • Llopart, X.; Ballabriga, R.; Campbell, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 581, Issue 1-2
  • DOI: 10.1016/j.nima.2007.08.079

Ion-ion coincidence imaging at high event rate using an in-vacuum pixel detector
journal, July 2017

  • Furch, Federico J.; Durá, Judith; Tremsin, Anton S.
  • The Journal of Chemical Physics, Vol. 147, Issue 1
  • DOI: 10.1063/1.4981126

Velocity map ion imaging applied to studies of molecular fragmentation with synchrotron radiation
journal, March 2007

  • Pešić, Z. D.; Rolles, D.; Perri, M.
  • Journal of Electron Spectroscopy and Related Phenomena, Vol. 155, Issue 1-3
  • DOI: 10.1016/j.elspec.2006.11.046

The attosecond nonlinear optics of bright coherent X-ray generation
journal, November 2010

The FLASH pump–probe laser system: Setup, characterization and optical beamlines
journal, April 2011

  • Redlin, H.; Al-Shemmary, A.; Azima, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 635, Issue 1
  • DOI: 10.1016/j.nima.2010.09.159

A velocity map imaging spectrometer for electron–ion and ion–ion coincidence experiments with synchrotron radiation
journal, August 2007

  • Rolles, D.; Pešić, Z. D.; Perri, M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 261, Issue 1-2
  • DOI: 10.1016/j.nimb.2007.04.186

Jitter-correction for IR/UV-XUV pump-probe experiments at the FLASH free-electron laser
journal, April 2017

  • Savelyev, Evgeny; Boll, Rebecca; Bomme, Cédric
  • New Journal of Physics, Vol. 19, Issue 4
  • DOI: 10.1088/1367-2630/aa652d

A compact free-electron laser for generating coherent radiation in the extreme ultraviolet region
journal, July 2008

Covariance imaging experiments using a pixel-imaging mass-spectrometry camera
journal, January 2014

Large-format, high-speed, X-ray pnCCDs combined with electron and ion imaging spectrometers in a multipurpose chamber for experiments at 4th generation light sources
journal, March 2010

  • Strüder, Lothar; Epp, Sascha; Rolles, Daniel
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 614, Issue 3
  • DOI: 10.1016/j.nima.2009.12.053

Photon Beam Transport and Scientific Instruments at the European XFEL
journal, June 2017

  • Tschentscher, Thomas; Bressler, Christian; Grünert, Jan
  • Applied Sciences, Vol. 7, Issue 6
  • DOI: 10.3390/app7060592

Recoil-ion and electron momentum spectroscopy: reaction-microscopes
journal, August 2003

Free-Electron Lasers: New Avenues in Molecular Physics and Photochemistry
journal, May 2012

SPIDR: a read-out system for Medipix3 & Timepix3
journal, December 2015

Coincidence velocity map imaging using Tpx3Cam, a time stamping optical camera with 1.5 ns timing resolution
journal, November 2017

  • Zhao, Arthur; van Beuzekom, Martin; Bouwens, Bram
  • Review of Scientific Instruments, Vol. 88, Issue 11
  • DOI: 10.1063/1.4996888
    [ × clear filter / sort ]

    Similar Records in DOE PAGES and OSTI.GOV collections: