Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures

Kalinin, Sergei V.; Kim, Yunseok; Fong, Dillon D.; Morozovska, Anna N.

doi:10.1088/1361-6633/aa915a

Title: Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures

Abstract

For over 70 years, ferroelectric materials have been one of the central research topics for condensed matter physics and material science, an interest driven both by fundamental science and applications. However, ferroelectric surfaces, the key component of ferroelectric films and nanostructures, still present a significant theoretical and even conceptual challenge. Indeed, stability of ferroelectric phase per se necessitates screening of polarization charge. At surfaces, this can lead to coupling between ferroelectric and semiconducting properties of material, or with surface (electro) chemistry, going well beyond classical models applicable for ferroelectric interfaces. In this paper, we summarize recent studies of surface-screening phenomena in ferroelectrics. We provide a brief overview of the historical understanding of the physics of ferroelectric surfaces, and existing theoretical models that both introduce screening mechanisms and explore the relationship between screening and relevant aspects of ferroelectric functionalities starting from phase stability itself. Given that the majority of ferroelectrics exist in multiple-domain states, we focus on local studies of screening phenomena using scanning probe microscopy techniques. We discuss recent studies of static and dynamic phenomena on ferroelectric surfaces, as well as phenomena observed under lateral transport, light, chemical, and pressure stimuli. Finally, we also note that the need for ionicmore »« less

Authors:

Kalinin, Sergei V. ^[1]; Kim, Yunseok ^[2]; Fong, Dillon D. ^[3]; Morozovska, Anna N. ^[4]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). The Center for Nanophase Materials Sciences
Sungkyunkwan Univ., Suwon (Korea, Republic of). School of Advanced Materials Science and Engineering
Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
National Academy of Sciences of Ukraine, Kyiv (Ukraine). Inst. of Physics

Publication Date:: 2018-01-25

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Sungkyunkwan Univ., Suwon (Korea, Republic of)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Research Foundation of Korea (NRF); Ministry of Science, ICT and Future Planning (MSIP) of Korea

OSTI Identifier:: 1427506

Grant/Contract Number:: AC02-06CH11357; AC05-00OR22725; 2014R1A4A1008474

Resource Type:: Accepted Manuscript

Journal Name:: Reports on Progress in Physics

Additional Journal Information:: Journal Volume: 81; Journal Issue: 3; Journal ID: ISSN 0034-4885

Publisher:: IOP Publishing

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; ferroelectrics; surface; scanning probe microscopy; chemical effects; light effects

Citation Formats


                    Kalinin, Sergei V., Kim, Yunseok, Fong, Dillon D., and Morozovska, Anna N.. Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures.  United States: N. p., 2018. 
Web.  doi:10.1088/1361-6633/aa915a.

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                    Kalinin, Sergei V., Kim, Yunseok, Fong, Dillon D., & Morozovska, Anna N.. Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures.  United States.  https://doi.org/10.1088/1361-6633/aa915a

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                    Kalinin, Sergei V., Kim, Yunseok, Fong, Dillon D., and Morozovska, Anna N.. Thu .  
"Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures".  United States.  https://doi.org/10.1088/1361-6633/aa915a.  https://www.osti.gov/servlets/purl/1427506.

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@article{osti_1427506,

  title        = {Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures},

  author       = {Kalinin, Sergei V. and Kim, Yunseok and Fong, Dillon D. and Morozovska, Anna N.},

  abstractNote = {For over 70 years, ferroelectric materials have been one of the central research topics for condensed matter physics and material science, an interest driven both by fundamental science and applications. However, ferroelectric surfaces, the key component of ferroelectric films and nanostructures, still present a significant theoretical and even conceptual challenge. Indeed, stability of ferroelectric phase per se necessitates screening of polarization charge. At surfaces, this can lead to coupling between ferroelectric and semiconducting properties of material, or with surface (electro) chemistry, going well beyond classical models applicable for ferroelectric interfaces. In this paper, we summarize recent studies of surface-screening phenomena in ferroelectrics. We provide a brief overview of the historical understanding of the physics of ferroelectric surfaces, and existing theoretical models that both introduce screening mechanisms and explore the relationship between screening and relevant aspects of ferroelectric functionalities starting from phase stability itself. Given that the majority of ferroelectrics exist in multiple-domain states, we focus on local studies of screening phenomena using scanning probe microscopy techniques. We discuss recent studies of static and dynamic phenomena on ferroelectric surfaces, as well as phenomena observed under lateral transport, light, chemical, and pressure stimuli. Finally, we also note that the need for ionic screening renders polarization switching a coupled physical–electrochemical process and discuss the non-trivial phenomena such as chaotic behavior during domain switching that stem from this.},

  doi          = {10.1088/1361-6633/aa915a},

  journal      = {Reports on Progress in Physics},

  number       = 3,

  volume       = 81,

  place        = {United States},

  year         = {2018},

  month        = {1}

}

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Title: Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures

