Hard-sphere-like dynamics in highly concentrated alpha-crystallin suspensions

Vodnala, Preeti; Karunaratne, Nuwan; Lurio, Laurence; Thurston, George M.; Vega, Michael; Gaillard, Elizabeth; Narayanan, Suresh; Sandy, Alec; Zhang, Qingteng; Dufresne, Eric M.; Foffi, Giuseppe; Grybos, Pawel; Kmon, Piotr; Maj, Piotr; Szczygiel, Robert

doi:10.1103/PhysRevE.97.020601

Title: Hard-sphere-like dynamics in highly concentrated alpha-crystallin suspensions

Journal Article · 02 February 2018 · Physical Review E

DOI: https://doi.org/10.1103/PhysRevE.97.020601 · OSTI ID:1427480

Vodnala, Preeti ^[1]; Karunaratne, Nuwan ^[1]; Lurio, Laurence ^[1]; Thurston, George M. ^[2]; Vega, Michael ^[1]; Gaillard, Elizabeth ^[1]; Narayanan, Suresh ^[3]; Sandy, Alec ^[3]; Zhang, Qingteng ^[3]; Dufresne, Eric M. ^[3]; Foffi, Giuseppe ^[4]; Grybos, Pawel ^[5]; Kmon, Piotr ^[5]; Maj, Piotr ^[5]; Szczygiel, Robert ^[5]

Northern Illinois Univ., DeKalb, IL (United States)
Rochester Inst. of Technology, Rochester, NY (United States)
Argonne National Lab. (ANL), Lemont, IL (United States)
Univ. Paris-Sud, Orsay (France)
AGH - Univ. of Science and Technology, Krakow (Poland)

The dynamics of concentrated suspensions of the eye-lens protein alpha crystallin have been measured using x-ray photon correlation spectroscopy. Measurements were made at wave vectors corresponding to the first peak in the hard-sphere structure factor and volume fractions close to the critical volume fraction for the glass transition. Langevin dynamics simulations were also performed in parallel to the experiments. The intermediate scattering function f(q,τ) could be fit using a stretched exponential decay for both experiments and numerical simulations. The measured relaxation times show good agreement with simulations for polydisperse hard-sphere colloids.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC); National Institutes of Health (NIH)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1427480

Alternate ID(s):: OSTI ID: 1419369

Journal Information:: Physical Review E, Vol. 97, Issue 2; ISSN 2470-0045

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 23 works

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