The Fabrication of All-Solid-State Lithium-Ion Batteries via Spark Plasma Sintering

Wei, Xialu; Rechtin, Jack; Olevsky, Eugene

doi:10.3390/met7090372

Title: The Fabrication of All-Solid-State Lithium-Ion Batteries via Spark Plasma Sintering

Journal Article · 14 September 2017 · Metals

DOI: https://doi.org/10.3390/met7090372 · OSTI ID:1426194

^[1]; Rechtin, Jack ^[1]; Olevsky, Eugene ^[2]

San Diego State Univ., CA (United States)
San Diego State Univ., CA (United States); Univ. of California, San Diego, CA (United States)

Spark plasma sintering (SPS) has been successfully used to produce all-solid-state lithium-ion batteries (ASSLibs). Both regular and functionally graded electrodes are implemented into novel three-layer and five-layer battery designs together with solid-state composite electrolyte. The electrical capacities and the conductivities of the SPS-processed ASSLibs are evaluated using the galvanostatic charge-discharge test. Experimental results have shown that, compared to the three-layer battery, the five-layer battery is able to improve energy and power densities. Scanning electron microscopy (SEM) is employed to examine the microstructures of the batteries especially at the electrode–electrolyte interfaces. It reveals that the functionally graded structure can eliminate the delamination effect at the electrode–electrolyte interface and, therefore, retains better performance.

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Research Organization:: San Diego State Univ., CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0008581

OSTI ID:: 1426194

Journal Information:: Metals, Vol. 7, Issue 12; ISSN 2075-4701

Publisher:: MDPICopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 21 works

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