Abstract

Citation Formats

Resistive switching mechanisms in random access memory devices incorporating transition metal oxides: TiO 2 , NiO and Pr 0.7 Ca 0.3 MnO 3 journal, May 2011

Applications of Modern Ferroelectrics journal, February 2007

Equilibrium and stability of polarization in ultrathin ferroelectric films with ionic surface compensation journal, August 2011

Memristive devices and systems journal, January 1976

Real versus Measured Surface Potentials in Scanning Kelvin Probe Microscopy journal, March 2008

Doping-Based Stabilization of the M2 Phase in Free-Standing VO 2 Nanostructures at Room Temperature journal, February 2012

Sketched oxide single-electron transistor journal, April 2011

High-resolution characterization of piezoelectric ceramics by ultrasonic scanning force microscopy techniques journal, October 2002

Surface potential of ferroelectric thin films investigated by scanning probe microscopy journal, January 1999

Formation of snowflake domains during fast cooling of lithium tantalate crystals journal, April 2016

A decade of piezoresponse force microscopy: progress, challenges, and opportunities journal, December 2006

Direct observation of ferroelectric field effect and vacancy-controlled screening at the BiFeO3/LaxSr1−xMnO3 interface journal, August 2014

Scanning Impedance Microscopy: From Impedance Spectra to Impedance Images journal, February 2002

Humidity effects on tip-induced polarization switching in lithium niobate journal, March 2014

Applications of semi-implicit Fourier-spectral method to phase field equations journal, February 1998

A neutron powder investigation of the high-temperature structure and phase transition in LiNbO 3 journal, August 1994

Scanning force microscopy of domain structure in ferroelectric thin films: imaging and control journal, September 1997

Kelvin Probe Force Microscopy of Periodic Ferroelectric Domain Structure in KTiOPO 4 Crystals journal, May 2002

High-sensitivity quantitative Kelvin probe microscopy by noncontact ultra-high-vacuum atomic force microscopy journal, July 1999

Direct Observation of Continuous Electric Dipole Rotation in Flux-Closure Domains in Ferroelectric Pb(Zr,Ti)O3 journal, March 2011

Scanned potential microscopy of edge and bulk currents in the quantum Hall regime journal, February 1999

Piezoresponse force spectroscopy of ferroelectric-semiconductor materials journal, December 2007

Modification and detection of domains on ferroelectric PZT films by scanning force microscopy journal, January 1994

Friction force microscopy study of a cleaved ferroelectric surface: Time and temperature dependence of the contrast, evidence of domain structure branching journal, May 1996

Ferroelectric triggering of carbon monoxide adsorption on lead zirco-titanate (001) surfaces journal, October 2016

Atomic-scale structure of the Sr Ti O 3 ( 001 ) − c ( 6 × 2 ) reconstruction: Experiments and first-principles calculations journal, July 2007

Origin of the ferroelectric domain contrast observed in lateral force microscopy journal, January 1998

Controlled Patterning of Ferroelectric Domains: Fundamental Concepts and Applications journal, August 2008

Chemical Force Microscopy journal, August 1997

Ferroelectric Properties of Very Thin Pb(Zr 0.4 Ti 0.6 )O 3 Film Determined by Kelvin Force Microscope journal, November 2002

Atomic and Electronic Structure of the BaTiO 3 /Fe Interface in Multiferroic Tunnel Junctions journal, December 2011

CuGaSe2 solar cell cross section studied by Kelvin probe force microscopy in ultrahigh vacuum journal, September 2002

Interface-induced phenomena in polarization response of ferroelectric thin films journal, September 2006

Nanoscale Quantitative Measurement of the Potential of Charged Nanostructures by Electrostatic and Kelvin Probe Force Microscopy: Unraveling Electronic Processes in Complex Materials journal, April 2010

Computational Method of Activation Energy of Thick Domain Walls journal, April 1979

Ferroelectric polarization effect on surface chemistry and photo-catalytic activity: A review journal, March 2016

Screening Phenomena on Oxide Surfaces and Its Implications for Local Electrostatic and Transport Measurements journal, April 2004

