Probing the localization of magnetic dichroism by atomic-size astigmatic and vortex electron beams
Abstract
We report localization of a magnetic dichroic signal on atomic columns in electron magnetic circular dichroism (EMCD), probed by beam distorted by four-fold astigmatism and electron vortex beam. With astigmatic probe, magnetic signal to noise ratio can be enhanced by blocking the intensity from the central part of probe. However, the simulations show that for atomic resolution magnetic measurements, vortex beam is a more effective probe, with much higher magnetic signal to noise ratio. For all considered beam shapes, the optimal SNR constrains the signal detection at low collection angles of approximately 6–8 mrad. Irrespective of the material thickness, the magnetic signal remains strongly localized within the probed atomic column with vortex beam, whereas for astigmatic probes, the magnetic signal originates mostly from the nearest neighbor atomic columns. Due to excellent signal localization at probing individual atomic columns, vortex beams are predicted to be a strong candidate for studying the crystal site specific magnetic properties, magnetic properties at interfaces, or magnetism arising from individual atomic impurities.
- Authors:
-
- Uppsala Univ. (Sweden). Dept. of Physics and Astronomy
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Uppsala Univ. (Sweden)
- Sponsoring Org.:
- USDOE Office of Science (SC); Swedish Research Council (SRC); Goran Gustafsson’s Foundation (Sweden); Carl Tryggers Foundation (Sweden)
- OSTI Identifier:
- 1427589
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 8; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; magnetic properties and materials; matter waves and particle beams
Citation Formats
Negi, Devendra Singh, Idrobo, Juan Carlos, and Rusz, Ján. Probing the localization of magnetic dichroism by atomic-size astigmatic and vortex electron beams. United States: N. p., 2018.
Web. doi:10.1038/s41598-018-22234-8.
Negi, Devendra Singh, Idrobo, Juan Carlos, & Rusz, Ján. Probing the localization of magnetic dichroism by atomic-size astigmatic and vortex electron beams. United States. https://doi.org/10.1038/s41598-018-22234-8
Negi, Devendra Singh, Idrobo, Juan Carlos, and Rusz, Ján. Mon .
"Probing the localization of magnetic dichroism by atomic-size astigmatic and vortex electron beams". United States. https://doi.org/10.1038/s41598-018-22234-8. https://www.osti.gov/servlets/purl/1427589.
@article{osti_1427589,
title = {Probing the localization of magnetic dichroism by atomic-size astigmatic and vortex electron beams},
author = {Negi, Devendra Singh and Idrobo, Juan Carlos and Rusz, Ján},
abstractNote = {We report localization of a magnetic dichroic signal on atomic columns in electron magnetic circular dichroism (EMCD), probed by beam distorted by four-fold astigmatism and electron vortex beam. With astigmatic probe, magnetic signal to noise ratio can be enhanced by blocking the intensity from the central part of probe. However, the simulations show that for atomic resolution magnetic measurements, vortex beam is a more effective probe, with much higher magnetic signal to noise ratio. For all considered beam shapes, the optimal SNR constrains the signal detection at low collection angles of approximately 6–8 mrad. Irrespective of the material thickness, the magnetic signal remains strongly localized within the probed atomic column with vortex beam, whereas for astigmatic probes, the magnetic signal originates mostly from the nearest neighbor atomic columns. Due to excellent signal localization at probing individual atomic columns, vortex beams are predicted to be a strong candidate for studying the crystal site specific magnetic properties, magnetic properties at interfaces, or magnetism arising from individual atomic impurities.},
doi = {10.1038/s41598-018-22234-8},
journal = {Scientific Reports},
number = ,
volume = 8,
place = {United States},
year = {Mon Mar 05 00:00:00 EST 2018},
month = {Mon Mar 05 00:00:00 EST 2018}
}
Web of Science
Works referenced in this record:
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Detection of magnetic circular dichroism using a transmission electron microscope
journal, May 2006
- Schattschneider, P.; Rubino, S.; Hébert, C.
