Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures
Abstract
For over 70 years, ferroelectric materials have been one of the central research topics for condensed matter physics and material science, an interest driven both by fundamental science and applications. However, ferroelectric surfaces, the key component of ferroelectric films and nanostructures, still present a significant theoretical and even conceptual challenge. Indeed, stability of ferroelectric phase per se necessitates screening of polarization charge. At surfaces, this can lead to coupling between ferroelectric and semiconducting properties of material, or with surface (electro) chemistry, going well beyond classical models applicable for ferroelectric interfaces. In this paper, we summarize recent studies of surface-screening phenomena in ferroelectrics. We provide a brief overview of the historical understanding of the physics of ferroelectric surfaces, and existing theoretical models that both introduce screening mechanisms and explore the relationship between screening and relevant aspects of ferroelectric functionalities starting from phase stability itself. Given that the majority of ferroelectrics exist in multiple-domain states, we focus on local studies of screening phenomena using scanning probe microscopy techniques. We discuss recent studies of static and dynamic phenomena on ferroelectric surfaces, as well as phenomena observed under lateral transport, light, chemical, and pressure stimuli. Finally, we also note that the need for ionicmore »
- Authors:
-
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). The Center for Nanophase Materials Sciences
- Sungkyunkwan Univ., Suwon (Korea, Republic of). School of Advanced Materials Science and Engineering
- Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
- National Academy of Sciences of Ukraine, Kyiv (Ukraine). Inst. of Physics
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Sungkyunkwan Univ., Suwon (Korea, Republic of)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Research Foundation of Korea (NRF); Ministry of Science, ICT and Future Planning (MSIP) of Korea
- OSTI Identifier:
- 1427506
- Grant/Contract Number:
- AC02-06CH11357; AC05-00OR22725; 2014R1A4A1008474
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Reports on Progress in Physics
- Additional Journal Information:
- Journal Volume: 81; Journal Issue: 3; Journal ID: ISSN 0034-4885
- Publisher:
- IOP Publishing
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; ferroelectrics; surface; scanning probe microscopy; chemical effects; light effects
Citation Formats
Kalinin, Sergei V., Kim, Yunseok, Fong, Dillon D., and Morozovska, Anna N.. Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures. United States: N. p., 2018.
Web. doi:10.1088/1361-6633/aa915a.
Kalinin, Sergei V., Kim, Yunseok, Fong, Dillon D., & Morozovska, Anna N.. Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures. United States. https://doi.org/10.1088/1361-6633/aa915a
Kalinin, Sergei V., Kim, Yunseok, Fong, Dillon D., and Morozovska, Anna N.. Thu .
"Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures". United States. https://doi.org/10.1088/1361-6633/aa915a. https://www.osti.gov/servlets/purl/1427506.
@article{osti_1427506,
title = {Surface-screening mechanisms in ferroelectric thin films and their effect on polarization dynamics and domain structures},
author = {Kalinin, Sergei V. and Kim, Yunseok and Fong, Dillon D. and Morozovska, Anna N.},
abstractNote = {For over 70 years, ferroelectric materials have been one of the central research topics for condensed matter physics and material science, an interest driven both by fundamental science and applications. However, ferroelectric surfaces, the key component of ferroelectric films and nanostructures, still present a significant theoretical and even conceptual challenge. Indeed, stability of ferroelectric phase per se necessitates screening of polarization charge. At surfaces, this can lead to coupling between ferroelectric and semiconducting properties of material, or with surface (electro) chemistry, going well beyond classical models applicable for ferroelectric interfaces. In this paper, we summarize recent studies of surface-screening phenomena in ferroelectrics. We provide a brief overview of the historical understanding of the physics of ferroelectric surfaces, and existing theoretical models that both introduce screening mechanisms and explore the relationship between screening and relevant aspects of ferroelectric functionalities starting from phase stability itself. Given that the majority of ferroelectrics exist in multiple-domain states, we focus on local studies of screening phenomena using scanning probe microscopy techniques. We discuss recent studies of static and dynamic phenomena on ferroelectric surfaces, as well as phenomena observed under lateral transport, light, chemical, and pressure stimuli. Finally, we also note that the need for ionic screening renders polarization switching a coupled physical–electrochemical process and discuss the non-trivial phenomena such as chaotic behavior during domain switching that stem from this.},
doi = {10.1088/1361-6633/aa915a},
journal = {Reports on Progress in Physics},
number = 3,
volume = 81,
place = {United States},
year = {2018},
month = {1}
}
Web of Science
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