Nanoelectromechanics of piezoelectric indentation and applications to scanning probe microscopies of ferroelectric materials journal, April 2005

Polarization Dependence of Palladium Deposition on Ferroelectric Lithium Niobate (0001) Surfaces journal, August 2011

Scanning Near-Field Raman Microscopy on Ferroelectrics journal, January 2003

Temperature dependence of polarization and charge dynamics on the BaTiO3(100) surface by scanning probe microscopy journal, February 2001

Atomic Polarization and Local Reactivity on Ferroelectric Surfaces: A New Route toward Complex Nanostructures journal, June 2002

Surface potential decay on triglycine sulfate crystal journal, September 2005

Study of asymmetric charge writing on Pb(Zr,Ti)O3 thin films by Kelvin probe force microscopy journal, September 2006

Theoretical and Experimental Study on Nanoscale Ferroelectric Domain Measurement Using Scanning Nonlinear Dielectric Microscopy journal, September 2000

Extrinsic size effect in piezoresponse force microscopy of thin films journal, August 2007

Fractal-cluster kinetics in phase transformations in the relaxor ceramic PLZT journal, March 1999

Self-similar surface nanodomain structures induced by laser irradiation in lithium niobate journal, April 2008

Imaging mechanism of piezoresponse force microscopy of ferroelectric surfaces journal, March 2002

Ionic field effect and memristive phenomena in single-point ferroelectric domain switching journal, July 2014

Emergence of heterophase structures near phase transitions in photoferroelectric materials journal, April 1997

Direct Probing of Charge Injection and Polarization-Controlled Ionic Mobility on Ferroelectric LiNbO 3 Surfaces journal, November 2013

Polarization Effects on the Surface Chemistry of PbTiO 3 -Supported Pt Films journal, April 2007

The photogalvanic effect in media lacking a center of symmetry journal, March 1980

Screening and retardation effects on 180 ° -domain wall motion in ferroelectrics: Wall velocity and nonlinear dynamics due to polarization-screening charge interactions journal, December 2008

Electromechanical Detection in Scanning Probe Microscopy: Tip Models and Materials Contrast text, January 2006

Defect-mediated adsorption of methanol and carbon dioxide on BaTiO3(001) journal, September 2009

Time-resolved electrostatic force microscopy of polymer solar cells journal, August 2006

Self-assembled domain structures: From micro- to nanoscale journal, June 2015

Mechanically-Induced Resistive Switching in Ferroelectric Tunnel Junctions journal, February 2012

Electron emission from ferroelectrics - a review journal, February 1994

Surface Morphology of Ferroelectric Domains in B a T i O 3 Single Crystals: An Atomic Force Microscope Study journal, September 1997

Effect of local surface potential distribution on its relaxation in polycrystalline ferroelectric films journal, March 2010

Application of a sensitive catalytic reactor to the study of CO oxidation over SrTiO 3 (100) and BaTiO 3 /SrTiO 3 (100) ferroelectric surfaces : CO oxidation over SrTiO3(100) and BaTiO3/SrTiO3(100) surfaces journal, January 2014

Characterization of butterfly single crystals of by atomic force, optical and scanning electron microscopy techniques journal, October 1998

Ferroelectric properties of nano-size PZT grains determined by surface potential utilizing Kelvin force microscopy journal, October 2004

Temperature dependent surface images of several ferroic crystals observed by scanning probe microscopy journal, February 2001

Cross-Sectional Observation of Nano-Domain Dots Formed in Congruent Single-Crystal LiTaO 3 journal, December 2006

Ferroelectrics: A pathway to switchable surface chemistry and catalysis journal, August 2016

Formation of Broad Domain Boundary in Congruent Lithium Niobate Modified by Proton Exchange journal, February 2015

First-principles determination of chemical potentials and vacancy formation energies in Pb Ti O 3 and Ba Ti O 3 journal, December 2007

Tunable Metallic Conductance in Ferroelectric Nanodomains journal, December 2011

Electronic surface compensation of polarization in PbTiO3 films journal, September 2012

Effects of anisotropic elasticity in the problem of domain formation and stability of monodomain state in ferroelectric films journal, July 2011

Nanoscale electromechanics of paraelectric materials with mobile charges: Size effects and nonlinearity of electromechanical response of SrTiO 3 films journal, July 2011

TiO 2 —a prototypical memristive material journal, May 2011

Influence of carrier density on the friction properties of silicon p n junctions journal, August 2007