- Nature, Vol. 441, Issue 7092
Magnetic measurements with atomic-plane resolution
journal, August 2016
- Rusz, Ján; Muto, Shunsuke; Spiegelberg, Jakob
- Nature Communications, Vol. 7, Issue 1
Quantitative analysis of magnetic spin and orbital moments from an oxidized iron (1 1 0) surface using electron magnetic circular dichroism
journal, August 2015
- Thersleff, Thomas; Rusz, Jan; Rubino, Stefano
- Scientific Reports, Vol. 5, Issue 1
Skyrmions on the track
journal, March 2013
- Fert, Albert; Cros, Vincent; Sampaio, João
- Nature Nanotechnology, Vol. 8, Issue 3
Toward Single Mode, Atomic Size Electron Vortex Beams
journal, May 2014
- Krivanek, Ondrej L.; Rusz, Jan; Idrobo, Juan-Carlos
- Microscopy and Microanalysis, Vol. 20, Issue 3
Aberrated electron probes for magnetic spectroscopy with atomic resolution: Theory and practical aspects
journal, March 2016
- Rusz, Ján; Idrobo, Juan Carlos
- Physical Review B, Vol. 93, Issue 10
The physical significance of the mixed dynamic form factor
journal, August 2000
- Schattschneider, P.; Nelhiebel, M.; Souchay, H.
- Micron, Vol. 31, Issue 4
A single-atom transistor
journal, February 2012
- Fuechsle, Martin; Miwa, Jill A.; Mahapatra, Suddhasatta
- Nature Nanotechnology, Vol. 7, Issue 4
Dynamic scattering of electron vortex beams – A Bloch wave analysis
journal, February 2015
- Mendis, B. G.
- Ultramicroscopy, Vol. 149
Experimental application of sum rules for electron energy loss magnetic chiral dichroism
journal, August 2007
- Calmels, L.; Houdellier, F.; Warot-Fonrose, B.
- Physical Review B, Vol. 76, Issue 6
Magnetic circular dichroism in EELS: Towards 10nm resolution
journal, April 2008
- Schattschneider, Peter; Hébert, Cécile; Rubino, Stefano
- Ultramicroscopy, Vol. 108, Issue 5
Sum rules for electron energy loss near edge spectra
journal, August 2007
- Rusz, Ján; Eriksson, Olle; Novák, Pavel
- Physical Review B, Vol. 76, Issue 6
Observation of room-temperature magnetic skyrmions and their current-driven dynamics in ultrathin metallic ferromagnets
journal, February 2016
- Woo, Seonghoon; Litzius, Kai; Krüger, Benjamin
- Nature Materials, Vol. 15, Issue 5
Dynamics and inertia of skyrmionic spin structures
journal, February 2015
- Büttner, Felix; Moutafis, C.; Schneider, M.
- Nature Physics, Vol. 11, Issue 3
Iron-Based Layered Superconductor La[O 1- x F x ]FeAs ( x = 0.05−0.12) with T c = 26 K
journal, March 2008
- Kamihara, Yoichi; Watanabe, Takumi; Hirano, Masahiro
- Journal of the American Chemical Society, Vol. 130, Issue 11
Nonlocality in Imaging
journal, May 2005
- Oxley, M. P.; Cosgriff, E. C.; Allen, L. J.
- Physical Review Letters, Vol. 94, Issue 20
Localization of magnetic circular dichroic spectra in transmission electron microscopy experiments with atomic plane resolution
journal, May 2017
- Rusz, Ján; Spiegelberg, Jakob; Muto, Shunsuke
- Physical Review B, Vol. 95, Issue 17
Elastic Scattering of Electron Vortex Beams in Magnetic Matter
journal, March 2016
- Edström, Alexander; Lubk, Axel; Rusz, Ján
- Physical Review Letters, Vol. 116, Issue 12
Boundaries for Efficient Use of Electron Vortex Beams to Measure Magnetic Properties
journal, September 2013
- Rusz, Ján; Bhowmick, Somnath
- Physical Review Letters, Vol. 111, Issue 10
Modified automatic term selection v2: A faster algorithm to calculate inelastic scattering cross-sections
journal, June 2017
- Rusz, Ján
- Ultramicroscopy, Vol. 177
Native defect induced charge and ferromagnetic spin ordering and coexisting electronic phases in CoO epitaxial thin film
journal, December 2015
- Negi, D. S.; Loukya, B.; Datta, R.
- Applied Physics Letters, Vol. 107, Issue 23
Real-space observation of a two-dimensional skyrmion crystal
journal, June 2010
- Yu, X. Z.; Onose, Y.; Kanazawa, N.
- Nature, Vol. 465, Issue 7300
Production and application of electron vortex beams
journal, September 2010
- Verbeeck, J.; Tian, H.; Schattschneider, P.
- Nature, Vol. 467, Issue 7313
Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals
journal, April 2017
- Gong, Cheng; Li, Lin; Li, Zhenglu
- Nature, Vol. 546, Issue 7657
Image Contrast And Localized Signal Selection Techniques
journal, September 1979
- Howie, A.