Resistive switching mechanisms in random access memory devices incorporating transition metal oxides: TiO ₂ , NiO and Pr _0.7 Ca _0.3 MnO ₃
journal, May 2011

Applications of Modern Ferroelectrics
journal, February 2007

Equilibrium and stability of polarization in ultrathin ferroelectric films with ionic surface compensation
journal, August 2011

Memristive devices and systems
journal, January 1976

Real versus Measured Surface Potentials in Scanning Kelvin Probe Microscopy
journal, March 2008

Doping-Based Stabilization of the M2 Phase in Free-Standing VO ₂ Nanostructures at Room Temperature
journal, February 2012

Sketched oxide single-electron transistor
journal, April 2011

High-resolution characterization of piezoelectric ceramics by ultrasonic scanning force microscopy techniques
journal, October 2002

Surface potential of ferroelectric thin films investigated by scanning probe microscopy
journal, January 1999

Formation of snowflake domains during fast cooling of lithium tantalate crystals
journal, April 2016

A decade of piezoresponse force microscopy: progress, challenges, and opportunities
journal, December 2006

Direct observation of ferroelectric field effect and vacancy-controlled screening at the BiFeO3/LaxSr1−xMnO3 interface
journal, August 2014

Scanning Impedance Microscopy: From Impedance Spectra to Impedance Images
journal, February 2002

Humidity effects on tip-induced polarization switching in lithium niobate
journal, March 2014

Applications of semi-implicit Fourier-spectral method to phase field equations
journal, February 1998

A neutron powder investigation of the high-temperature structure and phase transition in LiNbO ₃
journal, August 1994

Scanning force microscopy of domain structure in ferroelectric thin films: imaging and control
journal, September 1997

Kelvin Probe Force Microscopy of Periodic Ferroelectric Domain Structure in KTiOPO ₄ Crystals
journal, May 2002

High-sensitivity quantitative Kelvin probe microscopy by noncontact ultra-high-vacuum atomic force microscopy
journal, July 1999

Direct Observation of Continuous Electric Dipole Rotation in Flux-Closure Domains in Ferroelectric Pb(Zr,Ti)O3
journal, March 2011

Scanned potential microscopy of edge and bulk currents in the quantum Hall regime
journal, February 1999

Piezoresponse force spectroscopy of ferroelectric-semiconductor materials
journal, December 2007

Modification and detection of domains on ferroelectric PZT films by scanning force microscopy
journal, January 1994

Friction force microscopy study of a cleaved ferroelectric surface: Time and temperature dependence of the contrast, evidence of domain structure branching
journal, May 1996

Ferroelectric triggering of carbon monoxide adsorption on lead zirco-titanate (001) surfaces
journal, October 2016

Atomic-scale structure of the $Sr Ti O_{3} (001) − c (6 \times 2)$ reconstruction: Experiments and first-principles calculations
journal, July 2007

Origin of the ferroelectric domain contrast observed in lateral force microscopy
journal, January 1998

Controlled Patterning of Ferroelectric Domains: Fundamental Concepts and Applications
journal, August 2008

Chemical Force Microscopy
journal, August 1997

Ferroelectric Properties of Very Thin Pb(Zr _0.4 Ti _0.6 )O ₃ Film Determined by Kelvin Force Microscope
journal, November 2002

Atomic and Electronic Structure of the BaTiO ₃ /Fe Interface in Multiferroic Tunnel Junctions
journal, December 2011

CuGaSe2 solar cell cross section studied by Kelvin probe force microscopy in ultrahigh vacuum
journal, September 2002

Interface-induced phenomena in polarization response of ferroelectric thin films
journal, September 2006

Nanoscale Quantitative Measurement of the Potential of Charged Nanostructures by Electrostatic and Kelvin Probe Force Microscopy: Unraveling Electronic Processes in Complex Materials
journal, April 2010

Computational Method of Activation Energy of Thick Domain Walls
journal, April 1979

Ferroelectric polarization effect on surface chemistry and photo-catalytic activity: A review
journal, March 2016

Screening Phenomena on Oxide Surfaces and Its Implications for Local Electrostatic and Transport Measurements
journal, April 2004

Nanoelectromechanics of piezoelectric indentation and applications to scanning probe microscopies of ferroelectric materials
journal, April 2005

Polarization Dependence of Palladium Deposition on Ferroelectric Lithium Niobate (0001) Surfaces
journal, August 2011

Scanning Near-Field Raman Microscopy on Ferroelectrics
journal, January 2003

Temperature dependence of polarization and charge dynamics on the BaTiO3(100) surface by scanning probe microscopy
journal, February 2001

Atomic Polarization and Local Reactivity on Ferroelectric Surfaces: A New Route toward Complex Nanostructures
journal, June 2002

Surface potential decay on triglycine sulfate crystal
journal, September 2005

Study of asymmetric charge writing on Pb(Zr,Ti)O3 thin films by Kelvin probe force microscopy
journal, September 2006

Theoretical and Experimental Study on Nanoscale Ferroelectric Domain Measurement Using Scanning Nonlinear Dielectric Microscopy
journal, September 2000

Extrinsic size effect in piezoresponse force microscopy of thin films
journal, August 2007

Fractal-cluster kinetics in phase transformations in the relaxor ceramic PLZT
journal, March 1999

Self-similar surface nanodomain structures induced by laser irradiation in lithium niobate
journal, April 2008

Imaging mechanism of piezoresponse force microscopy of ferroelectric surfaces
journal, March 2002

Ionic field effect and memristive phenomena in single-point ferroelectric domain switching
journal, July 2014

Emergence of heterophase structures near phase transitions in photoferroelectric materials
journal, April 1997

Direct Probing of Charge Injection and Polarization-Controlled Ionic Mobility on Ferroelectric LiNbO ₃ Surfaces
journal, November 2013

Polarization Effects on the Surface Chemistry of ${PbTiO}_{3}$ -Supported Pt Films
journal, April 2007

The photogalvanic effect in media lacking a center of symmetry
journal, March 1980

Screening and retardation effects on $180 °$ -domain wall motion in ferroelectrics: Wall velocity and nonlinear dynamics due to polarization-screening charge interactions
journal, December 2008

Electromechanical Detection in Scanning Probe Microscopy: Tip Models and Materials Contrast
text, January 2006

Defect-mediated adsorption of methanol and carbon dioxide on BaTiO3(001)
journal, September 2009

Time-resolved electrostatic force microscopy of polymer solar cells
journal, August 2006

Self-assembled domain structures: From micro- to nanoscale
journal, June 2015

Mechanically-Induced Resistive Switching in Ferroelectric Tunnel Junctions
journal, February 2012

Electron emission from ferroelectrics - a review
journal, February 1994

Surface Morphology of Ferroelectric Domains in B a T i O ₃ Single Crystals: An Atomic Force Microscope Study
journal, September 1997

Effect of local surface potential distribution on its relaxation in polycrystalline ferroelectric films
journal, March 2010

Application of a sensitive catalytic reactor to the study of CO oxidation over SrTiO ₃ (100) and BaTiO ₃ /SrTiO ₃ (100) ferroelectric surfaces : CO oxidation over SrTiO3(100) and BaTiO3/SrTiO3(100) surfaces
journal, January 2014

Characterization of butterfly single crystals of by atomic force, optical and scanning electron microscopy techniques
journal, October 1998

Ferroelectric properties of nano-size PZT grains determined by surface potential utilizing Kelvin force microscopy
journal, October 2004

Temperature dependent surface images of several ferroic crystals observed by scanning probe microscopy
journal, February 2001

Cross-Sectional Observation of Nano-Domain Dots Formed in Congruent Single-Crystal LiTaO ₃
journal, December 2006

Ferroelectrics: A pathway to switchable surface chemistry and catalysis
journal, August 2016

Formation of Broad Domain Boundary in Congruent Lithium Niobate Modified by Proton Exchange
journal, February 2015

First-principles determination of chemical potentials and vacancy formation energies in $Pb Ti O_{3}$ and $Ba Ti O_{3}$
journal, December 2007

Tunable Metallic Conductance in Ferroelectric Nanodomains
journal, December 2011

Electronic surface compensation of polarization in PbTiO3 films
journal, September 2012

Effects of anisotropic elasticity in the problem of domain formation and stability of monodomain state in ferroelectric films
journal, July 2011

Nanoscale electromechanics of paraelectric materials with mobile charges: Size effects and nonlinearity of electromechanical response of SrTiO $_{3}$ films
journal, July 2011

TiO ₂ —a prototypical memristive material
journal, May 2011

Influence of carrier density on the friction properties of silicon $p n$ junctions
journal, August 2007

Influence of ferroelectric polarization on the energetics of the reaction of 2-fluoroethanol on BaTiO3
journal, January 2009

Polar distortion in ultrathin ${BaTiO}_{3}$ films studied by in situ LEED $I − V$
journal, June 2008

Soft X-ray photon stimulated ion desorption from SrTiO3(100)-H2O
journal, April 1994