- Journal of Microscopy, Vol. 117, Issue 1
Atom size electron vortex beams with selectable orbital angular momentum
journal, April 2017
- Pohl, Darius; Schneider, Sebastian; Zeiger, Paul
- Scientific Reports, Vol. 7, Issue 1
Local electronic structure information contained in energy-filtered diffraction patterns
journal, August 2011
- Rusz, Ján; Rubino, Stefano; Eriksson, Olle
- Physical Review B, Vol. 84, Issue 6
Electron magnetic chiral dichroism in CrO2 thin films using monochromatic probe illumination in a transmission electron microscope
journal, November 2012
- Loukya, B.; Zhang, X.; Gupta, A.
- Journal of Magnetism and Magnetic Materials, Vol. 324, Issue 22
Delocalization of the effective interaction for inner-shell ionization in crystals
journal, February 1998
- Oxley, M. P.; Allen, L. J.
- Physical Review B, Vol. 57, Issue 6
Unwinding of a Skyrmion Lattice by Magnetic Monopoles
journal, May 2013
- Milde, P.; Kohler, D.; Seidel, J.
- Science, Vol. 340, Issue 6136
Localization in elastic and inelastic scattering
journal, September 2003
- Lupini, A. R.; Pennycook, S. J.
- Ultramicroscopy, Vol. 96, Issue 3-4
Mapping inelastic intensities in diffraction patterns of magnetic samples using the energy spectrum imaging technique
journal, April 2008
- Warot-Fonrose, B.; Houdellier, F.; Hÿtch, M. J.
- Ultramicroscopy, Vol. 108, Issue 5
Electron vortex beams prepared by a spiral aperture with the goal to measure EMCD on ferromagnetic films via STEM
journal, March 2015
- Pohl, Darius; Schneider, Sebastian; Rusz, Jan
- Ultramicroscopy, Vol. 150
Quantitative experimental determination of site-specific magnetic structures by transmitted electrons
journal, January 2013
- Wang, Z. Q.; Zhong, X. Y.; Yu, R.
- Nature Communications, Vol. 4, Issue 1
A pure state decomposition approach of the mixed dynamic form factor for mapping atomic orbitals
journal, August 2013
- Löffler, S.; Motsch, V.; Schattschneider, P.
- Ultramicroscopy, Vol. 131
Spontaneous atomic-scale magnetic skyrmion lattice in two dimensions
journal, July 2011
- Heinze, Stefan; von Bergmann, Kirsten; Menzel, Matthias
- Nature Physics, Vol. 7, Issue 9
Effect of Bloch wave electron propagation and momentum-resolved signal detection on the quantitative and site-specific electron magnetic chiral dichroism of magnetic spinel oxide thin films
journal, April 2015
- Loukya, B.; Negi, D. S.; Dileep, K.
- Physical Review B, Vol. 91, Issue 13
Molecular spintronics using single-molecule magnets
journal, March 2008
- Bogani, Lapo; Wernsdorfer, Wolfgang
- Nature Materials, Vol. 7, Issue 3
Giant magnetoresistance in oxypnictides (La,Nd)OMnAs
journal, January 2010
- Emery, Nicolas; Wildman, Eve J.; Skakle, Janet M. S.
- Chemical Communications, Vol. 46, Issue 36
Observation of Skyrmions in a Multiferroic Material
journal, April 2012
- Seki, S.; Yu, X. Z.; Ishiwata, S.
- Science, Vol. 336, Issue 6078
Scattering of electron vortex beams on a magnetic crystal: Towards atomic-resolution magnetic measurements
journal, April 2014
- Rusz, Ján; Bhowmick, Somnath; Eriksson, Mattias
- Physical Review B, Vol. 89, Issue 13
Atomic scale electron vortices for nanoresearch
journal, November 2011
- Verbeeck, J.; Schattschneider, P.; Lazar, S.
- Applied Physics Letters, Vol. 99, Issue 20
Quantitative characterization of nanoscale polycrystalline magnets with electron magnetic circular dichroism
journal, January 2014
- Muto, Shunsuke; Rusz, Ján; Tatsumi, Kazuyoshi
- Nature Communications, Vol. 5, Issue 1
Mapping spin-polarized transitions with atomic resolution
journal, April 2012
- Schattschneider, P.; Schaffer, B.; Ennen, I.
- Physical Review B, Vol. 85, Issue 13
Atomic-Resolution Electron Energy Loss Spectroscopy Imaging in Aberration Corrected Scanning Transmission Electron Microscopy
journal, September 2003
- Allen, L. J.; Findlay, S. D.; Lupini, A. R.
- Physical Review Letters, Vol. 91, Issue 10
EMCD with an electron vortex filter: Limitations and possibilities
journal, August 2017
- Schachinger, T.; Löffler, S.; Steiger-Thirsfeld, A.
- Ultramicroscopy, Vol. 179
Single-layer MoS2 transistors
journal, January 2011
- Radisavljevic, B.; Radenovic, A.; Brivio, J.
- Nature Nanotechnology, Vol. 6, Issue 3, p. 147-150
Electron Vortex Beams with High Quanta of Orbital Angular Momentum
journal, January 2011
- McMorran, B. J.; Agrawal, A.; Anderson, I. M.
- Science, Vol. 331, Issue 6014, p. 192-195
New algorithm for efficient Bloch-waves calculations of orientation-sensitive ELNES
journal, February 2013
- Rusz, Ján; Muto, Shunsuke; Tatsumi, Kazuyoshi
- Ultramicroscopy, Vol. 125
On the electron vortex beam wavefunction within a crystal
journal, October 2015
- Mendis, B. G.
- Ultramicroscopy, Vol. 157
Achieving Atomic Resolution Magnetic Dichroism by Controlling the Phase Symmetry of an Electron Probe
journal, September 2014
- Rusz, Ján; Idrobo, Juan-Carlos; Bhowmick, Somnath
- Physical Review Letters, Vol. 113, Issue 14
An in-plane magnetic chiral dichroism approach for measurement of intrinsic magnetic signals using transmitted electrons
journal, May 2017
- Song, Dongsheng; Tavabi, Amir H.; Li, Zi-An
- Nature Communications, Vol. 8, Issue 1
Single-atom electron energy loss spectroscopy of light elements
journal, July 2015
- Senga, Ryosuke; Suenaga, Kazu
- Nature Communications, Vol. 6, Issue 1
Detecting magnetic ordering with atomic size electron probes
journal, May 2016
- Idrobo, Juan Carlos; Rusz, Ján; Spiegelberg, Jakob
- Advanced Structural and Chemical Imaging, Vol. 2, Issue 1
Discovery of Intrinsic Ferromagnetism in Two-Dimensional van der Waals Crystals
conference, January 2017
- Gong, Cheng; Li, Lin; Li, Zhenglu
- CLEO: Applications and Technology, Conference on Lasers and Electro-Optics
Detection of magnetic circular dichroism on the two-nanometer scale
text, January 2008
- Schattschneider, Peter; Stöger-Pollach, Michael; Rubino, Stefano
- Universität Regensburg
An in-plane magnetic chiral dichroism approach for measurement of intrinsic magnetic signals using transmitted electrons
text, January 2017
- Song, Dongsheng; Tavabi, Amir H.; Li, Zi-An
- Karlsruhe
Mapping spin-polarised transitions with atomic resolution
text, January 2011
- Schattschneider, Peter; Schaffer, Bernhard; Ennen, Inga
- arXiv
A pure state decomposition approach of the mixed dynamic form factor for mapping atomic orbitals
text, January 2012
- Löffler, Stefan; Motsch, Viktoria; Schattschneider, Peter
- arXiv
Achieving atomic resolution magnetic dichroism by controlling the phase symmetry of an electron probe
text, January 2014
- Rusz, Jan; Idrobo, Juan-Carlos; Bhowmick, Somnath
- arXiv
Quantitative analysis of magnetic spin and orbital moments from an oxidized iron (1 1 0) surface using electron magnetic circular dichroism
preprint, January 2015
- Thersleff, Thomas; Rusz, Jan; Rubino, Stefano
- arXiv
Elastic scattering of electron vortex beams in magnetic matter
text, January 2015
- Edström, Alexander; Lubk, Axel; Rusz, Ján
- arXiv
Magnetic circular dichroism in EELS: Towards 10 nm resolution
text, January 2007
- Schattschneider, Peter; Hébert, Cécile; Rubino, Stefano
- arXiv
Works referencing / citing this record:
Prospect for detecting magnetism of a single impurity atom using electron magnetic chiral dichroism
journal, September 2019
- Negi, Devendra; Zeiger, Paul M.; Jones, Lewys
- Physical Review B, Vol. 100, Issue 10